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Optical Bloch equations for simulating trapped-ion qubits

H. A. Janacek

Published Jan 1, 2015• 2 citations
Publisher

Abstract

This thesis describes work on numerical modelling of the 43Ca+ ion in a Paul trap using the optical Bloch equations. This is a challenging system to study, with many states involved in the internal dynamics. A major outcome is the development of a cooling scheme for the 146.09 gauss atomic clock transitions which makes use of a dark resonance. It is much more effective than methods that avoid coherent effects. The scheme is realised in experiment. Complicated fluorescence data is modelled very well, and predictions for the ion's motional temperature show good agreement with measured values. Data and fits for an ion that has been Doppler cooled below the Doppler limit are presented. I describe GLOBES, a set of routines that simulates an arbitrary ion in the presence of an arbitrary system of laser beams using the optical Bloch equations. Techniques used to efficiently calculate the steady state, analyse fluorescence scans and solve time-dependent problems for small and large times are discussed. A new routine SILVER IMPER that leapfrogs over the initial dynamics to model the approach to the steady state is introduced. Doppler cooling in 40Ca+ is analysed and two extensions made to the basic theory. The ‘excursion method’ of calculation takes account of the non-linear variation with velocity of the scattering rate. The ‘dynamic method’ allows for the fact that the ion may not be in equilibrium with the incident radiation during its oscillations, a necessity as the timescale of the external motion is of order the characteristic timescale of the internal motion for standard secular frequencies. This 'dynamic effect' is a general property of trapped ion systems and is also observed in a two-state system. A two-variable fluorescence scan taken from a four-laser, five-level system in 40Ca+ is analysed. Techniques to fit large data sets and automatically resolve resonant features are demonstrated. A general treatment of resonant behaviour in three, four and five level pump/probe systems is used to describe the data. This is verified by a second, tailor-made set of scans.

DOI
10.5287/ora-zbbkoxpjv

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Laser systems and a linear radiofrequency (rf) Paul trap with an integrated co-axial cavity have been developed for experiments in cavity QED and probabilistic entanglement. Single 40Ca+ ions and large Coulomb crystals have been trapped routinely and laser cooled with long trapping lifetimes. A technique to achieve precise overlap of the pseudopotential minimum of the rf-field with the cavity mode has been implemented through variable capacitors in the resonant rf-circuit used to drive the trap. Three-dimensional micromotion compensation has been implemented. An 894 nm laser has been frequency stabilised to a Pound-Drever-Hall cavity which is in turn stabilised to atomic Cs using polarisation spectroscopy. The Allan variance of the error signal has been reduced to less than a kilohertz on timescales greater than a second. A novel implementation of the scanning cavity transfer lock has been developed to transfer the stability of the 894 nm laser to the 397 nm ion cooling and 866 nm repumping lasers. The bandwidth of the system has been increased to 380 Hz and the Allan variance of the error signal has been reduced to less than ten kilohertz on timescales of greater than a second. The pseudopotential minimum of the rf field has been overlapped optimally with the optical cavity mode through mapping of the fluorescence from cavity-field repumped ions as a function of their displacement. Coupling to the cavity mode has been confirmed by observation of resonant fluorescence into the cavity mode using the cavity-assisted Raman transition process. The thesis demonstrates that the setup is ready for the controlled production of single photons with pre-determined polarisation states, and progression onto new schemes to entangle multiple ions that are coupled to the optical cavity mode.

•May 21, 2012•1 citation
This thesis describes work on numerical modelling of the 43Ca+ ion in a Paul trap using the optical Bloch equations. This is a challenging system to study, with many states involved in the internal dynamics. A major outcome is the development of a cooling scheme for the 146.09 gauss atomic clock transitions which makes use of a dark resonance. It is much more effective than methods that avoid coherent effects. The scheme is realised in experiment. Complicated fluorescence data is modelled very well, and predictions for the ion's motional temperature show good agreement with measured values. Data and fits for an ion that has been Doppler cooled below the Doppler limit are presented. I describe GLOBES, a set of routines that simulates an arbitrary ion in the presence of an arbitrary system of laser beams using the optical Bloch equations. Techniques used to efficiently calculate the steady state, analyse fluorescence scans and solve time-dependent problems for small and large times are discussed. A new routine SILVER IMPER that leapfrogs over the initial dynamics to model the approach to the steady state is introduced. Doppler cooling in 40Ca+ is analysed and two extensions made to the basic theory. The ‘excursion method’ of calculation takes account of the non-linear variation with velocity of the scattering rate. The ‘dynamic method’ allows for the fact that the ion may not be in equilibrium with the incident radiation during its oscillations, a necessity as the timescale of the external motion is of order the characteristic timescale of the internal motion for standard secular frequencies. This 'dynamic effect' is a general property of trapped ion systems and is also observed in a two-state system. A two-variable fluorescence scan taken from a four-laser, five-level system in 40Ca+ is analysed. Techniques to fit large data sets and automatically resolve resonant features are demonstrated. A general treatment of resonant behaviour in three, four and five level pump/probe systems is used to describe the data. This is verified by a second, tailor-made set of scans.
We demonstrate simple and robust methods for Doppler cooling and obtaining high fluorescence from trapped 43 Ca + ions at a magnetic field of 146 Gauss. This field gives access to a magnetic-field-independent 'atomic clock' qubit transition within the ground level hyperfine structure of the ion, but also causes the complex internal structure of the 64 states relevant to Doppler cooling to be spread over many times the atomic transition line-width. Using a time-dependent optical Bloch equation simulation of the system we develop a simple scheme to Doppler-cool the ion on a two-photon dark resonance, which is robust to typical experimental variations in laser intensities, detunings and polarizations. We experimentally demonstrate cooling to a temperature of 0.3 mK, slightly below the Doppler limit for the corresponding two-level system, and then use Raman sideband laser cooling to cool further to the ground states of the ion's radial motional modes. These methods will enable two-qubit entangling gates with this ion, which is one of the most promising qubits so far developed.
In this paper, we present a method to measure transient fluorescent dynamics with single trapped ions in a Paul trap. We use 40 Ca + ions that exhibit a Λ-type three-level system and measure the characteristic optical pumping times between the ground S 1/2 and the meta-stable D 3/2 levels. We prepare one of these states and then pump it to the opposite via the excited P 1/2 state. By measuring the scattered photons of the ion, we retrieve transient curves of the atomic fluorescence. These curves provide fundamental information about the atomic system, such as branching fractions and excited-state lifetimes, as well as experimental parameters like the efficiency of the detection system and the saturation parameter of one of the transitions. Finally, we study the time-dependent fluorescence as a function of optical power and detuning of the lasers and find a very good agreement with simulating the dynamics via a three-level open quantum system through a set of optical Bloch equations. Being able to record time-dependent fluorescence is of particular interest as it contains information about the temperature, cooling, and heating dynamics of the ion.
The outstanding degree of control over trapped ions in Paul traps gives rise to the development of novel quantum manipulation techniques. Optical transitions can be used for precise manipulation of internal and external states. This way, non-classical states can be created which are a key component of quantum algorithms based on quantum logic operations. This powerful optical toolbox enabled the trapped ion system to assume leadership in the field of quantum computation. This thesis addresses two major challenges in the field of micro ion trap quantum optics. The temperature dependence of the heating rate from the ion trap surface is analysed in a novel cryogenic micro ion trap. Furthermore segmented traps allow state manipulations by time dependent electrical potentials, generated by the control voltages. These electrical fields provide a fast and reliable control handle to the ions external degrees of freedom. Quantum computation in Paul trap arrays is based on a combination of ion crystal transport, splitting and merging operations, while laser driven quantum state manipulations are mainly carried out on small ion crystals. Within this thesis a basic building block was realised by performing transport operations with a single ground-state cooled ion. As a highlight of experimental achievements, shuttling in the non-adiabatic regime, on the timescale of the motional period was demonstrated with low residual energy transfer. For his endeavour a specialised low noise arbitrary function generator was designed and manufactured during this thesis. Arbitrary voltage ramps at a sampling rate of up to 2.5 MS/s on up to 12 channels allow the study of a novel excitation method by directly manipulating the ion using electrical forces. Accurate numerical simulations in combination with the fast high resolution voltage supply allow deterministic quantum manipulations via momentum kicks. I report the first experimental demonstration of displaced number states with trapped ions.
A two-ion pair in a linear Paul trap is extensively used in the research of the simplest quantum-logic system; however, there are few quantitative and comprehensive studies on the motional mode coupling of two-ion systems yet. This study proposes a method to investigate the motional mode coupling of sympathetically cooled two-ion crystals by quantifying three-dimensional (3D) secular spectra of trapped ions using molecular dynamics simulations. The 3D resonance peaks of the 40Ca+–27Al+ pair obtained by using this method were in good agreement with the 3D in- and out-of-phase modes predicted by the mode coupling theory for two ions in equilibrium and the frequency matching errors were lower than 2%. The obtained and predicted amplitudes of these modes were also qualitatively similar. It was observed that the strength of the sympathetic interaction of the 40Ca+–27Al+ pair was primarily determined by its axial in-phase coupling. In addition, the frequencies and amplitudes of the ion pair’s resonance modes (in all dimensions) were sensitive to the relative masses of the ion pair, and a decrease in the mass mismatch enhanced the sympathetic cooling rates. The sympathetic interactions of the 40Ca+–27Al+ pair were slightly weaker than those of the 24Mg+–27Al+ pair, but significantly stronger than those of 9Be+–27Al+. However, the Doppler cooling limit temperature of 40Ca+ is comparable to that of 9Be+ but lower than approximately half of that of 24Mg+. Furthermore, laser cooling systems for 40Ca+ are more reliable than those for 24Mg+ and 9Be+. Therefore, 40Ca+ is probably the best laser-cooled ion for sympathetic cooling and quantum-logic operations of 27Al+ and has particularly more notable comprehensive advantages in the development of high reliability, compact, and transportable 27Al+ optical clocks. This methodology may be extended to multi-ion systems, and it will greatly aid efforts to control the dynamic behaviors of sympathetic cooling as well as the development of low-heating-rate quantum logic clocks.
We describe a simple approach to the problem of incorporating the response time of an atom or ion being Doppler-cooled into the theory of the cooling process. The system being cooled does not in general respond instantly to the changing laser frequencies it experiences in its rest frame, and this ‘dynamic effect’ can affect significantly the temperatures attainable. It is particularly important for trapped ions when there is a slow decay out of the cooling cycle requiring the use of a repumping beam. We treat the cases of trapped ions with two and three internal states, then apply the theory to 40Ca+. For this ion experimental data exist showing the ion to be cold under conditions for which heating is predicted if the dynamic effect is neglected. The present theory accounts for the observed behaviour.
Laser systems and a linear radiofrequency (rf) Paul trap with an integrated co-axial cavity have been developed for experiments in cavity QED and probabilistic entanglement. Single 40Ca+ ions and large Coulomb crystals have been trapped routinely and laser cooled with long trapping lifetimes. A technique to achieve precise overlap of the pseudopotential minimum of the rf-field with the cavity mode has been implemented through variable capacitors in the resonant rf-circuit used to drive the trap. Three-dimensional micromotion compensation has been implemented. An 894 nm laser has been frequency stabilised to a Pound-Drever-Hall cavity which is in turn stabilised to atomic Cs using polarisation spectroscopy. The Allan variance of the error signal has been reduced to less than a kilohertz on timescales greater than a second. A novel implementation of the scanning cavity transfer lock has been developed to transfer the stability of the 894 nm laser to the 397 nm ion cooling and 866 nm repumping lasers. The bandwidth of the system has been increased to 380 Hz and the Allan variance of the error signal has been reduced to less than ten kilohertz on timescales of greater than a second. The pseudopotential minimum of the rf field has been overlapped optimally with the optical cavity mode through mapping of the fluorescence from cavity-field repumped ions as a function of their displacement. Coupling to the cavity mode has been confirmed by observation of resonant fluorescence into the cavity mode using the cavity-assisted Raman transition process. The thesis demonstrates that the setup is ready for the controlled production of single photons with pre-determined polarisation states, and progression onto new schemes to entangle multiple ions that are coupled to the optical cavity mode.