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Acta Physica Polonica A

Highly Degenerated Ground States in Some Rings Modeled by the Ising Spins with Competing Interactions

Wojciech Florek, Michał Antkowiak, G. Kamieniarz, K. Jaśniewicz-Pacer

Published Mar 1, 2018• 6 citations
Publisher

Abstract

We discuss three Ising ring systems with competing interactions which are analogs of quantum systems and we show that they exhibit similar properties.In particular, the archetypal system of three antiferromagnetically coupled spins s has two magnetically degenerated ground states with |M| s, when 0 J13 α 1 J12 J23.The same effect is observed in the centered rings and even-numbered systems with antiferromagnetic couplings between the second neighbors which are the geometrically frustrated.

DOI
10.12693/aphyspola.133.411

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Advanced Journal of Science Technology and Engineering•Feb 22, 2023•1 citation
We discuss three Ising ring systems with competing interactions which are analogs of quantum systems and we show that they exhibit similar properties.In particular, the archetypal system of three antiferromagnetically coupled spins s has two magnetically degenerated ground states with |M| s, when 0 J13 α 1 J12 J23.The same effect is observed in the centered rings and even-numbered systems with antiferromagnetic couplings between the second neighbors which are the geometrically frustrated.
In this work the ordering processes in classical frustrated Ising models and the ground-state behavior of frustrated quantum spin models are investigated. In the first part the phase transition from a high-temperature paramagnetic phase to a antiferromagnetic ground state is analyzed for the square-lattice Ising model with competing antiferromagnetic interactions between nearest- and next-nearest-neighbor spins. In the case of spatially isotropic interactions the phase transition to a collinear state is of special interest. Using Monte-Carlo simulations on finite lattices as well as field-theoretical methods for the continuous model it is shown that depending on the frustration three different sectors can be distinguished that show (i) Ising-universal behavior (ii) Ashkin-Teller-like non-universal behavior (varying critical exponents) and (iii) non-critical first-order behavior. For spatially anisotropic interactions the emergence of an intermediate incommensurate phase is verified by means of Monte-Carlo simulations which has been predicted by earlier mean-field calculations. The nature of this phase is studied analyzing spin-spin correlation functions and its ordering wave-vector reveals a strong temperature and size dependence. In the second part the influence of quantum fluctuations on classical antiferromagnetic ground states are investigated in anisotropic quantum spin-1/2 Heisenberg models with competing interactions. Using quantum Monte-Carlo simulations, exact diagonalization and perturbation theory the ground-state phase diagrams are calculated for a square lattice with nearest- and next-nearest-neighbor interactions and a honeycomb lattice with up to third-nearest-neighbor interactions whereby the fluctuations are chosen to be non-frustrating. For both cases the stability regions of classical magnetic states are identified and an intermediate phase is detected that shows no sign of long-range magnetic order. Further calculations also rule out valence-bond-crystal or topological order for this state, thus a quantum disordered ground state is stabilized in these models.
The ground-state properties and low-lying excitations of spin systems with competing interactions are studied for various finite two-dimensional S= 1 / 2 Heisenberg systems of 8 spins and corresponding Ising systems of up to 60 spins. The response of the spin systems on the conflict in the interactions is studied using numerical exact results. In the Ising model the competition of the interactions influences the ground state and the excitations essentially. Contrary to conventional Ising systems in disordered strongly frustrated Ising systems the low-energy density of states is smooth, the gap between the ground state and the first excitations vanishes. The low-lying excitations are characterised by a large portion of multiple spin excitations. Thermodynamic consequences are indicated. In the Heisenberg case the influence of the conflict in the interactions is less obvious, the character of the ground state and of the first excitation has similarities with that of conventional antiferromagnets, the spins have an enlarged number of possibilities to evade the conflict in the interactions.
The spin-1/2 Ising-Heisenberg model on martini and martini-diced lattices is exactly solved using a star-triangle transformation, which affords an exact mapping correspondence to an effective spin-1/2 Ising model on a triangular lattice. The ground-state phase diagram of both investigated quantum spin models display two spontaneously ordered ferromagnetic phases and one macroscopically degenerate disordered phase. In contrast to a classical ferromagnetic phase where the spontaneous magnetization of the Ising as well as Heisenberg spins acquire fully saturated values, the spontaneous magnetization of the Heisenberg spins is subject to a quantum reduction to one-third of its saturated value within a quantum ferromagnetic phase. The spontaneous magnetization and logarithmic divergence of the specific heat as the most essential features of both ferromagnetic phases disappear whenever the investigated quantum spin model is driven to the highly degenerate disordered phase. The disordered phase with nonzero residual entropy originates either from a geometric spin frustration caused by antiferromagnetic interactions or more strikingly it may also alternatively arise from a competition of the ferromagnetic Ising and Heisenberg interactions of easy-axis and easy-plane type, respectively. All three available ground states coexist together at a single triple point, around which anomalous magnetic and thermodynamic behavior can be detected.
In selected lattice systems, it is impossible to satisfy all the antiferromagnetic interactions between the spins simultaneously. Due to this frustration the degeneracy of the ground state becomes very large, often scaling with the size of the system. An antiferromagnetic model of Ising spins with on the three-dimensional Swedenborgite lattice will similarly be frustrated and will behave like a spin liquid in all parameter regimes. \n\nFluctuations, which may be either thermal or quantum-mechanical in nature, between the states in the large (disordered) ground state manifold may be biased towards one of them. This causes the system to select a unique (ordered) ground state, in an effect called order-by-disorder. Our objective is now to investigate the effects of quantum fluctuations on the ground states of the Swedenborgite Ising model and to examine it for potential order-by-disorder effects. This will ultimately result in the construction of a tentative phase diagram of this system.
The spin-1/2 Ising-Heisenberg model on martini and martini-diced lattice is exactly solved using a star-triangle transformation, which affords an exact mapping correspondence to an effective spin-1/2 Ising model on a triangular lattice. The ground-state phase diagram of both investigated quantum spin models display two spontaneously ordered ferromagnetic phases and one macroscopically degenerate disordered phase. In contrast to a classical ferromagnetic phase where the spontaneous magnetization of the Ising as well as Heisenberg spins acquire fully saturated values the spontaneous magnetization of the Heisenberg spins is subject to a quantum reduction to one-third of its saturated value within a quantum ferromagnetic phase. The spontaneous magnetization and logarithmic divergence of the specific heat as the most essential features of both ferromagnetic phases disappear whenever the investigated quantum spin model is driven to the highly degenerate disordered phase. The disordered phase with nonzero residual entropy originates either from a geometric spin frustration caused by antiferromagnetic interactions or more strikingly it may also alternatively arise from a competition of the ferromagnetic Ising and Heisenberg interactions of easy-axis and easy-plane type, respectively. All three available ground states coexist together at a single triple point, around which anomalous magnetic and thermodynamic behavior can be detected.
In this research work, frustrations arising from the geometries of triangular lattices have been studied with the aid of Ising and Heisenberg models. The study reveals that geometrical frustrations can generate multiple degeneracies in the ground state. The quantum spin flip terms in the Heisenberg model are observed to play a vital role in the partial lifting up of these degeneracies. Hence, multiple degeneracies as consequence of frustrations are more pronounced for the Ising systems, which are devoid of quantum fluctuations. The observed six- and four-fold ground state degeneracies at zero field for three spins Ising and Heisenberg systems respectively are broken down to half at finite longitudinal fields. For this three-spin system, quantum phase transitions (QPT) are observed at critical longitudinal fields of J and 1.5J respectively for the Ising and Heisenberg models. At these critical fields, the ground states are observed to shift from quasi-antiferromagnet to ferromagnet. However, for the Heisenberg three-spin system in the presence of a transverse field, no transition is observed.