In the field of nanoelectronics, one seeks to combine quantum mechanical effects with macroscopic entities such as currents in order to find new ways of storing and manipulating information. One possibility to accomplish this is to use the quantum correlations found in superconductors. Teaming superconductors with normal metals and magnetic systems, one can obtain novel correlation and fluctuation effects. \n\nIn the first work of this thesis, we examine how charge correlations in a metallic dot are modified due to the presence of a capacitively coupled superconducting island. It is possible to overcome the Coulomb repulsion between electrons in a hybrid double-dot system consisting of a metallic island coupled capacitively to a Cooper-pair box. The superconducting island S acts as a dynamic gate on the metallic island N and in the strong coupling regime the electric charge of the Cooper pairs in S and their fluctuations are able to overscreen the repulsion between electrons in N. This produces an attractive interaction between two additional electrons in the metallic island and results in a non-monotonous charging curve of the metallic island. \n\nThe second part of the thesis considers how the dynamics of a precessing molecular magnetic moment affects the Josephson current. The precession gives rise to a time-dependent tunnel potential which not only creates different tunneling probabilities for spin-up and spin-down quasiparticles, but also introduces a time-dependent spin-flip term. In particular, we study the effects of the spin-flip term alone on the Josephson current between two spin-singlet superconductors as a function of precession frequency and junction transparency. The system displays a nonequilibrium steady-state solution which depends on the precession frequency of the classical spin.\n\n\n
In the field of nanoelectronics, one seeks to combine quantum mechanical effects with macroscopic entities such as currents in order to find new ways of storing and manipulating information. One possibility to accomplish this is to use the quantum correlations found in superconductors. Teaming superconductors with normal metals and magnetic systems, one can obtain novel correlation and fluctuation effects. \n\nIn the first work of this thesis, we examine how charge correlations in a metallic dot are modified due to the presence of a capacitively coupled superconducting island. It is possible to overcome the Coulomb repulsion between electrons in a hybrid double-dot system consisting of a metallic island coupled capacitively to a Cooper-pair box. The superconducting island S acts as a dynamic gate on the metallic island N and in the strong coupling regime the electric charge of the Cooper pairs in S and their fluctuations are able to overscreen the repulsion between electrons in N. This produces an attractive interaction between two additional electrons in the metallic island and results in a non-monotonous charging curve of the metallic island. \n\nThe second part of the thesis considers how the dynamics of a precessing molecular magnetic moment affects the Josephson current. The precession gives rise to a time-dependent tunnel potential which not only creates different tunneling probabilities for spin-up and spin-down quasiparticles, but also introduces a time-dependent spin-flip term. In particular, we study the effects of the spin-flip term alone on the Josephson current between two spin-singlet superconductors as a function of precession frequency and junction transparency. The system displays a nonequilibrium steady-state solution which depends on the precession frequency of the classical spin.\n\n\n
We consider the hybrid setup formed by a metallic dot, capacitively coupled to a superconducting island S connected to a bulk superconductor by a Josephson junction. Charge fluctuations in S act as a dynamical gate and overscreen the electronic repulsion in the metallic dot, producing an attractive interaction between two additional electrons. As the offset charge of the metallic dot is increased, the dot charging curve shows charge-skipping positive steps $(+2\ensuremath{\mid}e\ensuremath{\mid})$ followed by negative ones $(\ensuremath{-}\ensuremath{\mid}e\ensuremath{\mid})$ signaling the occurrence of a negative differential capacitance. A necessary condition for such an effect is that the capacitance coupling the two islands should be larger than the Josephson junction capacitance. A proposal for experimental detection is given, and potential applications in nanoelectronics are outlined.
The work presented in this thesis investigates transitions between quantum states in superconducting double dots (SDDs), a nanoscale device consisting of two aluminium superconducting islands coupled together by a Josephson junction, with each dot connected to a normal state lead. The energy landscape consists of a two level manifold of even charge parity Cooper pair states, and continuous bands corresponding to charge states with single quasiparticles in one or both islands. These devices are fabricated using shadow mask evaporation, and are measured at sub Kelvin temperatures using a dilution refrigerator. We use radio frequency reflectometry to measure quantum capacitance, which is dependent on the quantum state of the device. We measure the quantum capacitance as a function of gate voltage, and observe capacitance maxima corresponding to the Josephson coupling between even parity states. We also perform charge sensing and detect odd parity states. These measurements support the theoretical model of the energy landscape of the SDD. By measuring the quantum capacitance in the time domain, we observe random switching of capacitance between two levels. We determine this to be the stochastic breaking and recombination of single Cooper pairs. By carrying out spectroscopy of the bath responsible for the pair breaking we attribute it to black-body radiation in the cryogenic environment. We also drive the breaking process with a continuous microwave signal, and find that the rate is linearly proportional to incident power. This suggests that a single photon process is responsible, and demonstrates the potential of the SDD as a single photon microwave detector. We investigate this mechanism further, and design an experiment in which the breaking rate is enhanced when the SDD is in the antisymmetric state rather than the symmetric state. We also measure the quantum capacitance of a charge isolated double dot. We observe 2e periodicity, indicating the tunnelling of Cooper pairs and the lack of occupation of quasiparticle states. This work is relevant to the range of experiments investigating the effect of non-equilibrium quasiparticles on the operation of superconducting qubits and other superconducting devices.
This thesis presents measurements of quantum coherence in a single Cooper pair box, where quantum oscillations of charge between a reservoir and a small superconducting island have been observed. The single Cooper pair box (SCB) consists of a small metallic island which is connected to a reservoir via a tunnel junction. In the superconducting state, Cooper pairs are free to tunnel to and from the island, whose potential can be controlled by a gate voltage. A graded gap method was used to prevent quasiparticles from tunneling onto the island. For this purpose, a magnetic field suppressed the superconducting gap in the SCB leads more than in the island. This created an additional energy barrier for quasiparticles to tunnel to the island, making the gate voltage modulation periodic in Cooper pair charge. For a limited range of gate voltage, the SCB was found to behave as a model two-level quantum mechanical system. A non-adiabatic change in the induced island charge was used to bring two charge states into resonance. The resulting time evolution showed clear charge oscillations between the ground and excited state, with a frequency given by the energy level separation divided by Planck's constant. These oscillations had a longest coherence time of T2=9 ns at a point where the pure charge states are degenerate. The coherence time at this point was found to be limited by the relaxation rate, ?1. Away from this point, the coherence time was limited by the dephasing rate, ??. Away from the charge degeneracy, the dependence of T2 on gate charge suggested that low frequency fluctuators were the main source of dephasing. The charge of the Cooper pair box was measured by coupling the SCB capacitively to a radio frequency single electron transistor (RF-SET). The RF-SET was used as an electrometer by measuring the amount of reflection from a resonant microwave circuit in which a single electron transistor (SET) was embedded. A best charge sensitivity of 2.3·10-6 e/sqrt(Hz) and a 7 MHz bandwidth was reached in an improved setup. Another part of this thesis concerns an investigation of electrical filters for use in single electronics experiments. The characteristics of seven different types of cryogenic filters were evaluated.
The transport properties of a small superconductor--normal-metal--superconducting tunnel junction can be controlled by a gate electrode coupled capacitively to the central island. We evaluate the critical Josephson current Ic through such a system as a function of the gate voltage Vg taking into account parity effects in the superconductors. The dependence Ic(Vg) shows resonant singularities and has a qualitatively different character for \ensuremath{\Delta}EC and \ensuremath{\Delta}>EC, \ensuremath{\Delta} being the superconducting gap and EC=e2/2C being the charging energy. Due to the sweeping of the gate voltage, the system can be driven to states which are metastable with respect to a change of the number of electrons on the central island. Since the lifetime of the metastable states can be macroscopically large, one can observe a remarkable bistability of the Josephson current. A weak magnetic field suppresses the interference of the electrons propagating through the central electrode, and, consequently, the magnitude of the critical current.
We consider a system of two superconducting islands, each of which is coupled to a bulk superconductor via Josephson tunneling. One of the islands represents a ``Cooper-pair box,'' i.e., it is an effective two-level system. The other island has a smaller charging energy and approximates a harmonic oscillator. A capacitive interaction between the islands results in a dependence of the oscillator frequency on the quantum state of the box. Placing the latter in a coherent superposition of its eigenstates and exciting coherent oscillations in the large island will lead to a phase shift of these oscillations depending on the box quantum state, thereby producing a coherent superposition of two ``mesoscopically distinct'' quantum states in the large island.
This Thesis studies opportunities to create a quantum standard for the electric current with the help of tunnel junctions. We use two types of tunnel junctions: superconducting Josephson junctions, and NIS junctions where one of the electrodes is normal (N) and the other one superconducting (S). In both cases, tunnel junctions are employed in a single-electron transistor (SET) structure, which is used to transfer a controlled number k of electrons (e) with the repetition frequency f. The magnitude of the resulting current is thus I = kef. First, we study the Cooper pair sluice, where Josephson junctions are connected as two superconducting quantum interference devices (SQUID). A gate electrode is used to control the charge state of the superconducting island formed between the SQUIDs. The sluice is based on tuning the tunneling rates through the SQUIDs with local magnetic fluxes, which allows to control the direction of the charge transfer. Weak traces of current quantization can be observed up to above 1 nA, which is large enough current for many metrological purposes. However, the accuracy of the current is still far from what is required in metrology. We study also a new type of SQUID structure, the balanced SQUID, which could be used to improve the accuracy of the sluice or in, e.g., some quantum computing applications. Second, we employ NIS junctions in the hybrid (SINIS) single-electron transistor with superconducting leads and a normal-metal island. This structure can be used as the SINIS turnstile which lets electrons to flow one by one in the direction determined by the bias voltage. We report the first experimental results on the SINIS turnstile and two methods to improve the accuracy of the current: increasing the charging energy of the island or connecting the turnstile in a resistive environment. We also show that the SINIS turnstile can be used as an electronic radio-frequency refrigerator where tunneling processes cool the electron temperature of the normal-metal island.