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Experimental platform towards in-fibre atom optics and laser cooling

Muhammad Adnan

Published Dec 18, 2017• 0 citations
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Abstract

This thesis reports on the design and fabrication of an experimental platform for in-fibre laser cooling of Rb and atom optics. By in-fibre laser cooling, we mean the long term aim of laser cooling thermal Rb atoms of a Photonic MicroCell (PMC), and subsequently developing what would be cold-atom photonic crystal fibre (PCF). The platform was designed to harbor several experiments on cold and thermal atom guidance and in-fibre spectroscopy so to address several open questions related for example to the effect of the core inner-wall surface on the atom energy structure and on selective fibre mode excitation for atom trapping and cooling. The completed platform comprises a specific and large ultra-high vacuum (UHV) chamber and a set of lasers for both atom cooling and atom guiding inside highly tailored hollow-core PCF (HC-PCF). The UHV chamber was designed to accommodate several HC-PCFs and two magneto-optical traps (MOT). The HC-PCF were designed, fabricated and post-processed to exhibit different core diameter, modal content and core inner surface material. For example, the mode field diameters range from ~30 µm to ~80 µm for the fundamental Gaussian-like core mode, and the surface materials include pure silica, a layer of Aluminosilicate or a layer of PDMS so to provide a large parameter space in assessing the effect of surface on the fibre-confined atoms. The system has been constructed and characterized. The cooling/repumping laser was frequency-stabilized, with measured Allan variance deviation of σ(τ)=3.8×10^(-11)/√τ. With the system we generated MOT with both isotopes of the Rb atom, with a cooling temperature as low as 7 µK. The platform is now operational to undertake the first atom guidance and explore the feasibility of atom cooling inside a HC-PCF.

DOI
10.70675/0196aff3z168cz4ee9zaeafzf2277149b707

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This thesis reports on the design and fabrication of an experimental platform for in-fibre laser cooling of Rb and atom optics. By in-fibre laser cooling, we mean the long term aim of laser cooling thermal Rb atoms of a Photonic MicroCell (PMC), and subsequently developing what would be cold-atom photonic crystal fibre (PCF). The platform was designed to harbor several experiments on cold and thermal atom guidance and in-fibre spectroscopy so to address several open questions related for example to the effect of the core inner-wall surface on the atom energy structure and on selective fibre mode excitation for atom trapping and cooling. The completed platform comprises a specific and large ultra-high vacuum (UHV) chamber and a set of lasers for both atom cooling and atom guiding inside highly tailored hollow-core PCF (HC-PCF). The UHV chamber was designed to accommodate several HC-PCFs and two magneto-optical traps (MOT). The HC-PCF were designed, fabricated and post-processed to exhibit different core diameter, modal content and core inner surface material. For example, the mode field diameters range from ~30 µm to ~80 µm for the fundamental Gaussian-like core mode, and the surface materials include pure silica, a layer of Aluminosilicate or a layer of PDMS so to provide a large parameter space in assessing the effect of surface on the fibre-confined atoms. The system has been constructed and characterized. The cooling/repumping laser was frequency-stabilized, with measured Allan variance deviation of σ(τ)=3.8×10^(-11)/√τ. With the system we generated MOT with both isotopes of the Rb atom, with a cooling temperature as low as 7 µK. The platform is now operational to undertake the first atom guidance and explore the feasibility of atom cooling inside a HC-PCF.
This thesis reported on atomic spectroscopy for the development of alkaline atomic vapor photonic microcell (PMC). The work is motivated by reproducing the outstanding laboratory environment based performances achieved in the fields of frequency standard and coherent optics in highly compact and stand-alone devices that can be accessible to a wider scientific community or to a commercial market. In our case these future devices will be based a Hollow-core photonic crystal fiber (HC-PCF) filled with a gas phase material to form a PMC, and outstands with an ultra-long long interaction length and micrometric modal area. However, the micrometric scale of the fiber core harboring the atoms raises several technical and scientific challenges. Among the technical challenges, we list the development of efficient process for atom loading inside long hollow fiber with small core diameter, the suppression or mitigation of physio-chemical reactivity of the atoms (i.e. Rubidium) with the fiber core inner-surface silica etc. In parallel, the large surface-to-volume ratio of the fiber-core raises questions like the coherence relaxation dynamics and the nature and effect of the atom-surface interaction. The thesis reports on fiber-core inner surface coating with different materials to mitigate the physio-chemical reactions of the confined atoms with the surface, on tapering large core inhibited coupling Kagome HC-PCF, and splicing technique that ensures low splice loss and no atomic reactivity during the splicing process. In parallel, the thesis reports on a set of spectroscopy experiments to assess the relaxation dynamics of atoms inside HC-PCF and to report on novel sub-Doppler transparencies.
Plateforme expérimentale pour l’optique atomique et refroidissement d'atomes intra-fibre creuse Cette thèse décrit la conception et la réalisation d'une plateforme expérimentale pour le refroidissement par laser et le guidage d’atomes de Rb dans les fibres à cristal photonique à cœur creux (HC-PCF). Cette plateforme a pour but de fournir un système polyvalent pour explorer le refroidissement par laser à l’intérieur des fibres avec l'objectif à plus long terme de réaliser une fibre optique constituée d’un cœur rempli d’atomes froids (micro-cellule photonique). La plateforme a été conçue pour héberger plusieurs expériences sur le guidage d'atomes froids et thermiques ainsi que la spectroscopie dans les HC-PCFs pour répondre à plusieurs questions ouvertes liées par exemple à l'effet de la surface interne des HC-PCFs sur la structure énergétique des atomes ainsi que le piégeage et le refroidissement des atomes. La plateforme comprend une chambre spécifique à vide ultra-élevée (UHV) et un ensemble de lasers pour le refroidissement et le guidage des atomes à l'intérieur du HC-PCF hautement adapté. La chambre UHV a été conçue pour accueillir plusieurs HC-PCFs et deux pièges magnéto-optiques (MOT). Les HC-PCFs ont été conçus et fabriqués avec différents diamètres de cœur, contenu modal et post-traités avec des matériaux différents pour la surface interne du cœur. Par exemple, les diamètres du cœur varient de ~ 30 μm à ~ 80 μm traités avec une couche d'aluminosilicate ou une couche de PDMS afin de fournir un grand espace de paramètres pour évaluer l'effet de la surface sur les atomes confinés dans les fibres. Ainsi, le système a été construit et caractérisé. Le laser de refroidissement/repompage a été stabilisé en fréquence, avec une variance d'Allan de σ(τ)=3,8×10^(-11)/√τ. Avec ce système nous avons généré un MOT avec les deux isotopes du Rb, avec une température de refroidissement faible de l’ordre de 7 μK. La plateforme est maintenant opérationnelle pour entreprendre le premier guidage atomique et explorer la faisabilité du refroidissement des atomes à l'intérieur des HC-PCFs.
This thesis describes developments in atomic vapour loading in hollow core photonic crystal fibre (HC-PCF) for fabrication of atomic vapour loaded photonic microcells (PMC). These developments have been targeted at addressing some of the issues associated with loading atomic vapours in confined waveguiding geometries such as increased dephasing and physio-chemical wall absorptions. Atomic vapour loaded HC-PCF and PMC’s have applications in laser metrology, coherent optics and magneto optical spectroscopy. State of the art HC-PCF have been fabricated for loading with atomic vapour including both photonic bandgap (PBG) guiding and inhibited coupling (IC) hypocycloidal core shape Kagome HC-PCF. Record loss of 70 dB/km has been achieved in IC hypocycloid core shape Kagome HC-PCF in the spectral region centred at 800 nm. This fibre retains excellent single mode propagation combined with large core and increased optical bandwidth in comparison with specialist PBG HC-PCF optimised for operation around 800 nm. Aluminosilicate sol-gel coatings have been developed and successfully applied to the inner core wall of HC-PCF’s to reduce the atomic vapour surface interaction. Confining atomic vapours in micron scaled HC-PCF results in increased dephasing rates because of the frequent atom wall collisions. Anti relaxation coating materials have been applied to the inner core wall and the longitudinal relaxation time has been measured in coated and uncoated fibres utilising a magneto optical technique. Additionally sub Doppler transparencies are investigated in anti relaxation coated and uncoated HC-PCF.
Light can exert optical forces on matter. In the macroscopic world these forces are minuscule, but on the microscopic or atomic scale, these forces are large enough to trap and manipulate particles. They may even be used to cool atoms to a fraction of a degree above absolute zero. \n \nThis thesis details a number of experiments concerned with the optical manipulation of atoms and micron-size particles using free space light beams and photonic crystal fibres. \n \nTwo atom guiding experiments are described. In the first experiment, a spatial light modulator is used to generate higher blue-detuned azimuthal Laguerre-Gaussian LG) beams, which are annular beams with a hollow core. These LG beams are then used to guide laser cooled rubidium-85 atoms within the dark core over a distance of 30 mm. The second atom guiding experiment involves attempting to guide laser cooled and thermal rubidium atoms through a hollow-core photonic crystal fibre using red-detuned light. Hollow-core photonic crystal fibres are fibres that are able to guide light with low attenuation within a hollow core. For this experiment a hot wire detection system was designed, along with a number of complex vacuum systems. \n \nThe first dual-beam fibre trap for micron-size particles constructed using endlessly single-mode photonic crystal fibre (ESM-PCF) is described. The characteristics of dual-beam fibre traps are governed by the fibres used. As ESM-PCF has considerably different properties in comparison to conventional single- or multimode fibres, this dual beam ESM-PCF trap exhibits some novel characteristics. I show that the dual beam ESM-PCF trap can form trapping, repulsive and line potentials; an interference-free ‘white light’ trap; and a dual-wavelength optical conveyor belt.
In this thesis I describe experimental work and present data on the guiding of \nRubidium atoms along free-space propagating light beams as well as within hollow \ncore glass fibres, namely photonic crystal fibres. I describe experiments, laser systems \nand vacuum trap assemblies designed to facilitate this guiding. \nThese experiments are intended to aid progression within the field of cold \natom guidance wherein narrow diameter, long distance hollow-fibre guides are a \ncurrent goal. Realisation of these guides could lead to promising applications such as \natom interferometers and spatially accurate, multi-source, atom depositors. \nHerein, guided fluxes are observed in free-space guiding experiments for \ndistances up to 50mm and up to 10GHz red-detuning from resonance. Additionally \nhollow-core, Kagome structured, quasi- and true-photonic crystal fibres are \ncharacterised. Finally a number of detailed fibre-guiding magneto-optic traps are \ndeveloped. \nBoth cold atomic-beams and cold atomic clouds are reliably positioned above \nfibre entrance facets in conjunction with a guiding laser beam coupled into the fibre \ncore. \nIssues regarding optical flux detection outwith fibre confinement appear to \nhave hindered observation of guided atoms. A far more sensitive detection system has \nbeen developed for use in current, ongoing fibre-guide experiments.
This thesis reports on the design and construction of, and results from, an optical-dipole trapping apparatus developed to confine ultracold rubidium atoms in a conservative, large period, optical-dipole trap. An ultra-high vacuum system was designed and constructed to create a very low- background pressure. A new technique of viewport construction was developed, allowing for the fabrication of economical, high-quality windows for transmission of mid-infra-red laser radiation. The construction of a magneto-optical trap (MOT) and an optical molasses, and the subsequent characterisation, are discussed. A theory for the ac-Stark shift of atoms in a far-detuned laser field was developed. The nature of the scalar and tensorial light-shifts of the ground and first excited states of alkali atoms - the 5s(^2)S1/2 and 5p(^2)P3/2 states of Rb - has been examined. The effect of the differential light-shifts between these states on the operation of efficient laser cooling is discussed. A quasi-electrostatic dipole trap (QUEST) was formed from 50 W of CO2 laser power (٢ = 10.6 μm), focussed to <100 μm. The transfer of ultra-cold atoms from the MOT and optical molasses to the QUEST have been examined. Single beam and standing wave geometries of the QUEST have been implemented, with lifetimes of many seconds. The theory for the ac-Stark effect due to a single laser field has been further developed to consider orthogonally polarised fields with independent wavelengths. The use of an auxiliary laser field, a Nd:YAG laser at λ = 1.064 μm, to enhance the number and density of atoms loaded into the QUEST has been proposed and realised.