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Quantum Simulation of Triangular, Honeycomb and Kagome Crystal Structures using Ultracold Atoms in Lattices of Laser Light

Claire Thomas

Published Jan 1, 2017• 1 citation
OpenAlex

Abstract

Ultracold atomic gases trapped at the interference of coherent beams of light constitute an artificial material. This optical lattice material may be used for controlled quantum simulations of condensed matter theories. The bulk of this dissertation concerns the construction and calibration of an optical superlattice that can form the triangular, honeycomb and kagome crystal structures. The properties and geometry of this artificial material may be dynamically changed, allowing for the experiments discussed in this thesis that would be impossible with real materials. The use of ultracold atoms in optical lattices for quantitative tests is challenging because of the novelty of many of the techniques in the field, and because of the myriad experimental differences between these artificial materials and true materials. This thesis reports the development of a method to characterize optical lattice potentials using matter-wave diffraction. We observe an enhancement of inversion asymmetry in matter-wave diffraction from a honeycomb lattice, which we explain using a time-independent perturbative treatment of the single-particle band structure of the lattice. Our experiment also provides new insight into a commonly used detection technique. This thesis culminates in the development and experimental realization of a quantitative test of a condensed-matter theory. The test is insensitive to the experimental differences between artificial materials and real materials. We focus on a prediction from a mean-field treatment of the Bose-Hubbard model that concerns the difference in behavior of itinerant particles on lattices that are identical but for their geometry. Using the tunable geometry of our quantum simulator, we measure the properties of ultracold atomic gases trapped in the triangular and kagome lattices under otherwise identical conditions and find that they are consistent with the mean-field scaling prediction.

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Ultracold atomic gases trapped at the interference of coherent beams of light constitute an artificial material. This optical lattice material may be used for controlled quantum simulations of condensed matter theories. The bulk of this dissertation concerns the construction and calibration of an optical superlattice that can form the triangular, honeycomb and kagome crystal structures. The properties and geometry of this artificial material may be dynamically changed, allowing for the experiments discussed in this thesis that would be impossible with real materials. The use of ultracold atoms in optical lattices for quantitative tests is challenging because of the novelty of many of the techniques in the field, and because of the myriad experimental differences between these artificial materials and true materials. This thesis reports the development of a method to characterize optical lattice potentials using matter-wave diffraction. We observe an enhancement of inversion asymmetry in matter-wave diffraction from a honeycomb lattice, which we explain using a time-independent perturbative treatment of the single-particle band structure of the lattice. Our experiment also provides new insight into a commonly used detection technique. This thesis culminates in the development and experimental realization of a quantitative test of a condensed-matter theory. The test is insensitive to the experimental differences between artificial materials and real materials. We focus on a prediction from a mean-field treatment of the Bose-Hubbard model that concerns the difference in behavior of itinerant particles on lattices that are identical but for their geometry. Using the tunable geometry of our quantum simulator, we measure the properties of ultracold atomic gases trapped in the triangular and kagome lattices under otherwise identical conditions and find that they are consistent with the mean-field scaling prediction.
Quantum simulation is the study of one quantum mechanical system via analog with another. In this thesis we explore a simple model of interacting bosons on a lattice, known as the Bose-Hubbard model, by experimental investigation of ultracold rubidium atoms in an optical lattice made from laser light. We describe the construction and stabilization of an optical superlattice with threefold symmetry, and its use in studying the Bose-Hubbard model on triangular and trimerized kagome lattices. We study the short range phase coherence of a Mott insulator on the triangular lattice, and develop a scheme to mitigate out-of-equilibrium effects arising from the state preparation. We show the first experimental realization of an optical trimerized kagome lattice for cold atoms, and discuss experiments characterizing this lattice. Finally, we provide evidence for a Mott insulating state with fractional average particle number per site with measurements of the nearest-neighbor phase coherence of strongly interacting atoms in the trimerized kagome lattice.
Ultracold atoms in optical lattices can be used to model condensed matter systems. They provide a clean, tuneable system which can be engineered to reach parameter regimes that are not accessible in condensed matter systems. Furthermore, they provide different techniques for probing the properties of these systems.This thesis presents an experimental and theoretical study of ultracold atoms in optical lattices for quantum simulation of two-dimensional systems.The first part of this thesis describes an experiment with a Bose-Einstein condensate of 87Rb loaded into a two-dimensional optical lattice. The beams that generate the optical lattice are controlled by acousto-optic deflection to provide a flexible optical lattice potential. The use of a dynamic ‘accordion’ lattice with ultracold atoms, where the spacing of the lattice is increased in both directions from 2.2 to 5.5 μm, is described. This technique allows an experiment such as quantum simulations to be performed with a lattice spacing smaller than the resolution limit of the imaging system, while allowing imaging of the atoms at individual lattice sites by subsequent expansion of the optical lattice. The optical lattice can also be rotated, generating an artificial magnetic field. Previous experiments with the rotating optical lattice are summarised, and steps to reaching the strongly correlated regime are discussed.The second part of this thesis details numerical techniques that can be used to describe strongly correlated two-dimensional systems. These systems are challenging to simulate numerically, as the exponential growth in the size of the Hilbert space with the number of particles means that they can only be solved exactly for very small systems. Recently proposed correlator product states [Phys. Rev. B 80, 245116 (2009)] provide a numerically efficient description which can be used to simulate large two-dimensional systems. In this thesis we apply this method to the two-dimensional quantum Ising model, and the Bose-Hubbard model subject to an artificial magnetic field in the regime where fractional quantum Hall states are predicted to occur.
Ultracold atoms in optical lattices can be used to model condensed matter systems. They provide a clean, tuneable system which can be engineered to reach parameter regimes that are not accessible in condensed matter systems. Furthermore, they provide different techniques for probing the properties of these systems.This thesis presents an experimental and theoretical study of ultracold atoms in optical lattices for quantum simulation of two-dimensional systems.The first part of this thesis describes an experiment with a Bose-Einstein condensate of 87Rb loaded into a two-dimensional optical lattice. The beams that generate the optical lattice are controlled by acousto-optic deflection to provide a flexible optical lattice potential. The use of a dynamic ‘accordion’ lattice with ultracold atoms, where the spacing of the lattice is increased in both directions from 2.2 to 5.5 μm, is described. This technique allows an experiment such as quantum simulations to be performed with a lattice spacing smaller than the resolution limit of the imaging system, while allowing imaging of the atoms at individual lattice sites by subsequent expansion of the optical lattice. The optical lattice can also be rotated, generating an artificial magnetic field. Previous experiments with the rotating optical lattice are summarised, and steps to reaching the strongly correlated regime are discussed.The second part of this thesis details numerical techniques that can be used to describe strongly correlated two-dimensional systems. These systems are challenging to simulate numerically, as the exponential growth in the size of the Hilbert space with the number of particles means that they can only be solved exactly for very small systems. Recently proposed correlator product states [Phys. Rev. B 80, 245116 (2009)] provide a numerically efficient description which can be used to simulate large two-dimensional systems. In this thesis we apply this method to the two-dimensional quantum Ising model, and the Bose-Hubbard model subject to an artificial magnetic field in the regime where fractional quantum Hall states are predicted to occur.
Quantum simulation using ultracold fermions in optical lattices provides valuable insights for strongly correlated many-body phenomena in regimes challenging for classical simulations. In this dissertation, we report the design and construction of an apparatus capable of producing quantum degenerate Bose and Fermi gases. The atoms are then loaded into hexagonal optical superlattices created using two commensurate wavelengths. The apparatus lays the foundation for studying interacting fermions in geometrically frustrated lattices.We also report our experimental results on the characterization of the quantum geometry of Bloch band structures. Using rubidium Bose-Einstein condensates in the honeycomb lattice, we were able to measure the quantum distance around band touching points using parallel transport. Additionally, by simulating optical excitations using noninteracting fermions in a periodically modulated lattice, we observe quasimomentum-dependent optical selection rules, which stem from interband quantum geometry of the honeycomb lattice.
Over recent years, exciting developments in the field of ultracold atoms confined in optical lattices have led to numerous theoretical proposals devoted to the quantum simulation of problems e.g. known from condensed matter physics. Many of those ideas demand experimental environments with non-cubic lattice geometries. In this paper, we report on the implementation of a versatile three-beam lattice allowing for the generation of triangular as well as hexagonal optical lattices. As an important step, the superfluid–Mott insulator (SF–MI) quantum phase transition has been observed and investigated in detail in this lattice geometry for the first time. In addition to this, we study the physics of spinor Bose–Einstein condensates (BEC) in the presence of the triangular optical lattice potential, especially spin changing dynamics across the SF–MI transition. Our results suggest that, below the SF–MI phase transition, a well-established mean-field model describes the observed data when renormalizing the spin-dependent interaction. Interestingly, this opens up new perspectives for a lattice-driven tuning of a spin dynamics resonance occurring through the interplay of the quadratic Zeeman effect and spin-dependent interaction. Finally, we discuss further lattice configurations that can be realized with our setup.
An optical lattice is the periodic potential that atoms experience via the ac-Stark shift when they are illuminated by counter-propagating laser beams that form a standing-wave pattern. Optical lattices have been widely used as a versatile platform in cooling, trapping, controlling atoms, and also for the study of a variety of problems in physics. The many-body states of ultracold atoms in optical lattices can be characterized by the quantum-correlations encoded in time-of-flight images. In this thesis, we mainly discuss the use of correlations function as a natural framework for characterizing quantum states in optical lattices.\nThe outline of the thesis is as follows. Chapter 1 gives a brief introduction to optical lattice potentials and ways for describing particles moving in a periodic potential. Chapter 2 explains the importance of correlations and discusses common methods to detect them in cold atom experiments.\nChapter 3 presents work done to study the many-body Schrödinger equation in a quasiperiodic potential and discusses its connection with the Kolmogorov-Arnold-Moser (KAM) problem of classical mechanics. We posed a possible visualization of such a connection in experimentally accessible many-body observables. These observables are useful probes for the three characteristic phases of the problem: the metallic, Anderson, and band-insulator phases. In addition, they exhibit fingerprints of nonlinear phenomena such as bifurcations and devil's staircases. Our numerical treatment is complemented with a perturbative analysis that provides insight on the underlying physics. The perturbative-theory approach is particularly useful in illuminating the distinction between the Anderson-insulator and the band-insulator phases in terms of paired sets of dimerized states.\nChapter 4 discusses several theoretical procedures developed to understand a recent experiment on macroscopic quantum self-trapping (ST) performed in a 2D optical lattice. Mean field and truncated-Wigner-approximation (TWA) calculations are performed trying to reproduce the experimental observations. The discrepancy between the theory and the experiment lead to the hypothesis of a new type of ST caused by strong correlations. We analyze toy models to support it.