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SIAM Journal on Control and Optimization

Adiabatic Ensemble Control of a Continuum of Quantum Systems

Nicolas Augier, Ugo Boscain, Mario Sigalotti

Published Jan 1, 2018• 42 citations
Publisher

Abstract

In this article we discuss how to control a parameter-dependent family of quantum systems. Our technique is based on adiabatic approximation theory and on the presence of curves of conical eigenvalue intersections of the controlled Hamiltonian. As particular cases, we recover chirped pulses for two-level quantum systems and counterintuitive solutions for three-level stimulated Raman adiabatic passages. The proposed technique works for systems evolving both in finite-dimensional and infinite-dimensional Hilbert spaces. We show that the assumptions guaranteeing ensemble controllability are structurally stable with respect to perturbations of the parameterized family of systems.

DOI
10.1137/17m1140327

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In this article we discuss how to control a parameter-dependent family of quantum systems. Our technique is based on adiabatic approximation theory and on the presence of curves of conical eigenvalue intersections of the controlled Hamiltonian. As particular cases, we recover chirped pulses for two-level quantum systems and counterintuitive solutions for three-level stimulated Raman adiabatic passages. The proposed technique works for systems evolving both in finite-dimensional and infinite-dimensional Hilbert spaces. We show that the assumptions guaranteeing ensemble controllability are structurally stable with respect to perturbations of the parameterized family of systems.
The main purpose of the thesis is to study the links between the singularities of the spectrum of a controlled quantum Hamiltonian and the controllability issues of the associated Schr"odinger equation.The principal issue that is developed is how to control a parameter-dependent family of quantum systems with a common control input. This problem of ensemble controllability is linked to the design of a robust control strategy when a parameter (a resonance frequency or a control field inhomogeneity for instance) is unknown, and is an important issue for experimentalists.Thanks to the study one-parametric families of Hamiltonians and their generic singularities, we give an explicit control strategy for the ensemble controllability problem when geometric conditions on the spectrum of the Hamiltonian are satisfied. The result is based on adiabatic approximation theory and on the presence of curves of conical eigenvalue intersections of the controlled Hamiltonian. The proposed technique works for systems evolving both in finite-dimensional and infinite-dimensional Hilbert spaces. Then we study the problem of ensemble controllability under less restrictive hypotheses on the spectrum, namely the presence of non-conical singularities. Under generic conditions such non-conical singularities are not present for single systems, but appear for one-parametric families of systems.For the study of a single system, we focus on a class of curves in the space of controls, called the non-mixing curves (defined in cite{Bos}), that can optimize the adiabatic dynamics near conical and non-conical intersections. They are linked to the geometry of the eigenspaces of the controlled Hamiltonian and the adiabatic approximation holds with higher precision along them.We propose to study the compatibility of the adiabatic approximation with the rotating wave approximation. Such approximations are usually done in cascade by physicists. My work shows that this is justified for finite dimensional quantum systems only under certain conditions on the time scales. We also study ensemble control issues in this case.
In this paper we consider the problem of inducing a transition in a controlled quantum mechanical system whose spectrum loses simplicity for some values of the control. We study the situation in which the Hamiltonian of the system is real, and we are in presence of two controls. In this case, eigenvalue crossings are generically conical. Adiabatic approximation is used to decouple a finite dimensional sub system from the original one (usually infinite dimensional). The main advantage of this method is that as a byproduct of the controllability result it permits to get an explicit expression of the controls. Moreover it may be used in the case in which the dependence of the Hamiltonian from the controls is non-linear, for which at the moment, no other method works. In this paper we study the basic block of this controllability method, that is a two by two system whose spectrum presents a conical intersection. We show how to control exactly this system with a control strategy that can be slowed down. The possibility of slowing down the control law is essential to obtain an adiabatic decoupling from the rest of the system with an arbitrary precision.
This work explores the relationship between optimal control theory and adiabatic passage techniques in quantum systems. The study is based on a geometric analysis of the Hamiltonian dynamics constructed from Pontryagin's maximum principle. In a three-level quantum system, we show that the stimulated Raman adiabatic passage technique can be associated to a peculiar Hamiltonian singularity. One deduces that the adiabatic pulse is solution of the optimal control problem only for a specific cost functional. This analysis is extended to the case of a four-level quantum system.
The stimulated Raman adiabatic passage shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity in three-level quantum systems based on adiabatic evolution. This technique has widely theoretical and experimental applications in many fields of physics, chemistry, and beyond. Here, we present a general approach to robust stimulated Raman shortcut-to-adiabatic passage with invariant-based optimal control. By controlling the dynamical process, we inversely design a family of Hamiltonians with non-divergent Rabi frequencies that can realize fast and accurate population transfer from the first to the third level, while the systematic errors are largely suppressed in general. Furthermore, a detailed trade-off relation between the population of the intermediate state and the amplitudes of Rabi frequencies in the transfer process is illustrated. These results provide an optimal route toward manipulating the evolution of three-level quantum systems in future quantum information processing.
Chirped pulses allow for non-adiabatic passage between dressed states of Raman processes. It is shown that using an appropriately chirped pulse, one can control the interference between resonant and non-resonant pathways in stimulated Raman processes. A three-level system is studied in detail and application to complete ro-vibrational level inversion to high vibration quantum numbers (v > 10) in H2 via RCNAP (Raman chirped non-adiabatic passage) is presented. Copyright © 2000 John Wiley & Sons, Ltd.