Practical system for the generation of pulsed quantum frequency combs
Piotr Roztocki, Michael Kues, Christian Reimer, Benjamin Wetzel, Stefania Sciara, Yanbing Young Zhang, Alfonso Carmelo Cino, Brent E. Little, Sai T. Chu, David Moss, Roberto Morandotti
The on-chip generation of large and complex optical quantum states will enable low-cost and accessible advances for quantum technologies, such as secure communications and quantum computation. Integrated frequency combs are on-chip light sources with a broad spectrum of evenly-spaced frequency modes, commonly generated by four-wave mixing in optically-excited nonlinear micro-cavities, whose recent use for quantum state generation has provided a solution for scalable and multi-mode quantum light sources. Pulsed quantum frequency combs are of particular interest, since they allow the generation of single-frequency-mode photons, required for scaling state complexity towards, e.g., multi-photon states, and for quantum information applications. However, generation schemes for such pulsed combs have, to date, relied on micro-cavity excitation via lasers external to the sources, being neither versatile nor power-efficient, and impractical for scalable realizations of quantum technologies. Here, we introduce an actively-modulated, nested-cavity configuration that exploits the resonance pass-band characteristic of the micro-cavity to enable a mode-locked and energy-efficient excitation. We demonstrate that the scheme allows the generation of high-purity photons at large coincidence-to-accidental ratios (CAR). Furthermore, by increasing the repetition rate of the excitation field via harmonic mode-locking (i.e. driving the cavity modulation at harmonics of the fundamental repetition rate), we managed to increase the pair production rates (i.e. source efficiency), while maintaining a high CAR and photon purity. Our approach represents a significant step towards the realization of fully on-chip, stable, and versatile sources of pulsed quantum frequency combs, crucial for the development of accessible quantum technologies.
The on-chip generation of large and complex optical quantum states will enable low-cost and accessible advances for quantum technologies, such as secure communications and quantum computation. Integrated frequency combs are on-chip light sources with a broad spectrum of evenly-spaced frequency modes, commonly generated by four-wave mixing in optically-excited nonlinear micro-cavities, whose recent use for quantum state generation has provided a solution for scalable and multi-mode quantum light sources. Pulsed quantum frequency combs are of particular interest, since they allow the generation of single-frequency-mode photons, required for scaling state complexity towards, e.g., multi-photon states, and for quantum information applications. However, generation schemes for such pulsed combs have, to date, relied on micro-cavity excitation via lasers external to the sources, being neither versatile nor power-efficient, and impractical for scalable realizations of quantum technologies. Here, we introduce an actively-modulated, nested-cavity configuration that exploits the resonance pass-band characteristic of the micro-cavity to enable a mode-locked and energy-efficient excitation. We demonstrate that the scheme allows the generation of high-purity photons at large coincidence-to-accidental ratios (CAR). Furthermore, by increasing the repetition rate of the excitation field via harmonic mode-locking (i.e. driving the cavity modulation at harmonics of the fundamental repetition rate), we managed to increase the pair production rates (i.e. source efficiency), while maintaining a high CAR and photon purity. Our approach represents a significant step towards the realization of fully on-chip, stable, and versatile sources of pulsed quantum frequency combs, crucial for the development of accessible quantum technologies.
Summary form only given. Here, we demonstrate the first scheme to generate pulsed quantum frequency combs without the need for an external laser. We constructed a laser cavity (Fig. 1a) around a 4-port integrated micro-ring resonator, featuring narrow bandpass filters to select a single resonance, an optical gain component (erbium-doped fiber amplifier), and a mode-locking element (an intensity modulator). By setting the intensity modulation frequency to the fundamental repetition rate of the cavity (determined by the external cavity length), we achieved mode-locked pulsed operation (Fig. 1b), exciting a pulsed two-photon comb. Driving the intensity modulator at multiples of the fundamental repetition rate (upwards of 4x) also resulted in stable mode-locking (Fig. 1c), significant as this enables an increase of the photon pair generation rate without sacrificing its coincidence-to-accidental ratio (CAR). We characterized the photon statistics as a function of the average ring input power (see Fig. 1d), achieving a maximum CAR of 110 that decreases with increasing power and increasing coincidence rates. Autocorrelation measurements confirmed the purity of the generated state (pure single-frequency modes, even at multiples of the repetition rate), confirming that the resonance was excited over its entire bandwidth, and obtained a heralded anti-bunching dip of 0.245<;0.5 as expected of a source operating in the single-photon regime.
We present a method for the generation and coherent manipulation of pulsed quantum frequency combs. Until now, methods of preparing high-dimensional states on-chip in a practical way have remained elusive due to the increasing complexity of the quantum circuitry needed to prepare and process such states. Here, we outline how high-dimensional, frequency-bin entangled, two-photon states can be generated at a stable, high generation rate by using a nested-cavity, actively mode-locked excitation of a nonlinear micro-cavity. This technique is used to produce pulsed quantum frequency combs. Moreover, we present how the quantum states can be coherently manipulated using standard telecommunications components such as programmable filters and electro-optic modulators. In particular, we show in detail how to accomplish state characterization measurements such as density matrix reconstruction, coincidence detection, and single photon spectrum determination. The presented methods form an accessible, reconfigurable, and scalable foundation for complex high-dimensional state preparation and manipulation protocols in the frequency domain.
Complex optical quantum states based on entangled photons are essential for investigations of fundamental physics and are the heart of applications in quantum information science. Recently, integrated photonics has become a leading platform for the compact, cost-efficient, and stable generation and processing of optical quantum states. However, onchip sources are currently limited to basic two-dimensional (qubit) two-photon states, whereas scaling the state complexity requires access to states composed of several (<2) photons and/or exhibiting high photon dimensionality. Here we show that the use of integrated frequency combs (on-chip light sources with a broad spectrum of evenly-spaced frequency modes) based on high-Q nonlinear microring resonators can provide solutions for such scalable complex quantum state sources. In particular, by using spontaneous four-wave mixing within the resonators, we demonstrate the generation of bi- and multi-photon entangled qubit states over a broad comb of channels spanning the S, C, and L telecommunications bands, and control these states coherently to perform quantum interference measurements and state tomography. Furthermore, we demonstrate the on-chip generation of entangled high-dimensional (quDit) states, where the photons are created in a coherent superposition of multiple pure frequency modes. Specifically, we confirm the realization of a quantum system with at least one hundred dimensions. Moreover, using off-the-shelf telecommunications components, we introduce a platform for the coherent manipulation and control of frequencyentangled quDit states. Our results suggest that microcavity-based entangled photon state generation and the coherent control of states using accessible telecommunications infrastructure introduce a powerful and scalable platform for quantum information science.
The on-chip generation of optical quantum states will enable accessible advances for quantum technologies. We demonstrate that integrated quantum frequency combs (based on high-Q microring resonators made from a CMOS-compatible, high refractive-index doped-glass platform) can enable the generation of pure heralded single photons, cross-polarized photon pairs, as well as bi- and multi-photon entangled qubit states over a broad frequency comb covering the S, C, L telecommunications band, with photon frequencies corresponding to standard telecommunication channels spaced by 200 GHz. Exploiting a self-locked, intra-cavity excitation configuration, a highly-stable source of multiplexed heralded single photons is demonstrated, operating continuously for several weeks with less than 5% fluctuations. The photon bandwidth of 110 MHz is compatible with quantum memories, and high photon purity was confirmed through single-photon auto-correlation measurements. In turn, by simultaneously exciting two orthogonal polarization mode resonances, we demonstrate the first realization of type-II spontaneous FWM (in analogy to type-II spontaneous parametric down-conversion), allowing the direct generation of orthogonally-polarized photon pairs on a chip. By using a double-pulse excitation, we demonstrate the generation of time-bin entangled photon pairs. We measure qubit entanglement with visibilities above 90%, enabling the implementation of quantum information processing protocols. Finally, the excitation field and the generated photons are intrinsically bandwidth-matched due to the resonant characteristics of the ring cavity, enabling the multiplication of Bell states and the generation of a four-photon time-bin entangled state. We confirm the generation of this four-photon entangled state through four-photon quantum interference.
The investigation of integrated frequency comb sources characterized by equidistant spectral modes was initially driven by considerations toward classical applications, seeking a more practical and miniaturized way to generate stable broadband sources of light. Recently, in the context of scaling the complexity of optical quantum circuits, these on-chip approaches have provided a new framework to address the challenges associated with non-classical state generation and manipulation. For example, multi-photon and high-dimensional states were to date either inaccessible, lacked scalability, or were difficult to manipulate, requiring elaborate approaches. The emerging field of quantum frequency combs studying spectral multimode sources based on the judicious excitation of (typically) third-order nonlinear optical micro-cavities has begun to address these issues. Several quantum sources based on this concept have already been demonstrated, among them are combs of correlated photons, cross-polarized photon pairs, entangled photon pairs, multi-photon states, and high-dimensional entangled states. While sources have achieved increasing complexity, so have coherent state processing operations, demonstrated in a practical manner using standard telecommunications components. Here, we review our recent work in the development of this framework, with a focus on multi-photon and high-dimensional states. The integrated frequency comb platform thus demonstrates significant potential for the development of meaningful quantum optical technologies.
Today’s quantum technology relies on the realization of large-scale non-classical systems in practical formats to enable quantum-accelerated computing, secure communications and enhanced sensing. Optical on-chip quantum frequency combs, characterized by many equidistantly spaced frequency modes, allow the storage of large amounts of quantum information. The combination with control techniques, using accessible state-of-the-art telecommunications infrastructure, can constitute a powerful frequency-domain quantum circuit with new functionalities and represents an approach towards realizing practical large-scale controllable quantum systems. In this presentation, we will review approaches for the efficient realization of quantum frequency combs in on-chip waveguide structures and micro-resonators. We will show their applicability for the realization of quantum systems with considerably enhanced complexity, particularly generating and manipulating on-chip multi-photon and high-dimensional quantum states as well as discrete high-dimensional cluster states, laying at the basis of measurement based-quantum computing. Building on this, the realization of frequency-domain Hong-Ou-Mandel interference of independent photons, fundamental to quantum information processing, as well as an outlook on frequency-domain circuits will be discussed.