Quantum correlations play a fundamental role in quantum information science. The variety of their manifestations has become increasingly apparent following the development of novel light sources, protocols and photodetectors. One broad classification identifies two instances of non-classical correlations: particle and mode entanglement. These categories mirror two coexisting descriptions of quantum systems in terms of discrete and continuous variables of the electromagnetic field. The past decades have generated a number of promising results based on schemes which encompass elements from both frameworks, rather than viewing the two descriptions as mutually exclusive. In this context, it is possible to conceive and realise experiments where either the quantum resource or the detection system is 'hybrid'. Optical weak-field homodyne detectors bring together phase sensitivity and photon counting; as such, they represent a detection scheme which works across continuous and discrete variables of the radiation field. In this thesis we present a two-mode weak-field homodyne detection layout with added photon-number resolution and apply it to the study of a split single-photon state and a squeezed vacuum state. As a first test of the capabilities of this system, we investigate the reconstruction of relevant features of a given quantum resource - such as its photon statistics - with our detection scheme. Further, we experimentally demonstrate the observation of an instance of non-classical optical coherence which combines the continuous- and discrete-variable descriptions explicitly. The ability to probe phenomena at the interface of wave and particle regimes opens the way to novel, improved schemes for quantum information processing. From a more fundamental perspective, such hybrid approaches may shed light on the very roots of quantum enhancement.
Quantum correlations play a fundamental role in quantum information science. The variety of their manifestations has become increasingly apparent following the development of novel light sources, protocols and photodetectors. One broad classification identifies two instances of non-classical correlations: particle and mode entanglement. These categories mirror two coexisting descriptions of quantum systems in terms of discrete and continuous variables of the electromagnetic field. The past decades have generated a number of promising results based on schemes which encompass elements from both frameworks, rather than viewing the two descriptions as mutually exclusive. In this context, it is possible to conceive and realise experiments where either the quantum resource or the detection system is 'hybrid'. Optical weak-field homodyne detectors bring together phase sensitivity and photon counting; as such, they represent a detection scheme which works across continuous and discrete variables of the radiation field. In this thesis we present a two-mode weak-field homodyne detection layout with added photon-number resolution and apply it to the study of a split single-photon state and a squeezed vacuum state. As a first test of the capabilities of this system, we investigate the reconstruction of relevant features of a given quantum resource - such as its photon statistics - with our detection scheme. Further, we experimentally demonstrate the observation of an instance of non-classical optical coherence which combines the continuous- and discrete-variable descriptions explicitly. The ability to probe phenomena at the interface of wave and particle regimes opens the way to novel, improved schemes for quantum information processing. From a more fundamental perspective, such hybrid approaches may shed light on the very roots of quantum enhancement.
Entangled photons are ideally suited to the transmission of photonic quantum information. Mitigating the effects of decoherence is fundamental to distributing photonic entanglement across large distances. One such proposal is entanglement distillation, in which operations on a large ensemble of weakly entangled states generate a smaller ensemble of more strongly entangled states. In this thesis, we experimentally and theoretically analyse various tools required for demonstrating continuous-variable (CV) entanglement distillation, following the proposal by Browne et al., [Phys. Rev. A 67, 062320 (2003)]. Specifically, we propose figures of merit to account for the practical limitations of non-deterministic non-Gaussian operations, and analyse the experimental parameters necessary to optimise them. We develop a source of pulsed two-mode squeezed states, which are the initial states of our entanglement distillation protocol. We use weak-field homodyne detection as a phase-dependent photon counting detector, and demonstrate its utility in conditional state generation. Using these states, we demonstrate sub-binomial light as a tool for benchmarking quantum states. Finally, we applied two-mode weak-field homodyne detection to two entangled states and demonstrate correlations in the photon counting statistics which depend on a joint phase from two independent local oscillators. This setup is sufficient to apply an entanglement witness developed by Puentes et al. [New J. Phys. 12, 033042 (2010)]. Despite encouraging simulations, we do not witness entanglement with this scheme, which we attribute to a noise source unaccounted for in the simulations. Although we do not demonstrate entanglement distillation outright, the tools we develop to do so represent a general, hybrid approach to CV quantum optics. Developing tools such as phase-resolved projective measurement on two-mode states allows us to probe both the wave and particle nature of entangled light at the single-photon level. Using and expanding these techniques to probe larger quantum systems may prove useful in studies of fundamental physics and quantum enhanced technologies.
The implementation of optical quantum technologies requires precise and complete characterisation tools for multi-mode nonclassical states of light. In this thesis, we propose and we implement experimentally three applications of optical quantum measurements, which combine aspects of light that are described by both discrete and continuous variables. In the rst part of this thesis, we present a new scheme for interferometric phase estimation, which uses double homodyne measurements as an alternative to photon counting. We show that, without requiring a phase reference, this scheme can achieve the optimum phase estimation precision for all path-symmetric probe states with a de ned number of photons. Furthermore, the estimation procedure is robust against state preparation imperfections, and naturally yields the same precision for all values of the estimated phase. We implement the proposed scheme experimentally, using a polarisation interferometer probed by a single-photon signal, and temporally multiplexing a single homodyne detector. We repeat the experiment with classical probe states. For both cases, we demonstrate the accuracy and precision of the proposed method, our implementation deviating by 5% from the fundamental precision bound. We demonstrate that, in our scheme, single-photon probe states can provide better precision than weak coherent ones. These results indicate that hybrid quantum resources, which combine tools from the discrete and continuous-variable paradigms, can play a signi cant role in practical sensing scenarios. In the second part of this thesis, we present an application in the eld of information thermodynamics, reporting an experimental realisation, in a photonic setup, of Maxwell's demon. We show that a measurement at the few-photons level, followed by a feed-forward operation, allows the extraction of work from intense thermal light into an electric circuit. The interpretation of the experiment leads us to the derivation of an equality relating work extraction to information acquired by measurement. We prove a bound using this relation, and show that it is in agreement with the experimental results. Our work puts forward photonic systems as a platform for experiments in the eld of information thermodynamics. In the third part of this thesis, we present a new method for the characterisation of broadband parametric down-conversion, based on stimulated frequency generation. In particular, we analyse the information contained in the frequency generation produced in the same mode as a seeding beam, for a type-II down-conversion process. We derive a model for this signal and argue that its detection can provide a useful characterisation tool in the high-gain regime, allowing for a self-referenced estimation of squeezing gain. We propose a method for measuring this signal and present an experimental realisation, based on a wave-guided source, at telecommunication wavelengths. Our experimental results demonstrate that the proposed measurement is an e ective experimental handle for discerning the intricate structure of broadband parametric down-conversion.
There are two traditionally-separated approaches to optical quantum information: the continuous- and discrete-variable strategies respectively linked to the wave-like and particle-like nature of light. This thesis work is focused on the novel hybrid approach aiming to join the capabilities of both strategies into single systems. Using hybrid methods, we report on the use of optical parametric oscillators and superconducting-nanowire single-photon detectors to generate highly non-classical non-Gaussian states such as high-purity single-photons, Schr\"odinger cat states and finally hybrid entanglement of light between continuous- and discrete-variable encoding. The potential of this resource is studied in a number of protocols. We first consider non-locality tests with hybrid entanglement such as Bell inequality violation and experimentally demonstrate the violation of Einstein-Podolsky-Rosen steering inequalities. We finally report on the progress made towards the implementation of a new setup for the demonstration of hybrid quantum teleportation between continuous and discrete-variable encodings. Our demonstrations prove the versatility of this hybrid resource and open the possibility of implementing scalable quantum networks linking systems of dissimilar nature.
The thesis focuses on the experimental investigation of the optical hybrid approach forquantum information processing. Specifically, two traditionally separated approaches, i.e.the discrete and the continuous-variable ones, are combined in the same experiment with twodistinct quantum measurements based on photon counting (photon number) and homodynedetection (quadrature components).The optical hybrid approach is first applied to generate high-fidelity non-Gaussian states,e.g. Fock states and Schrödinger cat states, which correspond to two types of qubit encodingsused in optical quantum information. The use of high-efficiency superconducting nanowiresingle-photon detectors leads to an unprecedented preparation rate, which facilitates thesubsequent use of these states. For instance, the two types of states are combined to generatefor the first time a hybrid entanglement between particle-like and wave-like optical qubits, aswell as the extension to hybrid qutrit entanglement. These novel resources may pave the wayto implement heterogeneous networks where discrete and continuous-variable operations andtechniques can be efficiently combined. Additionally, we also experimentally demonstratefor the first time the so-called squeezing-induced micro-macro entangled states.During this PhD, efforts have also been dedicated to implement a high-efficiency andlow-noise frequency up-conversion system based on two synchronized fiber lasers. Suchquantum frequency converter not only permits to extend the spectra of quantum statesto difficultly accessible wavelengths with current technology, but also constitutes a highperformancephoton detector especially in the infrared regime. Based on the conversionsystem, several applications are demonstrated, such as infrared photon-number-resolvingdetection, and few-photon-level infrared imaging.
A feature of quantum mechanical states is delocalised coherence. We directly observe this coherence up to the three photon level. Explicitly, we carry out two-mode weak-field homodyne of both a single photon split at a beam splitter and a two-mode squeezed state. While our measurements are insufficient to quantify or witness entanglement directly, with improved collection efficiency and measurement stability we aim to show that this can be achieved with such a scheme. Thus we have shown how such a detector can directly probe coherence in both the discrete and continuous variable pictures.
Abstract The generation and manipulation of hybrid entanglement of light involving discrete- and continuous-variable states have recently appeared as essential resources towards the realization of heterogeneous quantum networks. Here we investigate a scheme for the remote generation of hybrid entanglement between particle-like and wave-like optical qubits based on a non-local heralding photon detection. We also extend this scheme with additional local or non-local detections. An additional local heralding allows the resulting state to exhibit a higher fidelity with the targeted entangled qubits while a two-photon non-local heralding detection gives access to a higher dimensionality in the discrete-variable subspace, resulting thereby in the generation of hybrid entangled qutrits. The implementation of the presented schemes, in combination with ongoing works on high-fidelity quantum state engineering, will provide novel non-classical light sources for the development of optical hybrid architectures.