Dynamic Pairing and Semiclassical Trajectories

Sophya V. Garashchuk, Vitaly A. Rassolov

Christof Sparber

Michael F. Herman, D. F. Coker

The relationship between the diverging of classical trajectories in chaotic many-body systems, the spreading of quantum wave packets, and the validity and use of classical molecular dynamics is explored. This analysis, which is based on the semiclassical description of wave function propagation in terms of a weighted integration over a traveling fixed width coherent state basis, suggests that the exponential divergence of nearby classical trajectories in chaotic many-body systems should result in the rapid delocalization of an initially localized quantum wave packet describing the state of the system. Thus the justification for the use of classical molecular dynamics procedures for these supposedly classical systems cannot be based on the picture of the system wave function remaining localized as its center follows a nearly classical trajectory. The quantum evolution of the system density, on the other hand, requires two propagators, and each of these propagators is represented as an integration over trajectories in the semiclassical picture. The interference between the contributions from these two integrations over classical trajectories focuses the analysis on the most important points in this trajectory pair space, which are shown to occur when both trajectories in the pair are the same. Given reasonable assumptions for the initial density for a system that is expected to be well described by classical molecular dynamics, and given an appropriate choice for the width of the coherent state basis which is employed in the semiclassical description, it is shown that the semiclassical expressions for time dependent observables and correlation functions reduce the purely classical expressions, despite the fact that an initially localized wave packet would rapidly delocalize for the same system.

Nikola Burić

Quantum trajectories given by the quantum state diffusion theory are used to study the dynamics of a pair of qubits interacting with the quantized Duffing oscillator. The latter is a nonlinear dissipative and driven quantum system that in the semiclassical limit displays typical bifurcations and chaotic behavior of the classical model. It is shown that the oscillator part of the qubits-oscillator system in the semiclassical limit is well described by the classical model despite the oscillator-qubit interaction. On the other hand, exact quantum dynamics of the qubits pair is completely different from the classical model as long as there is non-negligible qubit-oscillator interaction. Dynamics of the interqubits entanglement and the qubits pair von Neumann entropy is studied in the deeply quantum and various degrees of semiclassical regimes and for different values of the oscillator's bifurcation parameter. It is concluded that the decoherence of the qubits pair by the dissipative nonlinear oscillator is more effective when the oscillator is in the more classical regime, and if the semiclassical oscillator dynamics is chaotic rather than regular.

Yujun Zheng, Libin Fu, Craig C. Martens +1 more