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Quantum Information Processing with Atomic Ensembles and Light

Klemens Hammerer

Published Jan 1, 2006• 8 citations
OpenAlex

Abstract

This thesis contributes to the theory of a light-matter quantum interface based on the Kerr-effect arising in the dispersive interaction of pulsed laser light with a spin-polarized atomic ensemble. The scattering process can be described on the basis of a simple, yet fully quantum mechanical model involving only a small number of bosonic modes referring to transverse spin components and quadratures of forward scattered light. Based on this model we derive protocols for the creation of entangled states of light and atoms and the teleportation of quantum states of light onto atoms employing this entanglement. Furthermore we present a protocol, which allows one to exchange the state of light and atoms and thus provides a quantum memory for states of the light field. For both, the storage and the teleportation of coherent states we prove a benchmark on the average fidelity, which is achievable by purely classical protocols. Both protocols allow one to significantly surpass this threshold and to demonstrate thereby a gain in employing quantum strategies. Under common experimental conditions the initial state of light and atoms is Gaussian and the given interaction preserves this property. Motivated by this observation, we examine in this context, how a given interaction can be used to simulate others and how it can be employed to create entanglement at optimal rates. The results are applied to construct protocols based on several passes of light through an atomic ensemble.

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This thesis contributes to the theory of a light-matter quantum interface based on the Kerr-effect arising in the dispersive interaction of pulsed laser light with a spin-polarized atomic ensemble. The scattering process can be described on the basis of a simple, yet fully quantum mechanical model involving only a small number of bosonic modes referring to transverse spin components and quadratures of forward scattered light. Based on this model we derive protocols for the creation of entangled states of light and atoms and the teleportation of quantum states of light onto atoms employing this entanglement. Furthermore we present a protocol, which allows one to exchange the state of light and atoms and thus provides a quantum memory for states of the light field. For both, the storage and the teleportation of coherent states we prove a benchmark on the average fidelity, which is achievable by purely classical protocols. Both protocols allow one to significantly surpass this threshold and to demonstrate thereby a gain in employing quantum strategies. Under common experimental conditions the initial state of light and atoms is Gaussian and the given interaction preserves this property. Motivated by this observation, we examine in this context, how a given interaction can be used to simulate others and how it can be employed to create entanglement at optimal rates. The results are applied to construct protocols based on several passes of light through an atomic ensemble.
Summary form only given. A new approach to the problem of the quantum interface between light and atoms has been recently developed. The method utilizes free space dispersive interaction between pulses of light and spin polarized atomic ensembles. Entanglement between the polarization state of light and the collective spin state of atoms is established by measurement, more precisely by detection of light in a certain polarization basis. In the first demonstration of this approach we have generated a long-lived entangled state of two separate macroscopic atomic samples by a polarization measurement on light transmitted through the samples. We then have shown that this approach also works for mapping of a quantum state of light onto long-lived atomic spin state paving the road towards realization of the quantum memory for light. Recently we have also extended the free space light-atoms interface beyond the continuous variables in the proposal, where a coherent superposition "cat" state of an atomic ensemble is generated by a measurement sequence. Progress with other communication protocols such as atomic state teleportation and multiparty networks will be presented.
We present two protocols, one for the storage of light in an atomic ensemble and the subsequent retrieval, and another one for the generation of entanglement between light and atoms. They rely on two passes of a single pulse through the ensemble, Larmor precessing in an external field. Both protocols work deterministically and the relevant figures of merit---such as the fidelity or the EPR variance---scale exponentially in the coupling strength. We solve the corresponding Maxwell-Bloch equations describing the scattering process and determine the resulting input-output relations which only involve one relevant light mode that, in turn, can be easily accessed experimentally.
We discuss theoretically quantum interface between light and a spin polarized ensemble of atoms with the spin $\ensuremath{\geqslant}1$ based on an off-resonant Raman scattering. We present the spectral theory of the light--atom interaction and show how particular spectral modes of quantum light couple to spatial modes of the extended atomic ensemble. We show how this interaction can be used for quantum memory storage and retrieval and for deterministic entanglement protocols. The proposed protocols are attractive due to their simplicity since they involve just a single pass of light through atoms without the need for elaborate pulse shaping or quantum feedback. As a practically relevant example we consider the interaction of a light pulse with hyperfine components of D1{D}_{1}D1​ line of 87Rb^{87}\mathrm{Rb}87Rb. The quality of the proposed protocols is verified via analytical and numerical analysis.
In this thesis I explore the use of collective spin angular momentum as a platform for quantum information processing. Such systems have several nice features that make them excellent choices for such protocols, especially ones where information is also stored in photonic variables. The longer coherence times of atoms makes it possible to store information from light in atoms for future use, and it is generally easier to couple atomic variables than to create nonlinear interactions of light. Above and beyond the advantages of atomic systems, collective atomic systems have additional strengths. In the limit of a large number of atoms, the collective variables of atomic systems have a natural connection to the bosonic algebra of light (known as the Holstein-Primakoff or HP approximation) where components of the collective spin angular momentum effectively act as quadratures, making them natural systems for coupling to light. Also, collectively addressing the atoms allows one to access a large state space without individual addressing of the atoms. A natural first step towards control of these collective variables is generating large amounts of atomic spin squeezing. In the HP approximation going from rotations to squeezing corresponds to going from linear to quadratic interactions in the atomic quadratures; for extremely large squeezing one should see the breakdown of the HP approximation and the ability to generate arbitrary collective atomic states. I have sought to improve previous schemes for the spin squeezing of atomic ensembles, such as the proposal of Takeuchi et. al. based on coherent quantum feedback. In this scheme a beam of linearly polarized light passes through the atomic ensemble (prepared in a coherent state), coupling to the atoms through a state-dependent index of refraction (the Faraday effect). The light is then passed through a wave-plate and reflected back through the atoms for a second pass. This double-pass scheme leads to an effective nonlinearity as the atomic fluctuations are mapped onto the light on the first pass and then back on to the atoms in the second pass. The light acts as a bus coupling each atom to each of the others. This nonlinear interaction forms a shearing of the atomic coherent state that results in squeezing. The light is entangled to the atoms through these interactions, and remains entangled as it escapes the system. This leads to decoherence of the atoms as the light is lost to the environment, reducing the amount of spin squeezing achieved. The first step towards improving the double-pass scheme was to add a quantum eraser step in which the light is disentangled from the squeezed atoms. By first measuring one quadrature of the light, and then performing a measurement-dependent rotation on the atomic ensemble, it is possible to decouple the atoms and light so that the loss of the light does not reduce the atomic squeezing. This results in an improvement of the rate of atomic spin squeezing. The nonlinear shearing interaction that remains still falls short of the exponential squeezing seen in optical parametric amplification. The reason for this can be seen by decomposing the shearing interaction into squeezing along a given quadrature followed by a rotation. The rotation leads to a constantly changing axis along which the squeezing occurs, and thus the squeezing builds up more slowly. This can be corrected for by breaking up the light pulse into a sequence of small pulses, and performing a small phase matching rotation after each pulse. The squeezing then adds up along a constant direction, rather than along a constantly varying direction. This results in still further improvement of the rate of atomic spin squeezing. A complete model includes the effects of photon-atom scattering and other noise and loss effects on the overall rate of squeezing. Previous derivations of noise due to photon-atom scattering have started with the unjustified assumptions that the atomic and photonic decoherence channels were both Gaussian and independent of correlations between the two subsystems. They then proceed with very general statistical arguments that rely upon these simplifications. My work begins with the more fundamental master equation picture in which I find the Linblad jump operators. I find that in general the photonic and atomic loss channels are not independent, with the intensity of the light dictating the details of this dependence, and find the conditions under which the Gaussian approximation holds. Squeezing and loss is initially treated assuming ensembles of spin-1/2 atoms, but this work is further extended to higher dimensional subsystems. For a higher spin case, preparing the atoms in spin coherent states is not optimal. One can engineer a stronger interaction by preparing the atoms in an atomic "cat state", i.e., a superposition of the two stretch states along the direction of propagation of the light beam. The fluctuations of such a state are more strongly coupled to the light, resulting in a stronger nonlinearity. This leads to strong correlations between the atoms, but they are not immediately useful for squeezing; the cat state must be coherently mapped to a coherent state to achieve atomic spin squeezing. The state created in this manner is ultimately more squeezed than that achieved with the same interaction but prepared initially in a coherent state.
We present a protocol for the teleportation of the quantum state of a pulse of light onto the collective spin state of an atomic ensemble. The entangled state of light and atoms employed as a resource in this protocol is created by probing the collective atomic spin, Larmor precessing in an external magnetic field, off resonantly with a coherent pulse of light. We take here full account of the effects of Larmor precession and show that it gives rise to a qualitatively different type of multimode entangled state of light and atoms. The protocol is shown to be robust against the dominating sources of noise and can be implemented with an atomic ensemble at room temperature interacting with free-space light. We also provide a scheme to perform the readout of the Larmor precessing spin state enabling the verification of successful teleportation as well as the creation of spin squeezing.
We propose a quantum interface which applies multiple passes of a pulse of light through an atomic sample with phase/polarization rotations in between the passes. Our proposal does not require nonclassical light input or measurements on the system, and it predicts rapidly growing entanglement of light and atoms from just coherent inputs. The proposed interface makes it possible to achieve a number of tasks within quantum-information processing, including teleportation between light and atoms, quantum memory for light, and squeezing of atomic and light variables.