Probing the out-of-equilibrium dynamics of quantum matter has gained renewed interest owing to immense experimental progress in artificial quantum systems. Dynamical quantum measures such as the growth of entanglement entropy and out-of-time-ordered correlators (OTOCs) have been shown to provide great insight by exposing subtle quantum features invisible to traditional measures such as mass transport. However, measuring them in experiments requires either identical copies of the system, an ancilla qubit coupled to the whole system, or many measurements on a single copy, thereby making scalability extremely complex and hence, severely limiting their potential. Here, we introduce an alternative quantity, the out-of-time-ordered measurement (OTOM), which involves measuring a single observable on a single copy of the system, while retaining the distinctive features of the OTOCs. We show, theoretically, that OTOMs are closely related to OTOCs in a doubled system with the same quantum statistical properties as the original system. Using exact diagonalization, we numerically simulate classical mass transport, as well as quantum dynamics through computations of the OTOC, the OTOM, and the entanglement entropy in quantum spin chain models in various interesting regimes (including chaotic and many-body localized systems). Our results demonstrate that an OTOM can successfully reveal subtle aspects of quantum dynamics hidden to classical measures and, crucially, provide experimental access to them.Probing the out-of-equilibrium dynamics of quantum matter has gained renewed interest owing to immense experimental progress in artificial quantum systems. Dynamical quantum measures such as the growth of entanglement entropy and out-of-time-ordered correlators (OTOCs) have been shown to provide great insight by exposing subtle quantum features invisible to traditional measures such as mass transport. However, measuring them in experiments requires either identical copies of the system, an ancilla qubit coupled to the whole system, or many measurements on a single copy, thereby making scalability extremely complex and hence, severely limiting their potential. Here, we introduce an alternative quantity, the out-of-time-ordered measurement (OTOM), which involves measuring a single observable on a single copy of the system, while retaining the distinctive features of the OTOCs. We show, theoretically, that OTOMs are closely related to OTOCs in a doubled system with the same quantum statistical properties as the original system. Using exact diagonalization, we numerically simulate classical mass transport, as well as quantum dynamics through computations of the OTOC, the OTOM, and the entanglement entropy in quantum spin chain models in various interesting regimes (including chaotic and many-body localized systems). Our results demonstrate that an OTOM can successfully reveal subtle aspects of quantum dynamics hidden to classical measures and, crucially, provide experimental access to them.

arXiv:1801.08949Physical Review AMar 29, 201811 citations

Weak probe readout of coherent impurity orbital superpositions in silicon

K. L. Litvinenko, P. Thornton Greenland, Britta Redlich +3 more

Pump-probe spectroscopy is the most common time-resolved technique for investigation of electronic dynamics, and the results provide the incoherent population decay time ${T}_{1}$ . Here we use a modified pump-probe experiment to investigate coherent dynamics, and we demonstrate this with a measurement of the inhomogeneous dephasing time ${T}_{2}^{*}$ for phosphorus impurities in silicon. The pulse sequence produces the same information as previous coherent all-optical (photon-echo-based) techniques but is simpler. The probe signal strength is first order in the pulse area but its effect on the target state is only second order, meaning that it does not demolish the quantum information. We propose simple extensions to the technique to measure the homogeneous dephasing time ${T}_{2}$ , or to perform tomography of the target qubit.Pump-probe spectroscopy is the most common time-resolved technique for investigation of electronic dynamics, and the results provide the incoherent population decay time ${T}_{1}$. Here we use a modified pump-probe experiment to investigate coherent dynamics, and we demonstrate this with a measurement of the inhomogeneous dephasing time ${T}_{2}^{*}$ for phosphorus impurities in silicon. The pulse sequence produces the same information as previous coherent all-optical (photon-echo-based) techniques but is simpler. The probe signal strength is first order in the pulse area but its effect on the target state is only second order, meaning that it does not demolish the quantum information. We propose simple extensions to the technique to measure the homogeneous dephasing time ${T}_{2}$, or to perform tomography of the target qubit.

Physical review. B./Physical review. BDec 20, 20162 citations

Probing quantum information propagation with out-of-time-ordered correlators

Jochen Braumüller, Amir H. Karamlou, Yariv Yanay +13 more

arXiv:2102.11751Nature PhysicsDec 23, 2021125 citations

Out-of-Time-Order Correlator Spectroscopy

Keisuke Fujii

Out-of-time-order correlators (OTOCs) are central probes of quantum scrambling, and their generalizations have recently become key primitives for both benchmarking quantum advantage and learning the structure of Hamiltonians. Yet their behavior has lacked a unified algorithmic interpretation. We show that higher-order OTOCs naturally fit within the framework of quantum signal processing (QSP): each $\mathrm{OTOC}^{(k)}$ measures the $2k$ -th Fourier component of the phase distribution associated with the singular values of a spatially resolved truncated propagator. This explains the contrasting sensitivities of time-ordered correlators (TOCs) and higher-order OTOCs to causal-cone structure and to chaotic, integrable, or localized dynamics. Based on this understanding, we further generalize higher-order OTOCs by polynomial transformation of the singular values of the spatially resolved truncated propagator. The resultant signal allows us to construct frequency-selective filters, which we call \emph{OTOC spectroscopy}. This extends conventional OTOCs into a mode-resolved tool for probing scrambling and spectral structure of quantum many-body dynamics.Out-of-time-order correlators (OTOCs) are central probes of quantum scrambling, and their generalizations have recently become key primitives for both benchmarking quantum advantage and learning the structure of Hamiltonians. Yet their behavior has lacked a unified algorithmic interpretation. We show that higher-order OTOCs naturally fit within the framework of quantum signal processing (QSP): each $\mathrm{OTOC}^{(k)}$ measures the $2k$-th Fourier component of the phase distribution associated with the singular values of a spatially resolved truncated propagator. This explains the contrasting sensitivities of time-ordered correlators (TOCs) and higher-order OTOCs to causal-cone structure and to chaotic, integrable, or localized dynamics. Based on this understanding, we further generalize higher-order OTOCs by polynomial transformation of the singular values of the spatially resolved truncated propagator. The resultant signal allows us to construct frequency-selective filters, which we call \emph{OTOC spectroscopy}. This extends conventional OTOCs into a mode-resolved tool for probing scrambling and spectral structure of quantum many-body dynamics.

quant-pharXiv:2511.22654Nov 28, 20250 citations

In Situ Coherence Measurements of Scattered Light in Magnetically Trapped Cold Atomic Clouds: Probe-Driven Atomic Dynamics

Amilson R. Fritsch, Hector Letellier, Leonardo Lima da Silva +4 more

The use of temporal correlations in scattered photons to probe the microscopic dynamics of ultracold quantum gases has emerged as a powerful, minimally destructive approach for in situ analysis. Here, we demonstrate that temporal coherence spectroscopy can quantitatively characterize atomic motion in a magnetic trap, despite the perturbative effects of the probing light. By measuring the first-order correlation function g (1) ( $τ$ ) of light scattered by a 87 Rb cloud confined in a quadrupole trap, we identify radiation-pressure-induced acceleration and heating as the origin of the apparent discrepancy between coherence spectra and temperatures inferred from time-of-flight measurements. A simple dynamical model incorporating these effects restores agreement between theory and experiment, establishing coherence spectroscopy as a reliable in situ probe of velocity distributions in trapped atomic ensembles. Our results pave the way for time-resolved studies of nonequilibrium dynamics and thermalization processes in confined cold gases, complementing conventional destructive imaging techniques.The use of temporal correlations in scattered photons to probe the microscopic dynamics of ultracold quantum gases has emerged as a powerful, minimally destructive approach for in situ analysis. Here, we demonstrate that temporal coherence spectroscopy can quantitatively characterize atomic motion in a magnetic trap, despite the perturbative effects of the probing light. By measuring the first-order correlation function g (1) ($τ$ ) of light scattered by a 87 Rb cloud confined in a quadrupole trap, we identify radiation-pressure-induced acceleration and heating as the origin of the apparent discrepancy between coherence spectra and temperatures inferred from time-of-flight measurements. A simple dynamical model incorporating these effects restores agreement between theory and experiment, establishing coherence spectroscopy as a reliable in situ probe of velocity distributions in trapped atomic ensembles. Our results pave the way for time-resolved studies of nonequilibrium dynamics and thermalization processes in confined cold gases, complementing conventional destructive imaging techniques.

arXiv:2607.18808Jul 21, 20260 citations

Pump-probe spectroscopy is the most common time-resolved technique for investigation of electronic dynamics, and the results provide the incoherent population decay time

{T}_{1}

. Here we use a modified pump-probe experiment to investigate coherent dynamics, and we demonstrate this with a measurement of the inhomogeneous dephasing time

{T}_{2}^{*}

for phosphorus impurities in silicon. The pulse sequence produces the same information as previous coherent all-optical (photon-echo-based) techniques but is simpler. The probe signal strength is first order in the pulse area but its effect on the target state is only second order, meaning that it does not demolish the quantum information. We propose simple extensions to the technique to measure the homogeneous dephasing time

{T}_{2}

, or to perform tomography of the target qubit.

\mathrm{OTOC}^{(k)}

measures the

2k

-th Fourier component of the phase distribution associated with the singular values of a spatially resolved truncated propagator. This explains the contrasting sensitivities of time-ordered correlators (TOCs) and higher-order OTOCs to causal-cone structure and to chaotic, integrable, or localized dynamics. Based on this understanding, we further generalize higher-order OTOCs by polynomial transformation of the singular values of the spatially resolved truncated propagator. The resultant signal allows us to construct frequency-selective filters, which we call \emph{OTOC spectroscopy}. This extends conventional OTOCs into a mode-resolved tool for probing scrambling and spectral structure of quantum many-body dynamics.

τ

) of light scattered by a 87 Rb cloud confined in a quadrupole trap, we identify radiation-pressure-induced acceleration and heating as the origin of the apparent discrepancy between coherence spectra and temperatures inferred from time-of-flight measurements. A simple dynamical model incorporating these effects restores agreement between theory and experiment, establishing coherence spectroscopy as a reliable in situ probe of velocity distributions in trapped atomic ensembles. Our results pave the way for time-resolved studies of nonequilibrium dynamics and thermalization processes in confined cold gases, complementing conventional destructive imaging techniques.