This thesis presents correlation measurements in two different few-fermion systems of ultracold 6Li atoms. The measurements have been performed with a new spatially and spin-resolved imaging method with single-atom sensitivity, with which we can probe coherences of the initial system as correlations in the momenta. First, we study attractively interacting atoms in a single microtrap, which serves as a basis for understanding the expansion dynamics of strongly interacting Fermi gases. We observe correlation features in the relative coordinate for different interaction strengths. We explain several of these features theoretically by calculating the initial interacting state in the microtrap and projecting it on a molecular bound state and scattering waves. Next, we study a small number of repulsively interacting particles in the ground state of a double-well potential. This system constitutes the fundamental building block of the Hubbard model. We observe interference patterns in the coordinates of the individual particles and in their relative coordinates. From the amplitude and phase of these patterns, we extract off-diagonal density matrix elements of the state, which we use to directly show coherence and entanglement in our system.
This thesis presents correlation measurements in two different few-fermion systems of ultracold 6Li atoms. The measurements have been performed with a new spatially and spin-resolved imaging method with single-atom sensitivity, with which we can probe coherences of the initial system as correlations in the momenta. First, we study attractively interacting atoms in a single microtrap, which serves as a basis for understanding the expansion dynamics of strongly interacting Fermi gases. We observe correlation features in the relative coordinate for different interaction strengths. We explain several of these features theoretically by calculating the initial interacting state in the microtrap and projecting it on a molecular bound state and scattering waves. Next, we study a small number of repulsively interacting particles in the ground state of a double-well potential. This system constitutes the fundamental building block of the Hubbard model. We observe interference patterns in the coordinates of the individual particles and in their relative coordinates. From the amplitude and phase of these patterns, we extract off-diagonal density matrix elements of the state, which we use to directly show coherence and entanglement in our system.
In this thesis, I report on the deterministic preparation and the observation of strongly correlated few-fermion systems in single and double-well potentials. In a first experiment, we studied a system of one impurity interacting with a number of majority atoms which we prepared in a single potential well in the one-dimensional limit. With increasing number of majority particles, we observed a decrease in the quasi-particle residue which is in agreement with expectations from the Anderson orthogonality catastrophe. In a second experiment, we prepared two fermions in a double-well potential which represents the fundamental building block of the Fermi-Hubbard model. By increasing the repulsion between the two fermions, we observed the crossover into the antiferromagnetic Mott-insulator regime. Furthermore, I describe a new imaging technique, which allows spin-resolved single-atom detection both in in-situ and in time-of-flight. We use this technique to investigate the emergence of momentum correlations of two repulsive fermions in the ground state of the double well. With the methods developed in this thesis, we have established a framework for quantum simulation of strongly correlated many-body systems in tunable potentials.
This thesis reports on the deterministic preparation of magnetically ordered states in systems of few fermionic atoms. We follow the concept of quantum simulation and use 6Li atoms in two different hyperfine states to mimic the behavior of electrons in a solidstate system. In a first experiment, we simulate the two-site Hubbard model by using two atoms in an isolated double-well potential. We prepare the two-particle ground state of this model with a fidelity exceeding 90%. By introducing strong repulsive interactions, we are able to realize a pure spin model and describe the energy spectrum with a two-site Heisenberg Hamiltonian. In a second experiment, we realize Heisenberg spin chains of up to four atoms in a single strongly-elongated trapping potential. Here, the atoms self-align along the potential axis due to strong repulsive interactions. We introduce two novel measurement techniques to identify the state of the spin chains and thereby confirm that we can deterministically prepare antiferromagnetic ground-state systems. This constitutes the first observation of quantum magnetism with fermionic atoms that exceeds nearest-neighbor correlations. Both the double-well system and the spin chains can be seen as building blocks of larger ground-state spin systems. Their deterministic preparation therefore opens up a new bottom-up approach to the experimental realization of quantum many-body systems with ultracold atoms.
This thesis reports on the microscopic investigation of antiferromagnetic order in Hubbard chains, realized with ultracold repulsively interacting fermions in an optical lattice. Extending a quantum gas microscope on spin resolution opened the possibility to Access the full charge and spin statistics of a strongly correlated fermionic many body system. Using this technique, we measured antiferromagnetic correlations over distances up to three lattice sites. Starting with a repulsive degenerate two component mixture of 6Li atoms trapped in a single plane of a vertical lattice, we loaded the Atoms into one-dimensional tubes of a transverse optical superlattice. By adiabatically ramping up the lattice potential along the tubes, we isentropically entered the strongly correlated regime of the one-dimensional Fermi-Hubbard Hamiltonian. We spatially separated the two spin states into opposite sites of local double wells orthogonal to the direction of the lattice before single atom and site sensitive imaging. In this way we extracted the spin information of every single lattice site and were able to evaluate spin-spin correlations. The two component degenerate gases were produced with sub-Poissonian atom number fluctuations by magnetically driven evaporative cooling in vicinity of a Feshbach resonance, used to set the scattering length. The dependence of antiferromagnetic correlations on the driving superexchange coupling was experimentally investigated by varying the interparticle scattering length before loading the atoms into the optical lattice. Taking advantage of the underlying trapping potential of the optical lattice, which shaped the filling and the entropy of the gases, the influence of density excitations and different entropies on spin correlations was observed. By post-selecting the Hubbard chains based on their average filling and local atom number fluctuations, spin correlations corresponding to 58% of the zero temperature predictions in the Heisenberg regime were measured. By comparing the obtained antiferromagnetic correlations to Quantum-Monte-Carlo predictions for our System the lowest measured entropy per particle could be stated as s = 0.51(4)kB, clearly below the critical value of s = ln(2)kB, which is required to form longer ranged correlations. Below this critical entropy, in contrast to local density fluctuations, these spin correlations strongly depend on the entropy of the system. In the future, such a spin thermometer can be used to benchmark novel cooling techniques, which are required to enter the temperature regime of d-wave superconducting states. The access to the full particle and spin statistics will enable us to read out multi-point correlation functions, which characterize such exotic states of matter.
Interacting Fermi systems in two dimensions display intriguing phenomena such as high temperature superfluidity and pseudogap physics. These features emerge from the collective behavior of the constituent particles but are extremely hard to predict from microscopic theory. I will report on experiments that realize microscopic two-dimensional systems with ultracold fermionic lithium atoms. With the ability to deterministically prepare few-body ground states and to observe individual particles in momentum space, they enable a microscopic view of strongly interacting two-dimensional Fermi systems. Surprisingly, we find that characteristic features of many-body Fermi gases can already be found in systems of no more than a dozen particles: In spectroscopy, we observe collective excitations that are the few-body precursor of the Higgs amplitude mode of a superfluid. Moreover, in spin-resolved momentum space probes, we can directly image individual ‘Cooper pairs’ and show the presence of fermionic pairing even in a microscopic setting. These findings may broaden our understanding of finite-size Fermi systems, such as atomic nuclei and superconducting grains.
Identification and understanding of the evolution of interference patterns in two-particle momentum correlations as a function of the strength of interatomic interactions are important in explorations of the nature of quantum states of trapped particles. Together with the analysis of two-particle spatial correlations, they offer the prospect of uncovering fundamental symmetries and structure of correlated many-body states, as well as opening vistas into potential control and utilization of correlated quantum states as quantum-information resources. With the use of the second-order density matrix constructed via exact diagonalization of the microscopic Hamiltonian, and an analytic Hubbard-type model, we explore here the systematic evolution of characteristic interference patterns in the two-body momentum and spatial correlation maps of two entangled ultracold fermionic atoms in a double well, for the entire attractive- and repulsive-interaction range. We uncover quantum-statistics-governed bunching and antibunching, as well as interaction-dependent interference patterns, in the ground and excited states, and interpret our results in light of the Hong-Ou-Mandel interference physics, widely exploited in photon indistinguishability testing and quantum-information science.
Strongly-correlated electron systems generate some of the richest phenomena and most challenging theoretical problems studied in physics. One approach to understanding these systems is with ultracold fermionic atoms in optical lattices, which can provide a level of control and ways of observing strongly-correlated fermionic systems that are not accessible with conventional materials. This thesis describes the development of an experimental technique where a quantum gas of fermionic 6Li atoms is prepared in a two-dimensional optical lattice and each atom can be frozen in place and imaged with single-site resolution. Combining a vacuum-compatible large numerical aperture microscope with Raman sideband cooling enables site-resolved fluorescence imaging with high fidelity. We observe several phases of the Hubbard model, including band and Mott insulators. The observed in-situ occupation distributions of atoms in the lattice are compared to theory with unprecedented detail and are used to determine the thermodynamic properties of the system. By combining site-resolved imaging with a spin-removal technique, we observe antiferromagnetic correlations in the Hubbard model with single-site resolution. We observe, for the first time in cold atom systems, beyond-nearest-neighbor magnetic correlations, which provide a direct measurement of the correlation length. We also present detailed measurements of the formation of correlations during lattice loading.