Bose–Einstein condensation is a quantum statistical phase transition that occurs in a system consisting of bosons when a single-particle quantum state becomes macroscopically occupied. This peculiar state of matter was first predicted in 1925 and finally realized seventy years later in vapours of weakly-interacting alkali-metal atoms. Since then, Bose–Einstein condensates have been one of the most fascinating research fields in modern physics. \n \nThe gaseous condensates offer a robust platform to accurately study interacting many-particle systems from the first principles. Experimentally, the possibility to precisely control a condensate with external fields and directly image its order parameter provides unforeseen opportunities to obtain deep insight into phenomena across different subfields of physics. In particular, gaseous condensates can emulate complicated models that arise in atomic, condensed-matter, and even particle physics, allowing realizations of exotic phenomena that are elusive in their original contexts. An outstanding example is the existence of various topological defects in ultacold quantum gases with internal degrees of freedom. \n \nIn this thesis, we investigate the creation, stability, and dynamical properties of various topological defects in spinor Bose–Einstein condensates. The majority of the theoretical results is obtained by numerically solving the dynamics using Gross–Pitaevskii equations for spin-1 condensates. Many theoretical predictions are confirmed by the very good agreement with experiments. \n \nThe first experimental observations of a topological point defect in an order parameter describing the quantum gas are presented. Such a point defect is reminiscent to the magnetic monopole particle appearing in grand unified theories. Therefore, the discovery of monopoles in quantum gases further encourages the quest for finding magnetic monopoles in natural electromagnetic fields, a search largely initiated by Paul Dirac almost a century ago. \n \nSubsequently, the fine structure and decay dynamics of the point defect are studied numerically and verified in experiments. The created monopole is gradually destroyed during the polar-to-ferromagnetic quantum phase transition, which results in the spontaneous emergence of a Dirac monopole in synthetic magnetic field. In addition to the singular point defect, the first experimental realization of a knot soliton in the context of quantum field is reported. This thesis lays the foundation for studies of the dynamics and stability of three-dimensional topological structures in quantum systems.
Bose–Einstein condensation is a quantum statistical phase transition that occurs in a system consisting of bosons when a single-particle quantum state becomes macroscopically occupied. This peculiar state of matter was first predicted in 1925 and finally realized seventy years later in vapours of weakly-interacting alkali-metal atoms. Since then, Bose–Einstein condensates have been one of the most fascinating research fields in modern physics. \n \nThe gaseous condensates offer a robust platform to accurately study interacting many-particle systems from the first principles. Experimentally, the possibility to precisely control a condensate with external fields and directly image its order parameter provides unforeseen opportunities to obtain deep insight into phenomena across different subfields of physics. In particular, gaseous condensates can emulate complicated models that arise in atomic, condensed-matter, and even particle physics, allowing realizations of exotic phenomena that are elusive in their original contexts. An outstanding example is the existence of various topological defects in ultacold quantum gases with internal degrees of freedom. \n \nIn this thesis, we investigate the creation, stability, and dynamical properties of various topological defects in spinor Bose–Einstein condensates. The majority of the theoretical results is obtained by numerically solving the dynamics using Gross–Pitaevskii equations for spin-1 condensates. Many theoretical predictions are confirmed by the very good agreement with experiments. \n \nThe first experimental observations of a topological point defect in an order parameter describing the quantum gas are presented. Such a point defect is reminiscent to the magnetic monopole particle appearing in grand unified theories. Therefore, the discovery of monopoles in quantum gases further encourages the quest for finding magnetic monopoles in natural electromagnetic fields, a search largely initiated by Paul Dirac almost a century ago. \n \nSubsequently, the fine structure and decay dynamics of the point defect are studied numerically and verified in experiments. The created monopole is gradually destroyed during the polar-to-ferromagnetic quantum phase transition, which results in the spontaneous emergence of a Dirac monopole in synthetic magnetic field. In addition to the singular point defect, the first experimental realization of a knot soliton in the context of quantum field is reported. This thesis lays the foundation for studies of the dynamics and stability of three-dimensional topological structures in quantum systems.
Since their experimental discovery in 1995, dilute Bose–Einstein condensates have proven to be excellent platforms for studying interacting many-body quantum systems. The gaseous condensates can be conveniently controlled in space and time with lasers and magnetic fields. Theoretically, these low-temperature systems can be described starting from first principles, and their dynamics is accurately captured by the mean-field approach. Dilute condensates with internal spin degrees of freedom may host various topological defects including vortices, monopoles, and skyrmions. Precise external control fields can be used to engineer and study these topological states. \n \nIn this thesis, we investigate the creation, stability, and dynamics of various topological defects in spinor Bose–Einstein condensates. A combination of numerical and analytical methods is used and a part of the research is carried out in collaboration with an experimental research group. The majority of the research involves numerically solving the mean-field Gross–Pitaevskii equation for a spin-1 condensate. The computations are accelerated with graphics processing units. \n \nWe find that the ground state of a ferromagnetic spin-1 condensate supports a Dirac monopole in its synthetic magnetic field in the presence of a quadrupole magnetic field. The energetics of various stationary states of spin-orbit coupled condensates are analyzed and a robust method to observe these exotic states in experiments is proposed. The creation of topological skyrmions is simulated and a very good quantitative agreement with a recent experiment is obtained. Importantly, the first experimental observations of both, Dirac monopoles and topological point defects in a system governed by a quantum field are presented. Subsequently, the decay dynamics of the point defect is studied, revealing the decay into a ferromagnetic state supporting the Dirac monopole. \n \nThe impact of the research conducted in this thesis is not limited to gaseous Bose–Einstein condensates, but due to the universality of quantum mechanics and topological defects, our work provides knowledge, ideas, and inspiration across research fields.
Topology provides deep conceptual links between the various branches of physics. Bose–Einstein condensates with spin degrees of freedom are among the most accessible quantum systems available for studying topological structures. A wide range of topological defects and textures available in condensates, such as vortices, monopoles, knots, and skyrmions, are analogous to those predicted in electromagnetism, high-energy physics, and cosmology.
In this dissertation, we numerically and experimentally investigate novel creation methods for topological structures and study their dynamical properties. Specifically, we experimentally observe the evolution of an isolated monopole into a Dirac monopole in the presence of a quadrupole magnetic field. The Dirac monopole appears in the synthetic magnetic field of the condensate and is accompanied by spontaneously emerging nodal lines. We observe the decay of a quantum knot into a polar-core spin vortex in the presence of a uniform magnetic field. Furthermore, we observe that a decaying coreless-vortex state gives rise to a pair of singular SO(3) vortices.
Many of the studied creation methods for topological structures in the condensate rely on adiabatic control of the external magnetic field. The counterdiabatic protocol offers a way to speed up the otherwise slow magnetic field driving required for adiabatic dynamics with a correcting magnetic field. Using this method, we numerically implement a scheme for fast vortex pumping which leads to the vortex with highest angular momentum reported to date in Bose–Einstein condensates with experimentally feasible methods. We further use the counterdiabatic protocol in a novel way to create quantum knots in the condensate.
Another focal point of this dissertation is the study on different types of skyrmions in spinor condensates. Our simulations of two-dimensional skyrmions are in a quantitative agreement with an experiment carried out elsewhere, explaining the experimentally observed instabilities. We numerically analyze the exotic spin-2 skyrmions available in the cyclic and biaxial nematic phases. Importantly, we present the first experimental observations of Shankar skyrmions in spin-1 condensates and analyze their synthetic electromagnetic properties.
This dissertation addresses an extensive amount of topological structures available in the condensate, but many different structures await future studies. In addition, the precise computational characterization of the elementary excitations of monopoles, knots, and skyrmions is of great interest. The results of this dissertation form a sturdy basis for future experimental studies on the dynamics of topological structures in spinor condensates.; Topologia tarjoaa syvallisia kasitteellisia yhteyksia fysiikan eri haarojen valilla. Bosen–Einsteinin kondensaatit spin-vapausasteilla ovat yksia monipuolisimmista systeemeista topologisten rakenteiden tutkimukseen. Laaja kirjo kondensaatissa esiintyvia topologisia rakenteita, kuten kvanttipyorteet, monopolit, solmut ja skyrmionit, ovat…
Topological defects play important roles throughout nature, appearing in contexts as diverse as cosmology, particle physics, superfluidity, liquid crystals, and metallurgy. Point defects can arise naturally as magnetic monopoles resulting from symmetry breaking in grand unified theories. We devised an experiment to create and detect quantum mechanical analogs of such monopoles in a spin-1 Bose-Einstein condensate. The defects, which were stable on the time scale of our experiments, were identified from spin-resolved images of the condensate density profile that exhibit a characteristic dependence on the choice of quantization axis. Our observations lay the foundation for experimental studies of the dynamics and stability of topological point defects in quantum systems.
We experimentally study the dynamics of quantum knots in a uniform magnetic field in spin-1 Bose-Einstein condensates. The knot is created in the polar magnetic phase, which rapidly undergoes a transition toward the ferromagnetic phase in the presence of the knot. The magnetic order becomes scrambled as the system evolves, and the knot disappears. Strikingly, over long evolution times, the knot decays into a polar-core spin vortex, which is a member of a class of singular SO(3) vortices. The polar-core spin vortex is stable with an observed lifetime comparable to that of the condensate itself. The structure is similar to that predicted to appear in the evolution of an isolated monopole defect, suggesting a possible universality in the observed topological transition.
Single topological defects and related structures have been experimentally created inside clouds of Bose-Einstein condensates. However, a practical protocol for creating multiple defects inside a single cloud—a prerequisite for studying defect interactions—has been lacking. Here we propose, and theoretically analyze, a practical protocol for the creation of configurations of topological monopoles, quantum knots, and skyrmions in Bose-Einstein condensates by employing fictitious magnetic fields induced by the interaction of the atomic cloud with coherent light fields. It is observed that a single coherent field is not enough for this purpose, but instead we find incoherent superpositions of several coherent fields that introduce topological point charges. We numerically estimate the experimentally achievable strengths and gradients of the induced fictitious magnetic fields and find them to be adjustable at will to several orders of magnitude greater than those of the physical magnetic fields employed in previous experimental studies. This property together with ultrafast control of the optical fields paves the way for advanced engineering of topological defects in quantum gases. Published by the American Physical Society 2024
Just a couple decades ago bosonic low-temperature physics was synonymous with one particular liquid at a temperature of several degrees Kelvin. This liquid, helium-4, and its famous Helium-II phase, has revealed remarkable quantum properties such as quantized vortices and second sound. Yet, despite many things learned by investigating helium, its study has certain limitations. On the one hand, helium is a strongly interacting liquid, which makes first-principles theoretical research challenging. To name one example, establishing a connection between the non-interacting condensate state described by Bose and Einstein, and the helium properties observed in the lab took decades. Furthermore, helium is a specific chemical element, and hence there is no surprise that its physical properties are fixed by nature. However, every particular chemical element has particular physical properties, so for a long time it seemed that it was as good as it gets. The picture has changed drastically when the first Bose-Einstein condensate (BEC) was observed in an ultracold atomic gas. “Low temperature” has become synonymous with “ultracold”, and the latter implies temperatures on the order of nanokelvins. Most strikingly, the relationship between what is fixed by nature and what is experimentally changeable has evolved. In particular, systems of different particle statistics, spin, and interactions have been engineered using ultracold vapours of various alkali atoms. This versatile manipulation not only makes emulating various condensed-matter physics models in a controlled system without impurities possible, but also opens a path towards novel phenomena that are at present not achievable in any other manner. In this thesis, we have explored some of the novel phenomena that arise in systems of bosonic particles with internal degrees of freedom, such as (pseudo)spin and electric dipole moment. In the introduction, we describe a ferromagnetically coupled spin-1/2 Bose gas with contact interactions in the mean- field approximation. In particular, we compute and discuss the phase diagram of this gas, since it is a simple system which nevertheless has two order parameters. In the chapters that follow, the ideas touched upon in the introduction are developed in more detail. In Chapter 2 we develop a hydrodynamic description of the ferromagnetic spin-1/2 Bose gas at arbitrary temperatures. We study magnetization relaxation and geometric forces. In particular, we consider the topological Hall effect due to the presence of a skyrmion. In Chapter 3 we investigate the miscible (non-ferromagnetic) spin-1/2 Bose gas at arbitrary temperatures, construct its hydrodynamic description, calculate the thermodynamic properties, and study the collective modes of this system. In Chapter 4 we discuss the influence of the off-diagonal Berry curvature on the Bose-Einstein condensation temperature. Finally, in Chapter 5 we study a Bose-Einstein condensate of dipolar molecules in a weak electric field and find it to be described by a quantum rotor model. Moreover, we show that the molecular Bose-Einstein condensate is a ferroelectric material that is fully disordered by quantum fluctuations.