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Analytic Expressions for a Spin-Half Particle Dressed by a Polychromatic Field.

Ben Yuen

Published May 15, 2018• 0 citations
OpenAlex

Abstract

Analytic expressions are derived for the time evolution of a spin half in a multi-frequency coherent field, described by a polychromatic Rabi model. We transform to a picture where the spin is dressed progressively by each frequency component of the field. In this picture the time evolution operator takes a simple approximate form, and can be transformed back to the undressed picture where it contains resonant and off-resonant terms. Furthermore, we simplify these transformations to leading order in the field amplitudes, and describe the some of the dominant effects in such multi-frequency processes.

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Analytic expressions are derived for the time evolution of a spin half in a multi-frequency coherent field, described by a polychromatic Rabi model. We transform to a picture where the spin is dressed progressively by each frequency component of the field. In this picture the time evolution operator takes a simple approximate form, and can be transformed back to the undressed picture where it contains resonant and off-resonant terms. Furthermore, we simplify these transformations to leading order in the field amplitudes, and describe the some of the dominant effects in such multi-frequency processes.
A vast collection of light-matter interactions are described by the single-frequency Rabi model. However, the physical world is polychromatic, and until now there is no general method to find analytic solutions to the multi-frequency Rabi model. We present the first general method to solve the Rabi model with N frequency modes. Analytic expressions are derived for a spin-half particle in a multi-frequency coherent field, and accurately describe the time evolution even when the interactions are strong. The dynamics are solved in an extended dressed atom picture whereby the spin is progressively dressed by each frequency mode. For weak fields, the closed form expressions for the time evolution of atoms or their analogues take a particularly simple form. These results analytically solve problems in a wide range of fields including quantum information processing, coherent control and resonant nonlinear optics.
We present a formalism that enables the analytic calculation of the interaction of a spin-half particle with a polychromatic electromagnetic field. This powerful new approach provides a clear physical picture even for cases with highly degenerate energy levels, which are complicated to interpret in the standard dressed-atom picture. Typically semi-classical methods are used for such problems (leading to equations that are solved by Floquet theory). Our formalism is derived from quantum electrodynamics and thus is more widely applicable. In particular it makes accessible the intermediate regime between quantum and semi-classical dynamics. We give examples of the application to multi-frequency multi-photon processes in strong fields by deriving the Hamiltonians of such systems, and also to the dynamics of weak fields at long times for which semi-classical methods are insufficient.
We considered the semiclassical Rabi model, that is, a two-level system interacting with a single-mode, classical field. In resonance and for an arbitrary initial state of the system, we obtained a simple, approximate, and analytic solution that takes into account the counterrotating terms and that is accurate as long as the Rabi frequency is smaller than or equal to 1/2 (1/4) of the angular frequency of the field and 1 (10) Rabi oscillations are considered. In addition, the approximate solution has the same level of complexity as that obtained with the rotating-wave-approximation (RWA) and allows one to describe the evolution of the Bloch vector of the system in terms of a \textit{slow-precessional} and a \textit{fast-nutational} motion similar to that of a symmetric top with one point fixed. Finally, the approximate solution also leads to a simple criterion that allows one to determine the accuracy of the solution in the RWA.
In the framework of the nonsecular perturbation theory based on the Bogoliubov averaging method, the coherent dynamics of multiphoton Raman transitions in a two-level spin system driven by an amplitude-modulated microwave field is studied. Closed-form expressions for the Rabi frequencies of these transitions are obtained beyond the rotating-wave approximation for the low-frequency driving component. It is shown that spin states dressed by the high-frequency component of the driving field are shifted due to the Bloch-Siegert-like effect caused by antiresonant interactions with the strong low-frequency driving. We predict that with increasing the order of the Raman transition, the Rabi frequency decreases and the contribution of the Bloch-Siegert shift to this frequency becomes dominant. It is found that the amplitude and phase of the Rabi oscillations strongly depend on the initial phase of the low-frequency field as well as on detuning from multiphoton resonance. The recent experimental data for the second- and third-order Raman transitions observed for the nitrogen-vacancy center in diamond (Z. Shu et al., arXiv:1804.10492) are well described in the frame of our approach. Our results may provide new possibilities for coherent control of quantum systems.
The dynamics of a two-level spin system dressed by bichromatic radiation is studied under the conditions of double resonance when the frequency of one (microwave) field is equal to the Larmor frequency of the spin system and the frequency of the other (radio-frequency) field ω rf is close to the Rabi frequency ω 1 in a microwave field. It is shown theoretically that Rabi oscillations between dressed-spin states with the frequency ɛ are accompanied by higher-frequency oscillations at frequencies n ω rf and n ω rf ± ɛ, where n = 1, 2,.... The most intense among these are the signals corresponding to n = 1. The counter-rotating (antiresonance) components of the RF field give rise to a shift of the dressed-state energy, i.e., to a frequency shift similar to the Bloch-Siegert shift. In particular, this shift is manifested as the dependence of the Rabi-oscillation frequency ɛ on the sign of the detuning ω 1 − ω rf from resonance. In the case of double resonance, the oscillation amplitude is asymmetric; i.e., the amplitude at the sum frequency ω rf + ɛ increases, while the amplitude at the difference frequency ω rf − ɛ decreases. The predicted effects are confirmed by observations of the nutation signals of the electron paramagnetic resonance (EPR) of E ′ 1 centers in quartz and should be taken into account to realize qubits with a low Rabi frequency in solids.
Multiplication of spin qubits arises at double resonance in a bichromatic field when the frequency of the radio-frequency (rf) field is close to that of the Rabi oscillation in the microwave field, provided its frequency equals the Larmor frequency of the initial qubit. We show that the operational multiphoton transitions of dressed qubits can be selected by the choice of both the rotating frame and the rf phase. In order to enhance the precision of dressed qubit operations in the strong-field regime, the counter-rotating component of the rf field is taken into account.