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Scientific Reports

Population density gratings induced by few-cycle optical pulses in a resonant medium

Rostislav M. Arkhipov, A. V. Pakhomov, Mikhail V. Arkhipov, Ihar Babushkin, Ayhan Demircan, Uwe Morgner, Nikolay N. Rosanov

Published Sep 25, 2017• 52 citations
Publisher

Abstract

Creation, erasing and ultrafast control of population density gratings using few-cycle optical pulses coherently interacting with resonant medium is discussed. In contrast to the commonly used schemes, here the pulses do not need to overlap in the medium, interaction between the pulses is mediated by excitation of polarization waves. We investigate the details of the dynamics arising in such ultrashort pulse scheme and develop an analytical theory demonstrating the importance of the phase memory effects in the dynamics.

DOI
10.1038/s41598-017-12267-w

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Creation, erasing and ultrafast control of population density gratings using few-cycle optical pulses coherently interacting with resonant medium is discussed. In contrast to the commonly used schemes, here the pulses do not need to overlap in the medium, interaction between the pulses is mediated by excitation of polarization waves. We investigate the details of the dynamics arising in such ultrashort pulse scheme and develop an analytical theory demonstrating the importance of the phase memory effects in the dynamics.
In the regime of resonant coherent light-matter interaction, light pulses may interact with each other indirectly via a polarization wave created by the other pulse. We show that such interaction allows fast creation and erasing of high-contrast dynamic population density gratings, as well as control of their period in a few-cycle regime. Our scheme uses counter-propagating optical pulses, which do not cross each other in the medium. The mechanism is able to work with pulse durations up to the single-cycle limit. Somewhat surprisingly, ultrafast grating wave vector control requires the generation of polarization waves with the phase velocity much smaller than that of light.
Abstract Recently, the possibility of the creation, erasing and ultrafast control of polarization and population inversion gratings by sequences of few-cycle bipolar pulses interacting with a medium in a resonant and coherent way was predicted. In this case, the overlapping of pulses in the medium is not needed for the creation of gratings. In this paper, we study the possibility of the ultrafast creation and control of spatial periodic gratings in a resonant medium when subcycle unipolar pulses (that is ones containing the constant spectral component of an electric field) propagate in the coherent regime.
Electromagnetically induced gratings (EMIGs) of atomic populations are formed in the resonant media at the interference of two or more overlapping monochromatic beams. They are of great interest in the view of the possibility of numerous applications in optics and spectroscopy. The significant progress has been achieved recently in the generation of ultrashort femto- and attosecond pulses. Such ultrashort pulses cannot provide an interference pattern because the region of their overlapping is very small and insufficient to form even few interference fringes. However, when the pulse duration is shorter than the relaxation times in the medium in the presence of a coherent interaction with the medium, they can rapidly change of the population of atomic levels owing to carrier-wave Rabi flopping. In this case, population gratings can be formed without the instantaneous overlapping of ultrashort light pulses in the medium. The latest results on the production and control of EMIGs received by means of a sequence of single- and subcycle light pulses have been reviewed. It has been shown that the unipolar subcycle pulses can be used to control more efficiently the EMIGs compared to multipolar multicycle pulses. Various applications of these gratings have been discussed in the ultrafast optics and for the holographic recording.
Abstract Electromagnetically induced gratings (EIG) are created by standing-wave laser field in resonant media. Such gratings can be also created by few-cycle electromagnetic pulses counter-propagating in the medium via coherent Rabi oscillations of atomic inversion. In this case, instantaneous cross-section of the pulses in the medium is not necessary for grating formation. In this paper, we revise our recent results in study of such grating formation and their control by few-cycle pulses coherently propagating in a resonant medium. We demonstrate the grating formation and their control in three-level medium excited by three subcycle THz pulses.