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Towards Generation of Heralded Time-Frequency-Entangled Photon Pairs

Dashiell L. P. Vitullo, Michael G. Raymer, Brian J. Smith, Michał Karpiński, Lasse Mejling, Karsten K. Rottwitt

Published Feb 1, 2018• 0 citations
OpenAlex

Abstract

Photonic time-frequency entanglement is a promising resource for quantum information processing technologies. We investigate swapping of continuous-variable entanglement in the time-frequency degree of freedom using three-wave mixing in the low-gain regime with the aim of producing heralded biphoton states with high purity and low multi-pair probability. Heralding is achieved by combining one photon from each of two biphoton sources via sum-frequency generation to create a herald photon. We present a realistic model with pulsed pumps, investigate the effects of resolving the frequency of the herald photon, and find that frequency-resolving measurement of the herald photon is necessary to produce high-purity biphotons. We also find a trade-off between the rate of successful entanglement swapping and both the purity and quantified entanglement resource (negativity) of the heralded biphoton state.

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Photonic time-frequency entanglement is a promising resource for quantum information processing technologies. We investigate swapping of continuous-variable entanglement in the time-frequency degree of freedom using three-wave mixing in the low-gain regime with the aim of producing heralded biphoton states with high purity and low multi-pair probability. Heralding is achieved by combining one photon from each of two biphoton sources via sum-frequency generation to create a herald photon. We present a realistic model with pulsed pumps, investigate the effects of resolving the frequency of the herald photon, and find that frequency-resolving measurement of the herald photon is necessary to produce high-purity biphotons. We also find a trade-off between the rate of successful entanglement swapping and both the purity and quantified entanglement resource (negativity) of the heralded biphoton state.
Photonic time-frequency entanglement is a promising resource for quantum information processing technologies. We investigate swapping of continuous-variable entanglement in the time-frequency degree of freedom using three-wave mixing in the low-gain regime with the aim of producing heralded biphoton states with high purity and low multipair probability. Heralding is achieved by combining one photon from each of two biphoton sources via sum-frequency generation to create a herald photon. We present a realistic model with pulsed pumps, investigate the effects of resolving the frequency of the herald photon, and find that frequency-resolving measurement of the herald photon is necessary to produce high-purity biphotons. We also find a trade-off between the rate of successful entanglement swapping and both the purity and quantified entanglement resource (negativity) of the heralded biphoton state.
We analyze the quantum-state purity of heralded single photons produced from frequency-anticorrelated biphotons. We find that the quantum-state purity in the time-frequency domain depends strongly on the response time uncertainty of the trigger-photon detector that heralds the generation of its paired photon. If the trigger response time is much shorter than the two-photon coherence time, the time-frequency quantum-state purity of heralded single photons approaches unity and the heralded single photon is in a nearly pure state. If the trigger response time is much longer than the two-photon coherence time, the heralded photon is then projected onto a mixed state. Making use of the time-frequency entanglement, heralded single photons with a well-defined temporal wave function or a frequency superposition state can be produced and engineered. This time-frequency entanglement allows for shaping heralded single photons through nonlocal spectral modulation.
Narrow-band time-frequency entangled biphotons are generated from spontaneous four-wave mixing in cold atom clouds. The coherence time of the entangled biphotons can be extended to sub-microseconds by the slow light effect. The temporal wavefunction of the biphotons can be manipulated through modulating the spectral or spatial mode of the controlling laser beams. Concerning a pair of entangled biphoton and the resulting heralded single photon, it was commonly believed that, time-frequency entanglement damages the temporal purity of the single photon. However, the case is totally different for biphotons with long coherence time which is far beyond the time resolution of single-photondetectors. We demonstrate that, the single photon heralded from these time-frequency entangled biphotons is in a pure temporal state. Therefore, single photons are able to be shaped through the time-frequency entanglement with their partner photons, while the single photons could be found to be still in a pure state and thus useful for quantum information processing and communication technology.
Entanglement is a unique property of quantum systems and an essential resource for many quantum technologies. The ability to transfer or swap entanglement between systems is an important protocol in quantum information science. Entanglement swapping between photons forms the basis of distributed quantum networks. Here an experiment demonstrating entanglement swapping from two independent multimode time-frequency entangled sources is presented, resulting in multiple heralded frequency-mode Bell states. Entanglement in the heralded states is verified by measuring conditional anticorrelated joint spectra and quantum beating in two-photon interference. Our experiment heralds up to five orthogonal Bell pairs within the same setup, and this number is ultimately limited only by the entanglement of the initial sources.
The generation of high purity single photons and entangled photon pairs is a crucial first step in many quantum optics experiments, including those that require quantum teleportation [1], entanglement swapping [2], and the generation of multi-photon entanglement [3]. The most widely used and established approach for creating photon pairs is spontaneous parametric down conversion (SPDC) - where pump photons undergo a non-linear optical process to create a down-converted photon pair [4]. Traditionally, the generation of high-purity heralded single photons required severe spectral filtering, introducing additional loss. However, through careful engineering of spectral correlations of the down-converted photon pairs one can circumvent the need for filtering and avoid the accompanying reduction in heralding efficiency.
Deterministic sources of high-fidelity entangled qubit pairs encoded in the dual-rail photonic basis, i.e., presence of a single photon in one of two orthogonal modes, are a key enabling technology of many applications of quantum information processing, including high-rate, high-fidelity quantum communications over long distances. The most popular and mature sources of such photonic entanglement, e.g., those that leverage spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing, generate an entangled (so-called continuous-variable) quantum state that contains contributions from high-order photon terms that lie outside the span of the dual-rail basis, which is detrimental to most applications. One often uses low pump power to mitigate the effects of those high-order terms. However, that reduces the pair generation rate, and the source becomes inherently probabilistic. We investigate a cascaded source that performs a linear-optical entanglement swap between two SPDC sources, to generate a heralded photonic entangled state that has a higher fidelity (to the ideal Bell state) compared to a free-running SPDC source. Furthermore, with the Bell swap providing a heralding trigger, we show how to build a multiplexed source, which despite reasonable switching losses and detector loss and noise, yields a fidelity versus success probability trade-off of a high-efficiency source of high-fidelity dual-rail photonic entanglement. We find, however, that there is a threshold of 1.51.51.5 dB of loss per switch, beyond which multiplexing hurts the fidelity versus success probability trade-off.