Quantum sources that provide broadband biphotons entangled in both polarization and time-energy degrees of freedom are a rich quantum resource that finds many applications in quantum communication, sensing, and metrology. Creating such a source while maintaining high entanglement quality over a broad spectral range is a challenge, which conventionally requires various compensation steps to erase temporal, spectral, or spatial distinguishabilities. Here, we point out that in fact compensation is not always necessary. The key to generate broadband polarization-entangled biphotons via type-II spontaneous parametric downcoversion (SPDC) without compensation is to use nonlinear materials with sufficiently low group birefringence that the biphoton bandwidth becomes dispersion-limited. Most nonlinear crystals or waveguides cannot meet this condition, but it is easily met in fiber-based systems. We reveal the interplay of group birefringence and dispersion on SPDC bandwidth and polarization entanglement quality. We show that periodically poled silica fiber (PPSF) is an ideal medium to generate high-concurrence (>0.977) polarization-entangled photons over a broad spectral range (>77nm), directly and without compensation. This is the highest polarization-entanglement concurrence reported that is maintained over a broad spectral range from a compensation-free source.
Quantum sources that provide broadband biphotons entangled in both polarization and time-energy degrees of freedom are a rich quantum resource that finds many applications in quantum communication, sensing, and metrology. Creating such a source while maintaining high entanglement quality over a broad spectral range is a challenge, which conventionally requires various compensation steps to erase temporal, spectral, or spatial distinguishabilities. Here, we point out that in fact compensation is not always necessary. The key to generate broadband polarization-entangled biphotons via type-II spontaneous parametric downcoversion (SPDC) without compensation is to use nonlinear materials with sufficiently low group birefringence that the biphoton bandwidth becomes dispersion-limited. Most nonlinear crystals or waveguides cannot meet this condition, but it is easily met in fiber-based systems. We reveal the interplay of group birefringence and dispersion on SPDC bandwidth and polarization entanglement quality. We show that periodically poled silica fiber (PPSF) is an ideal medium to generate high-concurrence (>0.977) polarization-entangled photons over a broad spectral range (>77nm), directly and without compensation. This is the highest polarization-entanglement concurrence reported that is maintained over a broad spectral range from a compensation-free source.
Entangled photons are a fundamental resource in quantum applications. Broadband entangled photon sources have been used in applications such as high-resolution quantum sensing and wavelength-multiplexed quantum communication. In particular, in fiber-based quantum applications such as long-distance quantum clock synchronization and quantum key distribution in deployed fiber networks, a practical entangled source that is robust and compatible with silica fiber is highly sought after. Periodically poled silica fiber (PPSF) has been demonstrated to be a promising resource of entangled photon-pairs. PPSF uses the induced second-order nonlinearity in poled fiber to generate polarization-entangled photon pairs based on type-II spontaneous parametric down-conversion. The negligible group birefringence of the PPSF ensures high-quality and broadband polarization entanglement without compensation, making it particularly suitable for these quantum applications. The PPSF-based source has a lot of potentials to be tapped because of its high entanglement quality, broadband emission bandwidth, simple structure, and its compatibility with the existing fiber infrastructure. In this thesis, I focus on the development of the PPSF-based entangled photon sources. I first investigate the design and the manufacturing process of the PPSF where I try to produce PPSF with improved performance and innovative properties. Next, I study the compensation-free nature of the PPSF-based polarization entanglement source and discuss the interplay between dispersion, birefringence, emission bandwidth, and polarization entanglement. Based on the theory, a commercial PPSF-based photon-pair source prototype is developed and patented. It has to my knowledge the simplest design of all polarization-entangled sources reported so far in the literature. Furthermore, I broaden the biphoton bandwidth by building a PPSF photon-pair source that emits biphotons at telecom O-band. With more than 24THz bandwidth, the biphotons generated in this source are the broadest of all O-band polarization-entangled photon sources reported to my knowledge. I also propose and experimentally demonstrate a polarization-frequency hyperentangled photon source using PPSF, which provides higher dimensionality by making use of entanglement in multiple degrees of freedom. Overall, this thesis contributes to the development of PPSF technology for practical quantum applications. I anticipate that the PPSF-based photon-pair source will play an important role in the era of quantum technology.
In this Letter, we report a polarization-entangled photon-pair source based on type-II spontaneous parametric downconversion at telecom O-band in periodically poled silica fiber (PPSF). The photon-pair source exhibits more than 130 nm ( ∼ 24 T H z ) emission bandwidth centered at 1306.6 nm. The broad emission spectrum results in a short biphoton correlation time, and we experimentally demonstrate a Hong–Ou–Mandel interference dip with a full width of 26.6 fs at half-maximum. Owing to the low birefringence of the PPSF, the biphotons generated from type-II SPDC are polarization-entangled over the entire emission bandwidth, with a measured fidelity to a maximally entangled state greater than 95.4%. The biphoton source provides the broadest bandwidth entangled biphotons at O-band to our knowledge.
The time-energy entangled photon source is a core resource in quantum key distribution, quantum teleportation, and quantum metrology. The output of orthogonally polarized photon pairs can enhance the effective coincidence counts of the entangled source in these applications. Additionally, an all-fiber entangled source offers small size and high mobility advantages. However, most current orthogonally polarized all-fiber time-energy entangled sources are limited to a bandwidth of around 1 nm, which is detrimental to the effective utilization of channel resources in fiber networks and restricts precision in quantum metrology. To address this issue, we employ a fiber-coupled 775 nm narrow linewidth pump laser in a periodically poled lithium niobate (PPLN) waveguide to achieve type-II spontaneous parametric down-conversion (SPDC). This results in an all-fiber orthogonally polarized time-energy entangled photon source with a bandwidth greater than 7 nm. We measured the single counts, coincidence counts, coincidence to accidental coincidence ratio (CAR), single photon spectra, and joint spectral intensity of the entangled source, calculating the Schmidt number S = 7.8. Furthermore, we measured Hong-Ou-Mandel (HOM) interference by inserting two 2 nm bandpass filters, and the interference visibility remained around 95.8% after continuous operation for 3 hours. The experimental results indicate that while maintaining an all-fiber structure, this source possesses a broadband range, low noise, and high stability, providing efficient and reliable biphoton resources for applications in quantum communication, quantum networks, and precision metrology.
We demonstrate a broadband entangled photon source based on a single-pass, type-0 phase-matched, non-collinear spontaneous parametric down-conversion (SPDC) process. By spatially multiplexing the intrinsically random transverse momentum states of biphotons emitted in an annular spatial distribution from a single-frequency-pumped, 2-mm-long periodically poled KTP crystal, we generate polarization-entangled pair photons with a spectral bandwidth of ∼130 nm centered at 810 nm. The negligible group-velocity mismatch of the co-polarized near-degenerate photons in single-pass and low birefringence of standard optical components preserves indistinguishability across the broadband emission without phase compensation, enabling high-quality polarization entanglement over the entire emission bandwidth. The source achieves a brightness of 0.57 Mpairs/s/mW and a two-photon coherence length of 6.97 μm, while exhibiting an interference visibility exceeding 95%, a Bell–CHSH parameter of 2.526 ± 0.005 that remains stable over 12 h of continuous operation and violates the Bell inequality by more than 100 standard deviations, and a state fidelity of 96.3%. The generic scheme providing the broadest bandwidth entangled biphotons at 810 nm, to our knowledge, can readily be used for other wavelengths as required for multiparty quantum networks and quantum sensing applications.
We demonstrate a broadband entangled photon source based on a single-pass, type-0 phase-matched, non-collinear spontaneous parametric down-conversion (SPDC) process. By spatially multiplexing the intrinsically random transverse momentum states of biphotons emitted in an annular spatial distribution from a single-frequency-pumped, 2-mm-long periodically poled KTP crystal, we generate polarization-entangled pair photons with a spectral bandwidth of ∼130 nm centered at 810 nm. The negligible group-velocity mismatch of the co-polarized near-degenerate photons in single-pass and low birefringence of standard optical components preserves indistinguishability across the broadband emission without phase compensation, enabling high-quality polarization entanglement over the entire emission bandwidth. The source achieves a brightness of 0.57 Mpairs/s/mW and a two-photon coherence length of 6.97 μm, while exhibiting an interference visibility exceeding 95%, a Bell–CHSH parameter of 2.526 ± 0.005 that remains stable over 12 h of continuous operation and violates the Bell inequality by more than 100 standard deviations, and a state fidelity of 96.3%. The generic scheme providing the broadest bandwidth entangled biphotons at 810 nm, to our knowledge, can readily be used for other wavelengths as required for multiparty quantum networks and quantum sensing applications.
Fibre optics is a mature technology that revolutionized telecommunication. Quantum photonics is an emerging technology still under development. The fusion of the two can bring technologically-robust solutions for quantum applications. Here we give one concrete example of a fiber-optic entangled photon source. Free of alignment, fiber coupling or any birefringence compensating schemes, it is arguably world’s simplest polarization-entangled photon source, and perfectly compatible with the vast fibre-optic network infrastructure. Furthermore, using it to form a fibre-based nonlinear interferometer results in the coupling of the spectral domain with the polarization domain, and tunability in both domains. By manipulating the dispersion and birefringence properties of the linear medium in the interferometer, we experimentally demonstrate altering the biphoton spectrum through biphoton interference, as well as tuning the degree of polarization entanglement. Due to the low-birefringence nature of both the nonlinear and linear media in the interferometer, we can preserve the high-quality polarization entanglement while shaping the biphoton spectrum. Additionally, the coupling of the polarization degree of freedom with the spectral degree of freedom, allowing us to tune the degree of entanglement by simply tuning wavelength. Our fibre-based quantum entanglement sources demonstrate a great deal of flexibility in entanglement engineering for future fibre-optic quantum networks.