Quantum Fluids
In recent years, quantum fluids have been studied largely in gaseous form, such as the Bose-Einstein condensates (BECs) of alkali atoms and related species. Quantum liquids, other than liquid helium, have been comparatively more difficult to come by. Cabrera et al. combined two BECs and manipulated the atomic interactions to create droplets of a quantum liquid (see the Perspective by Ferrier-Barbut and Pfau). Because the interactions were not directional, the droplets had a roughly round shape. The simplicity of this dilute system makes it amenable to theoretical modeling, enabling a better understanding of quantum fluids.
Science , this issue p. [301][1]; see also p. [274][2]
[1]: /lookup/doi/10.1126/science.aao5686
[2]: /lookup/doi/10.1126/science.aar3785
Quantum Fluids
In recent years, quantum fluids have been studied largely in gaseous form, such as the Bose-Einstein condensates (BECs) of alkali atoms and related species. Quantum liquids, other than liquid helium, have been comparatively more difficult to come by. Cabrera et al. combined two BECs and manipulated the atomic interactions to create droplets of a quantum liquid (see the Perspective by Ferrier-Barbut and Pfau). Because the interactions were not directional, the droplets had a roughly round shape. The simplicity of this dilute system makes it amenable to theoretical modeling, enabling a better understanding of quantum fluids.
Quantum droplets are small clusters of atoms self-bound by the balance of attractive and repulsive forces. Here, we report on the observation of droplets solely stabilized by contact interactions in a mixture of two Bose-Einstein condensates. We demonstrate that they are several orders of magnitude more dilute than liquid helium by directly measuring their size and density via in situ imaging. We show that the droplets are stablized against collapse by quantum fluctuations and that they require a minimum atom number to be stable. Below that number, quantum pressure drives a liquid-to-gas transition that we map out as a function of interaction strength. These ultradilute isotropic liquids remain weakly interacting and constitute an ideal platform to benchmark quantum many-body theories.
The observation of Bose-Einstein condensation (BEC) in dilute atomic gases was the realization of many long-standing goals: (1) to cool neutral atoms into the ground state of the system, thus exerting ultimate control over the motion and position of atoms limited only by Heisenberg's uncertainty relation; (2) to generate a coherent sample of atoms all occupying the same quantum state (this was subsequently used to realize an atom laser, a device which generates coherent matter waves); and (3) to create a quantum fluid with properties quite different from the quantum liquids He-3 and He-4. This provides a test-ground for many-body theories of the dilute Bose gas which were developed many decades ago, but never tested experimentally.
The field of Bose-Einstein condensation (BEC) in dilute atomic gases provides a fruitful playground to test well-developed theories of quantum fluids. Research using BECs can address open questions relating to the many-body aspects of two-component quantum liquids, namely the interaction between the hydrodynamic normal and the superfluid component at finite temperatures. After the first realization of BEC some pilot experiments have been carried out, but detailed experiments are missing. This has to be compared to the case of liquid helium II, where many experiments since the 1950s have added to our understanding of novel phenomena in quantum liquids, like collective excitations, first and second sound, and others. One of the drawbacks of liquid helium is that the interactions are so strong that a clear distinction between the two components is difficult and the interpretation of the phenomena remains ambiguous. Most experimental studies of dilute Bose-Einstein condensed gases use clouds, which are in the collisionless regime. The reason for the lack of detailed experiments in BECs to study quantum liquids and in particular the hydrodynamical aspects of it, is the limited number of atoms (typically 1--10 million) in the experiments leaving the thermal atoms virtually collisionless. Efforts to decrease the mean free path by increasing the confinement limits the lifetime of the sample, since the density is limited by three-body decay. Experiments on dilute clouds of cold atoms are generally conducted in highly asymmetric traps. In these elongated, cigar-shaped geometries the mean free path of the atoms can become much shorter than the size of the cloud in the long, axial direction, but at the same time exceeds the size in the other, radial directions. In this so-called hydrodynamic-collisionless regime the system can be considered radially collisionless and axially hydrodynamic. In our setup we have created BECs containing up to 300 million sodium atoms by evaporation of atoms in an axially strongly decompressed trap with an aspect ratio of 1:65. Hot atoms created in three-body collisions are able to leave the sample in this highly asymmetric trap, before they can heat other atoms in an avalanche. The sample is axially hydrodynamic, but due to the large aspect ratio collisionless in the radial direction. Such samples are ideal for the observation of the interaction between the superfluid and normal fluid component of the cloud. In this thesis we describe the setup which is used to reach the hydrodynamic regime and we describe a novel implementation of the well-known phase contrast imaging technique. Next, we study collective excitations in the crossover from the collisionless toward the hydrodynamic regime, we determine the heat conduction in a cold, hydrodynamic thermal cloud and observe the propagation of a thermal wave in the two-fluid regime. Furthermore, we study the friction between the superfluid and normal fluid component of the cloud. In the final chapters of this thesis we study the propagation of second sound, as well as the formation and propagation of shock waves.
Ultra-dilute self bound droplets in Bose-Einstein condensates have been of great interest since their first prediction in 2015.The self-bound nature of these bosonic gases combined with their extremely low densities make them a prime target of investigation for both experimentalists and theoreticians.In this thesis work dipole-dipole interacting gases are simulated using the Gross-Pitaevskii equation applying a fourth order, split-operator imaginary time method in two dimensions.First, the systems are studied at collapse for dipoles aligned with a magnetic field that tilts the dipoles in the two-dimensional plane.For some angles the dipole interaction becomes partly attractive which can lead to the collapse of the mean field solution.However, quantum fluctuations can stabilize the gas.Introducing the so-called Lee-Huang-Yang (LHY) correction, the system can be stabilized and self-bound droplets may form.Here, we investigate this stabilization for a quasi two-dimensional set-up. Popular science Ultra-cold droplets intrigue physicistsA hot topic within ultra-cold atom physics has been the recent discovery of droplets formed out of Bose-Einstein condensates, a specific form of a super cold and very dilute gas.The condensate is however very different from any gas encountered in everyday life.A normal gas can be thought of as atoms or molecules moving around in all directions.If you cool this gas, all the particles move slower until they either form a liquid or freeze and become a solid.This is not the case for the Bose-Einstein condensate.Instead they spread through space due to quantum mechanics and together they form one entity.This entity, the so called condensate, behaves like no classical gas, as it is mainly governed by quantum mechanics and not by the random chance of a lot of small particles moving about.To add to this strangeness, droplets now seem to form out of these condensates.The existence of these droplets was quite a surprise.Among experimentalists working with creating Bose-Einstein condensates the expected result was a collapse of the system if forces pushing the condensate together won against the forces pushing it apart.However, experimentalists revealed that some other internal force stabilized drops inside the condensate.Not only that, this force seemed to be able to create drops that could exist outside a "trap", which usually is a number of lasers and magnets that keep the condensate together.Some droplets could not be formed without a trap, but instead formed crystal structures, a very intriguing result.This has led to an excited mood within the field of cold atom physics.But what to expect from this anti-collapse force, mainly being described as quantum fluctuations, and the droplets it creates needs further study to find out.In this thesis work we simulate the anti-collapse force and possible droplet systems solving the underlying quantum-mechanical many-particle equations numerically.One system of interest is the very thin disc of condensate, or a quasi two-dimensional condensate.This system is excellent for rotating the condensate in.Why? Imagine having a piece of pizza dough that in this case represents a condensate.If you spin this dough as a skilled pizza maker does, the pizza will become flat due to rotational forces.The same goes for the condensate.As you rotate it it will become flat anyways and therefore having a model where our very cold gas is already flat makes it easier to simulate rotating systems.But before you start rotating your drops, you have to find the drops.And to find the drops you have to study the forces pushing the condensate together and the forces pushing it apart.Therefore we presently aim at studying possible droplet formation in these pizza crust shaped condensates, to make way for the study of rotational excitations.Initial results show some promise that droplets can be found in these quasi two-dimensional systems.
Among settings which have recently been elaborated for the creation of stable multidimensional solitons, most advanced, as concerns the theory and experiment alike, is the work with quantum droplets (QDs) in atomic BEC. Important theoretical predictions for fundamental and topologically structured soliton-like (stably self-trapped) QDs have been published in many papers, starting from the pioneering work of Petrov [Phys. Rev. Lett. 115, 155302 (2015)]. Simultaneously, the experimental advancement in the making of QDs in binary BECs, as well as in single-component BECs of atoms carrying magnetic dipole moments, have been really remarkable and unique. Successful experiments followed the first theoretical prediction of the QDs very quickly, and the progress in the experimental work was much faster than in other areas of physics where stable multidimensional solitons were predicted. The basis of these works is a correction to the MF (mean-field) BEC dynamics produced by quantum fluctuations around MF states. The correction was first predicted in 1957 by Lee, Huang, and Yang (LHY). The breakthrough proposal made by Petrov [Phys. Rev. Lett. 115, 155302 (2015)] was to use the effective higher-order (quartic) self-repulsion, produced by the LHY effect in the atomic BEC, as a mechanism arresting the collapse driven by mutual attraction of two self-repulsive components in a binary quantum bosonic gas. The balance between the inter-species attraction and LHY-induced self-repulsion gives rise to stable 3D and quasi-2D (pancake-shaped) localized bound states in the form of the quantum droplets (QDs). In single-component condensates of magnetic atoms, the attraction is provided by the long-range dipole–dipole interaction (Chomaz et al., 2016; Schmitt et al., 2016). The competition between the MF attraction and LHY repulsion maintains a superfluid state whose density (taking very low values) cannot exceed a certain maximum, thus making it effectively incompressible. This is a reason why this quantum macroscopic state of matter is identified as a superfluid. Accordingly, localized states filled by this quantum fluid are called “droplets.” In addition to the 3D QDs, droplets in the effectively 2D setting, which may exist under the action of tight confinement in one direction, imposed by an external potential, were theoretically predicted [Petrov and Astrakharchik, Phys. Rev. Lett. 117, 100401 (2016)] and experimentally created [Cabrera et al., Science 359, 301-304 (2018)] too. This chapter provides a condensed review of basic theoretical results for stable QDs in binary BECs, maintained through the stable balance between the inter-species attraction and intra-species LHY repulsion. Both fundamental modes and ones with embedded vorticity are considered. The presentation is partly based on a review article by Luo et al. [Front. Phys. 16, 32501 (2021)]. In addition to 2D and 3D self-trapped QDs in free space, the present chapter addresses 2D fundamental and vortex modes trapped in a singular attractive potential, ∼−1/r2, which are stabilized by the LHY repulsion. Two subsequent chapters present a summary of experimental findings for QDs in binary BECs and for QDs in single-component BECs of magnetic atoms.