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Journal of Physics B Atomic Molecular and Optical Physics

Sympathetic sideband cooling of a 40 Ca + – 27 Al + pair toward a quantum logic clock

Kaifeng Cui, Junjuan Shang, Sijia Chao, Shaomao Wang, Jinbo Yuan, Ping Zhang, Jian Zhong Cao, Hua-lin Shu, Xue-Ren Huang

Published Jan 5, 2018• 17 citations
Publisher

Abstract

Abstract We achieve the sympathetic sideband cooling of a 40 Ca + – 27 Al + pair. Both axial modes of the two-ion chain are cooled simultaneously to near the ground state of the motion. The center of mass mode is cooled to an average phonon number of 0.052(9), and the breathing mode is cooled to 0.035(6). The heating rates of both a single 40 Ca + and the 40 Ca + – 27 Al + pair are measured and compared. This work is a fundamental step toward the implementation of a 40 Ca + – 27 Al + quantum logic clock.

DOI
10.1088/1361-6455/aaa591

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Abstract We achieve the sympathetic sideband cooling of a 40 Ca + – 27 Al + pair. Both axial modes of the two-ion chain are cooled simultaneously to near the ground state of the motion. The center of mass mode is cooled to an average phonon number of 0.052(9), and the breathing mode is cooled to 0.035(6). The heating rates of both a single 40 Ca + and the 40 Ca + – 27 Al + pair are measured and compared. This work is a fundamental step toward the implementation of a 40 Ca + – 27 Al + quantum logic clock.
We report on electromagnetically induced transparency cooling of 40Ca+ to sympathetically cool the three-dimensional secular modes of motion in a 40Ca+–27Al+ two-ion pair near the ground state. We observe simultaneous ground state cooling across all radial modes and axial modes of a 40Ca+–27Al+ ion pair, occupying a broader cooling range in frequency space over 3 MHz. The cooling time is observed to be less than 1 ms. The mean phonon number and heating rates of all motional modes are measured. This study is not only an important step for reducing the secular motion time-dilation shift uncertainty and uptime ratio of 27Al+ optical clock, but also essential for high-fidelity quantum simulations and quantum information processors using trapped ions.
Raman sideband cooling of 25^{25}25Mg+^++ -27^{27}27Al+^++ ions pair and observation of quantum logic spectra
We perform quantum logic spectroscopy (QLS) on 27^{27}27Al+^++ ion 1^11S0_00​ - 3^33P1_11​ transition, which is an important step toward the QLS based 27^{27}27Al+^++ ion optical clock. As a precondition of QLS, both the stretch (STR) mode and the common (COM) mode of the 27^{27}27Al+^++ and 25^{25}25Mg+^++ ions pair are cooled to the vibrational ground state by Raman sideband cooling. The mean phonon number is measured to be 0.10(1) for the STR mode and 0.01(1) for the COM mode, respectively. The heating rate is evaluated to be 13(3) phonons/s for the STR mode and 5.5(1) phonons/s for the COM mode.
The 27 Al + ion optical clock is one of the most attractive optical clocks due to its own advantages such as low black-body radiation shift at room temperature and insensitivity to the magnetic drift. However, it cannot be laser-cooled directly in the absence of 167nm laser to date. This problem can be solved by sympathetic cooling. In this work, a linear Paul trap is used to trap both 40 Ca + and 27 Al + ions simultaneously, and a single Doppler-cooled 40 Ca + ion is employed to sympathetically cool a single 27 Al + ion. Thus a 'bright-dark' two-ion crystal has been successfully synthesized. The temperature of the crystal has been estimated to be about 7 mK by measuring the ratio of carrier and sideband spectral intensities. Finally, the dark ion is proved to be an 27 Al + ion by precise measuring of the ion crystal's secular motion frequency, which means that it is a great step for our 27 Al + quantum logic clock.
Laser-cooled atomic ions have led to an unprecedented amount of control over the quantum states of matter. The Coulombic interaction allows for information to be transferred between neighboring ions, and this interaction can be used to entangle qubits for logic operations in quantum information processors. The same procedure for logic operations can be used for high resolution atomic spectroscopy, and is the basis for the most accurate atomic optical clocks to date. This thesis describes how laser-cooled atomic ions can impact physical chemistry through the development of molecular ion spectroscopy techniques and the simulation of magnetic systems by ion trap quantum computers. \n\t \n\tA new technique developed for spectroscopy, Sympathetic Heating Spectroscopy (SHS), takes advantage of the Coulombic interaction between two trapped ions: the control ion and a spectroscopy ion. SHS uses the back action of the interrogating laser to map spectroscopy ion information onto the Doppler shift of the control ion for measurement. SHS only requires Doppler cooling of the ions and fluorescence measurement and represents a simplification of quantum logic spectroscopy. This technique is demonstrated on two individual isotopes of calcium: Ca-40(+) for cooling and Ca-44(+) as the spectroscopy ion. \n \n\tHaving demonstrated SHS with atomic ions, the next step was to extend the technique by loading and characterizing molecular ions. The identification of an unknown molecular ion is necessary and can be achieved by monitoring the change in motion of the two ion crystal, which is dependent on the molecular ion mass. The motion of two trapped ions is described by their normal modes, which can be accurately measured by performing resolved sideband spectroscopy of the S(1/2)-D(5/2) transition of calcium. The resolved sidebands can be used to identify unknown ions (atomic and molecular) by calculating the mass based on the observed value in axial normal mode frequencies. Again, the trapped molecular ion is sympathetically cooled via the Coulombic interaction between the Ca-40(+) and the unknown molecular ion. The sensitivity of SHS could be improved by implementing sympathetic sideband cooling and determining the heating by measuring single quanta of motion. \n\t \n\tThe ultimate limit of control would be the development of an ion trap quantum computer. Many theoretical quantum computing researchers have made bold claims of the exponential improvement a quantum computer would have over a classical computer for the simulation of physical systems such as molecules. These claims are true in principle for ideal systems, but given non-ideal components it is necessary to consider the scaling due to error correction. An estimate of the resource requirements, the total number of physical qubits and computational time, required to compute the ground state energy of a 1-D quantum Transverse Ising Model (TIM) of N spin-1/2 particles, as a function of the system size and the numerical precision, is presented. This estimate is based on analyzing the impact of fault-tolerant quantum error correction in the context of the quantum logic array architecture. The results show that a significant amount of error correction is required to implement the TIM problem due to the exponential scaling of the computational time with the desired precision of the energy. Comparison of this result to the resource requirements for a fault-tolerant implementation of Shor's quantum factoring algorithm reveals that the required logical qubit reliability is similar for both the TIM problem and the factoring problem.
A two-ion pair in a linear Paul trap is extensively used in the research of the simplest quantum-logic system; however, there are few quantitative and comprehensive studies on the motional mode coupling of two-ion systems yet. This study proposes a method to investigate the motional mode coupling of sympathetically cooled two-ion crystals by quantifying three-dimensional (3D) secular spectra of trapped ions using molecular dynamics simulations. The 3D resonance peaks of the 40Ca+–27Al+ pair obtained by using this method were in good agreement with the 3D in- and out-of-phase modes predicted by the mode coupling theory for two ions in equilibrium and the frequency matching errors were lower than 2%. The obtained and predicted amplitudes of these modes were also qualitatively similar. It was observed that the strength of the sympathetic interaction of the 40Ca+–27Al+ pair was primarily determined by its axial in-phase coupling. In addition, the frequencies and amplitudes of the ion pair’s resonance modes (in all dimensions) were sensitive to the relative masses of the ion pair, and a decrease in the mass mismatch enhanced the sympathetic cooling rates. The sympathetic interactions of the 40Ca+–27Al+ pair were slightly weaker than those of the 24Mg+–27Al+ pair, but significantly stronger than those of 9Be+–27Al+. However, the Doppler cooling limit temperature of 40Ca+ is comparable to that of 9Be+ but lower than approximately half of that of 24Mg+. Furthermore, laser cooling systems for 40Ca+ are more reliable than those for 24Mg+ and 9Be+. Therefore, 40Ca+ is probably the best laser-cooled ion for sympathetic cooling and quantum-logic operations of 27Al+ and has particularly more notable comprehensive advantages in the development of high reliability, compact, and transportable 27Al+ optical clocks. This methodology may be extended to multi-ion systems, and it will greatly aid efforts to control the dynamic behaviors of sympathetic cooling as well as the development of low-heating-rate quantum logic clocks.