This thesis undertakes new investigations with respect to hybrid systems that interacts microwave radiation with spin and phonons. In this work, YSO and YAP samples had their permittivity tensor characterized with YAP subjected to an electron spin resonance spectroscopy. Furthermore, reentrant cavities were explored to promote the interaction of photons with different physical systems. Hence, a piezoelectric controlled cavity was developed and upgraded to a superconducting tunable device, and a parametric transducer based on optomechanical coupling was tested. Finally, an optoacoustic device was built allowing the coupling between photons and phonons in a quartz bulk acoustic wave resonator.
This thesis undertakes new investigations with respect to hybrid systems that interacts microwave radiation with spin and phonons. In this work, YSO and YAP samples had their permittivity tensor characterized with YAP subjected to an electron spin resonance spectroscopy. Furthermore, reentrant cavities were explored to promote the interaction of photons with different physical systems. Hence, a piezoelectric controlled cavity was developed and upgraded to a superconducting tunable device, and a parametric transducer based on optomechanical coupling was tested. Finally, an optoacoustic device was built allowing the coupling between photons and phonons in a quartz bulk acoustic wave resonator.
Microscale and nanoscale mechanical resonators have been used in advanced technological applications, from high precision time keeping and mass sensing, to processing high frequency signals in mobile communications. In the last few decades, they have been an important part of progress in the field of quantum information and metrology and have been proposed as quantum memories or transducers for measuring or connecting different types of quantum systems. The field of cavity optomechanics and electromechanics is concerned with coupling the electromagnetic field of a resonant optical cavity or electrical circuit to mechanical motion. These systems provide potential means to control and engineer the state of a mechanical object at the quantum level. This thesis contains the description of mechanical systems in megahertz to a few hundred megahertz frequency range formed by nano-fabricating photonic, phononic, and electrical circuits on a chip. These structures are designed to provide a large radiation pressure coupling between mechanical motion and electromagnetic fields to address and manipulate motional degrees of freedom. Qualitatively novel quantum effects are expected when one takes a step beyond linear coupling and exploits higher order interactions. To that end, we integrate electrical, mechanical and photonic structures in a multimode photonic crystal structure to observe "x2-coupling", where the optical cavity frequency is coupled to the square of the mechanical displacement. Moreover, we have developed two integrated on-chip platforms based on Si3N4 and Si nanomembranes capable of interfacing superconducting qubits and optical photons and realizing reversible microwave-to-optical conversion. We employ radiation pressure to cool these mechanical resonators to their quantum ground state. Finally, we demonstrate a form of electromechanical crystal for coupling microwave photons and hypersonic phonons of frequency ωm/2π = 0.425 GHz by capacitively coupling a phononic crystal acoustic cavity to a superconducting microwave resonator. Moving to higher frequency acoustic cavities not only facilitates the integration of electromechanical circuits and nanophotonic systems capable of operation in the resolved sideband limit of optomechanics for noise-free quantum signal conversion, but it opens up the possibility of using phonons as information carriers via phononic circuits. Utilizing a two-photon resonance condition for efficient microwave pumping and phononic bandgap shield to eliminate acoustic radiation, we achieve large cooperative electromechanical coupling (C ≈ 30) and intrinsic decay time of 2.3 ms. Moreover, electrical read-out of the phonon occupancy shows that the acoustic mode thermalizes close to its quantum ground-state of motion (phonon occupancy nm=1.5) at a fridge temperature of Tf = 10 mK. We conclude by considering several designs and fabrication improvements to the hypersonic electromechanical crystals that would enable them to perform quantum conversion between the electrical and acoustic domain.
We introduce a hybrid tripartite quantum system for strong coupling between a semiconductor spin, a mechanical phonon, and a microwave photon. Consisting of a piezoelectric resonator with an integrated diamond strain concentrator, this system achieves microwave-acoustic and spin-acoustic coupling rates ∼MHz or greater, allowing for simultaneous ultra-high cooperativities (∼103 and ∼102, respectively). From finite-element modeling and master equation simulations, we estimate photon-to-spin quantum state transfer fidelities exceeding 0.97 based on separately demonstrated device parameters. We anticipate that this device will enable hybrid quantum architectures that leverage the advantages of both superconducting circuits and solid-state spins for information processing, memory, and networking.
The past 20 years has seen rapid developments in circuit quantum electrodynamics, where superconducting qubits and resonators are used to control and study quantum light-matter interaction at a fundamental level. The development of this field is strongly influenced by quantum information science and the prospect of realizing quantum computation, but also opens up opportunities for combinations of different physical systems and research areas. Superconducting circuits in the microwave domain offer a versatile platform for interfacing with other quantum systems thanks to strong nonlinearities and zero-point fluctuations, as well as flexibility in design and fabrication. Hybrid quantum systems based on circuit quantum electrodynamics could enable novel functionalities by exploiting the strengths of the individual components.This thesis covers experiments coupling superconducting circuits to surface acoustic waves (SAWs), mechanical waves propagating along the surface of a solid. Strong coupling can be engineered using the piezoelectric properties of GaAs substrates, and our experiments exploit this to investigate phenomena in quantum field-matter interaction. A key property of surface acoustic waves is the slow propagation speed, typically five orders of magnitude slower than light in vacuum, and the associated short wavelength. This enables the giant atom regime where the artificial atom in the form of a superconducting circuit is large compared to the wavelength of interacting SAW radiation, a condition which is difficult to realize in other systems. Experiments described in this thesis use these properties to demonstrate electromagnetically induced transparency for a mechanical mode, as well as non-Markovian interactions between an artificial giant atom and the SAW field. When the SAW field is confined to a resonant cavity, the short wavelength allows multimode spectra suitable for interacting with a frequency comb. We use a multimode SAW resonator to characterize the ensemble of microscopic two-level system defects with a two-tone spectroscopy approach. Finally, we introduce a hybrid superconducting-SAW resonator with applications in quantum information processing in mind. Experiments with this device demonstrate entanglement of SAW modes, and show promising results on the way to engineer cluster states for quantum computation in continuous variables.
Hybrid systems that couple superconducting qubits to mechanical oscillators facilitate quantum control of individual phonons and have the potential to enable compact, highly coherent quantum memories and processors. To date, however, the utility of hybrid quantum acoustic devices has been limited by poor qubit and mechanical coherence times that are far shorter than those exhibited by their unhybridized counterparts. A primary challenge lies in the intrinsic nature of elastic waves in solids: the slow speed of sound results in a dense spectrum of acoustic modes, making it difficult to prevent spontaneous emission of the qubit into phononic degrees of freedom. In this thesis, I will present a systematic effort to suppress loss mechanisms in superconducting qubits and mechanical resonators in the context of circuit quantum acoustics. I begin by demonstrating the use of crystallographic orientation optimization to passively suppress diffraction losses in narrow-aperture quartz surface acoustic wave (SAW) resonators. We then study the coupling of SAW resonators to a quasi-continuum of bulk acoustic modes; this motivates us to abandon bulk piezoelectric media in favor of bandgap-protected thin-film devices. By fabricating suspended phononic crystal resonators from thin-film quartz, we demonstrate an order-of-magnitude improvement in the coherence of this class of devices. I conclude by presenting preliminary measurements of a new flip-chip architecture for circuit quantum acoustics -- the `acoustic trampoline' -- that is designed to maximize qubit-mechanical coupling while simultaneously suppressing spontaneous acoustic emission.
Progress in the emerging field of engineered quantum systems requires the development of devices that can act as quantum memories. In this thesis, a novel spectroscopic technique using electron spin resonance (ESR) is presented. Microwave whispering gallery modes (WGM) in cylindrical dielectric resonators are used to probe paramagnetic impurities at millikelvin temperatures under the influence of an applied dc magnetic field. This technique couples the naturally high quality factor and the relatively high magnetic filling factor of WGMs in crystalline hosts. Precision spectroscopy has been performed on a number of dielectric samples including, sapphire, ruby, quartz, yttrium orthosilicate (YSO) and yttrium aluminium garnet (YAG). Spectroscopic characterisation of sapphire reveals trace ion impurities at parts per billion, which have been used to control strong coupling between the WGM doublets. Moreover, time-reversal symmetry breaking has been observed when a WGM interacts with an ESR, a result of selection rules being created as a consequence of conservation of angular momentum. Following this, interactions between WGM microwave photons and spin resonances are shown in a range of systems. Results achieved include coupling between WGM photons and Cr3+ ions in ruby with normal mode splitting on the order of 600 MHz at 13.9 GHz, the coupling of iron group ion impurities to WGM photons in YSO, which also revealed a strong coupling regime with very low magnetic field, and coupling of Er3+ to WGMs in YAG with evidence of dilute ferromagnetism - the first observation of such an effect outside of iron group doped semiconductors. In addition a novel double-post re-entrant cavity is presented, which is able to focus the rf magnetic field into a small sample, in this case a sub-millimetre sized Yttrium Iron Garnet (YIG) ferrite microsphere that supports magnon resonances. Ultra-high cooperatively of 105 between photon and magnon modes is demonstrated at millikelvin temperatures and microwave frequencies. A coupling strength (normal mode splitting) of 2 GHz at 20 GHz, equivalent to 76 cavity linewidths, is achieved for the bright cavity mode. This constitutes about 10% of the photon energy and shows that ultra-strong coupling is possible in spin systems at microwave frequencies.
Acoustic waves are versatile excitations that couple to many different physical systems. They interact with optical fields in optomechanics, with spin defects through strain, and with superconducting circuits via capacitive or piezoelectric mechanisms. This versatility has motivated their use in hybrid quantum systems for quantum transduction, qubit control, and precision sensing, among other applications. In this thesis, the focus is on the optimization of microwave-to-acoustic coupling between superconducting circuits and Lamb modes in suspend thin-film lithium niobate (LiNbO₃). We leverage the strong piezoelectricity of this material to engineer strong interactions.The first part of the work addresses linear transduction. IDTs require impedance matching to operate efficiently, but this generally imposes a trade-off between efficiency and bandwidth. An optimal design can be identified in theory but is difficult to reach with standard microwave engineering. Here, high-impedance SQUID arrays are employed as linear, tunable inductors to realize the necessary impedance transformation. This approach enables transducers that operate close to the efficiency-bandwidth limit imposed by the piezoelectric coupling strength of LiNbO₃. The design strategy is applied to different types of devices: standard bi-directional IDTs, unidirectional IDTs where acoustic mirrors recover backward-emitted waves, and single-mode IDTs where additional transverse confinement produces quasi-one-dimensional propagation. Among these, unidirectional IDTs achieve unprecedented coupling, with efficiency–bandwidth products of ≈440 MHz and peak efficiencies of 62%. By leveraging flux tunability of SQUIDs we get tunable couplers between microwave circuits and Lamb-wave resonators.The second part investigates the nonlinear regime, where transmon qubits are coupled to Lamb-wave resonators. Unlike the high-Q but weakly coupled resonators often used in the literature, LiNbO₃ offers strong piezoelectric interactions that enable access to very strong coupling even without extremely high quality factors.Overall, this thesis establishes efficient linear transducers and explores strong nonlinear interactions, advancing superconducting-acoustic interfaces based on LiNbO₃. These results extend the superconducting circuit toolbox with sensitive acoustic elements and open pathways toward hybrid applications such as microwave-optical transduction, acoustic spectroscopy, and fundamental experiments exploring the interplay of quantum mechanics and gravity.