The interplay between spin and motional degrees of freedom in interacting electron systems has been a long-standing research topic in condensed matter physics. Interactions can modify the behavior of individual electrons and give rise to emergent collective phenomena such as superconductivity and colossal magnetoresistance. Theoretical understanding of non-equilibrium dynamics in interacting fermionic matter is limited, however, and many open questions remain. Ultracold atomic Fermi gases, with precisely controllable parameters, offer an outstanding opportunity to investigate the emergence of collective behavior in out-of-equilibrium settings. In this thesis we will describe how an optical lattice clock operated with neutral Fermionic atoms can be turned into a quantum simulator of charged particles in a strong magnetic field. We will then discuss the counterintuitive notion that weak interactions in a Fermi gas can lead to large scale collective behavior and global correlations. These ideas are being tested experimentally at JILA and the University of Toronto. We also investigate in detail the so-called spin model approximation which is used extensively throughout this thesis.
The interplay between spin and motional degrees of freedom in interacting electron systems has been a long-standing research topic in condensed matter physics. Interactions can modify the behavior of individual electrons and give rise to emergent collective phenomena such as superconductivity and colossal magnetoresistance. Theoretical understanding of non-equilibrium dynamics in interacting fermionic matter is limited, however, and many open questions remain. Ultracold atomic Fermi gases, with precisely controllable parameters, offer an outstanding opportunity to investigate the emergence of collective behavior in out-of-equilibrium settings. In this thesis we will describe how an optical lattice clock operated with neutral Fermionic atoms can be turned into a quantum simulator of charged particles in a strong magnetic field. We will then discuss the counterintuitive notion that weak interactions in a Fermi gas can lead to large scale collective behavior and global correlations. These ideas are being tested experimentally at JILA and the University of Toronto. We also investigate in detail the so-called spin model approximation which is used extensively throughout this thesis.
The study of out-of-equilibrium dynamics in ultra-cold gases is a new and exciting field, driven largely by the recent experimental advances in controlling and imaging cold clouds. The experimental and theoretical work thus far has been somewhat exploratory and largely numerical in nature, as the very paradigms for thinking about these systems are not well established. In this thesis I consider several different scenarios of ultra-cold bosonic and fermionic gases driven out of equilibrium and study their properties. In Chapter 1, I provide an overview of the phenomenology of ultra-cold gases, highlighting the timescales governing these systems and how the experimentalist can tune them. I discuss how cold gases can be cooled and trapped and discuss the basic physics behind optical lattices. I also discuss experimental probes of these gases, in particular the new high resolution imaging techniques developed recently at Chicago, Munich and Harvard. In Chapter 2, I discuss an early experiment (circa. 2008) which observed long lived spin dynamics in a thermal spin-1/2 Fermi gas. This experiment is an nice illustration of interesting physics resulting from the separation of timescales between spin and collisional dynamics. In my opinion, it is an excellent example of why cold gases are naturally suited to studying non-equilibrium dynamics. I simulate the experiment numerically using a collisionless Boltzmann equation and explain the observed spin dynamics both qualitatively and quantitively. In Chapter 3, I continue the discussion of spin waves in thermal gases by extending previous works on spin-1/2 gases to spin-1 Bose gases. In contrast to Chapter 2, the bulk of the work in this Chapter is analytic in nature. In particular, I find a spin wave instability in the thermal spin-1 Bose gas, which is the high temperature analog of the polar to ferromagnetic transition in a spin-1 Bose Einstein condensate. In Chapter 3, I turn my attention to bosonic systems and briefly review the the Bogoliubov mean-field theory. I calculate the momentum distribution and density-density correlation function of an interacting Bose gas within the Bogoliubov framework. Then I consider bosons in an optical lattice, and introduce the Bose Hubbard model. I calculate the mean-field phase diagram of the Bose Hubbard model and then consider fluctuations about the mean field, and derive the excitation spectrum of the lattice gas in the superfluid and insulating regimes. In Chapter 4, I ask what we learn by studying the dynamics of correlation functions following a sudden change in the interactions in a superfluid. Using the Bogoliubov theory developed in Chapter 3, I will show how the underlying excitation spectrum influences the long and short time behavior of the correlation functions. By considering a lattice dispersion, I study the analogous problem in a weak optical lattice and discuss how the lattice dispersion leads to additional features in the correlation functions. I will also discuss the timescale governing the revival of the condensate fraction in a quantum depleted gas. In Chapter 5, I derive equations of motion governing the dynamics of one and two body correlation functions in the single-band Bose Hubbard model, applicable to bosons in deep lattices. I then consider a simple quench from a Mott insulating initial state to a weakly interacting final state and produce analytic expressions describing the dynamics of correlations following such a quench. I discuss the timescale for the development of long range order following such a quench. I study the problem of chapter 4 using an equations of motion approach. This approach complements the Bogoliubov approach of Chapter 4. First, I derive exact expressions for a quench to a non-interacting state. I then consider how interactions redistribute quasi-momentum to first order in perturbation theory in different dimensions. In Chapter 6, I calculate the relevant timescales for local and global dynamics in trapped lattice Bose gases, a work done in collaboration with Dr. Kaden R. A Hazzard. Using a time-dependent Gutzwiller mean-field theory, I show that the timescale for local equilibration in these systems is fast in experimental terms. I then show that due to the spatial inhomogeneities inherent to cold gases, achieving global equilibrium can be quite complicated, sometimes taking longer than the lifetime of the experiment, an issue of practical importance to current day experiments. I continue this discussion in Chapter 7 which is a collaborative work with experimentalists David McKay and Prof. Brian DeMarco from the University of Toronto and the University of Illinois, Urbana Champaign. Using experimental and numerical methods, we show that the rapid timescales for local dynamics in interacting systems invalidates a frequently used cold atom technique for mapping out the momentum distribution of atoms in an optical lattice.
Interactions between quantum particles can give rise to behaviors greater than the sum of their parts. The low-dimensional cold atomic framework provides a unique platform with exquisite control and enhanced correlations to develop a deeper understanding of such quantum phenomena, with promise for emerging technologies. In this thesis, I study novel quantum many-body physics in spinor gases trapped in optical lattices and develop efficient theoretical tools for such investigations. My work illustrates the central role of spin and charge degrees of freedom for comprehending and manipulating intricate quantum behaviors. With a broad goal of understanding the emergent physics in strongly correlated many-body systems, in Chapter 2, I investigate the two-component coupled Bose gas. An unprecedented phase emerges from the coupling of two components in the nearest-neighbor sites via a resonant two-photon Raman transition. Furthermore, coupling provides a novel tuning knob for the controlled manipulation of spin phases. Probing for behaviors away from the Mott state, the limitations of existing theoretical approaches are exposed. To address this, in Chapter 3, I develop a powerful theoretical framework for the unrestricted study of strongly correlated systems, valid even for large spin systems. This generalized effective spin-chain (GESC) formalism has numerous advantages: elegant mathematical form, computationally efficient parameterization, generalized for arbitrary spin and statistics, and universality: not limited to lattice systems. Importantly, leveraging a spin–charge separated form, it provides a unique vantage into system behaviors originating from quantum fluctuations. Motivated by the immense potential of anyons in cold atomic setups, in Chapter 4, I investigate the combined effect of fractional statistics and the presence of multiple components on their ground state and dynamical properties. This reveals the potential of statistical-phase-induced transition between different system phenomena. The GESC formalism is extended to consider anyons and used to obtain insights into the origin of exchange-phase-dependent and independent behavior. I demonstrate the versatility of the GESC formalism, in Chapter 5, to Bose–Fermi mixtures, beyond one-dimensional systems, and to consider long-range interactions. In doing so, avenues are provided for leveraging the immense utility of this formalism in exploring the novel physics such systems have to offer.
Strongly correlated quantum systems display a myriad of complex, fascinating behaviour. The competition between charge, spin, orbital, or lattice degrees of freedom and their respective energy scales gives rise to rich and complex emergent phases. More recently, the non-equilibrium properties of correlated quantum many-body systems have come into the focus of active research, with remarkable advances. While the advent of tensor network based simulations on the theoretical side has allowed access to the full time-evolution of the quantum state as it traverses the Hilbert space, the experimental progress in the ultracold atom community has allowed physicists to enter the paradigm of analog quantum simulation. Their tunability and isolation from the environment makes them ideal platforms to emulate and study open problems in condensed matter physics and go beyond the simulational capabilities of state of the art classical simulations. In this thesis, we explore the dynamics of correlated Fermi gases. We develop and present different facets of applicability of radiofrequency modulation techniques to drive the system out of equilibrium. We begin by considering a homogeneous, three-dimensional Fermi gas in the BCS-BEC crossover and develop an off-resonant radiofrequency transfer scheme to excite the Higgs mode of the superfluid. In a subsequent study we investigate the tunability of the coherence between Cooper pairs by tuning the duration of interaction ramps of the internal interaction strength. These works highlight the possibility to externally tune and stabilise complex quantum many-body states away from equilibrium. Using quasi-exact matrix product state simulations, we study the response of an attractively interacting, one-dimensional Fermi-Hubbard model to weak radiofrequency perturbations. We reveal the emergence of two distinct dynamical regimes in the time evolution and are able to relate it back to the underlying excitation spectrum of the system. Finally, we explore the possibility to perform quantum quenches through radiofrequency π-pulses, achieving nearly complete population transfer between different interacting fermionic states. We reveal non-trivial dynamical effects in the pair correlation of the final state, as well as the excitation of a collective trap mode of the system.
This thesis explores certain extraordinary phenomena that occur when a gas of neutral atoms is cooled to the coldest temperatures in the universe --- much colder, in fact, than the electromagnetic radiation that permeates the vacuum of interstellar space. At those extreme temperatures, quantum effects dominate and the collective behaviour of the atoms can have unexpected consequences. For example, Bose-Einstein condensation may occur where the atoms lose their individual identities to coalesce into a macroscopic quantum particle. Although such ultracold atomic gases are interesting in their own right, much of the excitement generated in this field is due to the possibility that studying these gases could shed light on intractable problems in other areas of physics. This is predominantly due to the uniquely high degree of control over various physical parameters that ultracold atomic gases afford to experimentalists. Recent technological advances exploit this advantage to study quantum phenomena in a detail that would not be possible in other systems. For instance, atoms can be made to attract or repel each other, the strength of this interaction can be set to almost any value, and external potentials of various geometries and periodicities can be introduced. In this way, atoms can be used to model phenomena as diverse as the quark-gluon plasmas arising in high-energy particle physics, the colour superfluids conjectured to exist in the core of neutron stars, and the high-temperature superconductivity exhibited by electrons on the ion lattice of certain compounds. Indeed, ultracold atomic gases also have a demonstrated applicability to quantum information and computation. Due to a subtle interplay between electronic and nuclear spins known as the hyperfine interaction, atoms can have either an integer or half-integer total spin quantum number, making them either bosonic or fermionic at low temperatures, respectively. With the exception of chapter 7, the work presented here concerns fermionic atoms in periodic potential formed by interfering laser beams. Indeed, the standing light wave created by the interfering beams gives rise to a lattice potential because of the Stark effect which couples the electronic energy levels of the atoms to the spatially undulating electric field. Furthermore, fermionic atoms can be prepared in two different hyperfine states corresponding to the the \\spin-up" and \\spin-down" quantum states, and as such mimic electrons moving in the lattice structure of solids. This system is well described by the famous Hubbard model which we introduce in chapter 2 and, under certain conditions, undergoes a phase transition into the N eel state which believed to be a precursor to superconductivity in certain high-temperature superconductors. In chapter 3, we calculate precisely how the N eel state may be achieved in an ultracold fermionic atom gas. When the number of spin-up and spin-down atoms is unequal the system becomes spin-canted and exhibits both ferro- and antiferromagnetic characteristics, as we show in chapter 4. We also nd there are topological excitations present in the quantum spin texture known as merons which have never unambiguously been observed before. In order to form a Bose-Einstein condensate, fermionic atoms must rst form pairs, and can do so in two contrasting ways. The relationship between these two qualitatively di erent forms of pairing is described in chapter 5, and we examine how these two types of pairs transform into one another in an optical lattice in chapter 6. Finally, chapter 7 is a detailed eld-theoretic study of pairing as it occurs in an ultracold Bose gas. There, we nd there is an intriguing bosonic analogy of the two forms of fermion pairing and explore the properties of these pairs.
Recent experiments with dilute trapped Fermi gases observed that weak interactions can drastically modify spin transport dynamics and give rise to robust collective effects including global demagnetization, macroscopic spin waves, spin segregation, and spin self-rephasing. In this Letter, we develop a framework for studying the dynamics of weakly interacting fermionic gases following a spin-dependent change of the trapping potential which illuminates the interplay between spin, motion, Fermi statistics, and interactions. The key idea is the projection of the state of the system onto a set of lattice spin models defined on the single-particle mode space. Collective phenomena, including the global spreading of quantum correlations in real space, arise as a consequence of the long-ranged character of the spin model couplings. This approach achieves good agreement with prior measurements and suggests a number of directions for future experiments.
Advances in experiments on dilute ultracold atomic gases have given us access to highly tunable quantum systems. In particular, there have been substantial improvements in achieving different kinds of interaction between atoms. As a result, utracold atomic gases oer an ideal platform to simulate many-body phenomena in condensed matter physics, and engineer other novel phenomena that are a result of the exotic interactions produced between atoms. In this dissertation, I present a series of studies that explore the physics of dilute ultracold atomic gases in different settings. In each setting, I explore a different form of the inter-particle interaction. Motivated by experiments which induce artificial spin-orbit coupling for cold fermions, I explore this system in my first project. In this project, I propose a method to perform universal quantum computation using the excitations of interacting spin-orbit coupled fermions, in which effective p-wave interactions lead to the formation of a topological superfluid. Motivated by experiments which explore the physics of exotic interactions between atoms trapped inside optical cavities, I explore this system in a second project. I calculate the phase diagram of lattice bosons trapped in an optical cavity, where the cavity modes mediates effective global range checkerboard interactions between the atoms. I compare this phase diagram with one that was recently measured experimentally. In two other projects, I explore quantum simulation of condensed matter phenomena due to spin-dependent interactions between particles. I propose a method to produce tunable spin-dependent interactions between atoms, using an optical Feshbach resonance. In one project, I use these spin-dependent interactions in an ultracold Bose-Fermi system, and propose a method to produce the Kondo model. I propose an experiment to directly observe the Kondo effect in this system. In another project, I propose using lattice bosons with a large hyperfine spin, which have Feshbach-induced spin-dependent interactions, to produce a quantum dimer model. I propose an experiment to detect the ground state in this system. In a final project, I develop tools to simulate the dynamics of fermionic superfluids in which fermions interact via a short-range interaction.