The crystal-like structures of laser-cooled ions predicted by molecular dynamics calculations and recently observed In a miniature quadrupole storage ring have far-reaching implications.
We observed phase transitions and ordered structures of laser-cooled Mg+ ions stored in a radio-frequency quadrupole storage ring with a diameter of 115 mm. The ions are confined two dimensionally by a quadrupole field and can move freely along the ring circumference. By cooling the ions with tangentially intersecting laser beams, we observed a linear string of ions aligned along the center line of the quadrupole field. For higher ion densities the linear structure changes into a helical structure. The dynamics of the stored ions was studied.
The crystallization of ion beams has recently been established in the rf quadrupole storage ring PALLAS (PAul Laser CooLing Acceleration System) for laser-cooled 24 Mg + ion beams at an energy of about 1 eV. Yet, unexpectedly sharp constraints had to be met concerning the confinement strength and the longitudinal laser cooling rate. In this paper, related and up to now unseen heating mechanisms are pinpointed for crystalline beams. The weak but inevitable diffusive transverse heating associated with the laser cooling process itself is investigated, possibly allowing the future measurement of the latent heat of the ion crystal. As a function of the beam velocity, the influence of bending shear on the attainability of larger crystalline structures is presented. Finally, rf heating of crystalline beams of different structure is studied for discontinuous cooling.