A highly integrated device capable of interfacing light and matter on a chip is presented. 1e7 caesium-133 atoms are captured from a hot vapour into a magneto-optical trap held close to a chip-mounted single-mode fibre. Sub-Doppler optical molasses cools the atoms and transfers them into a tightly focused 18W vertical optical dipole trap which intersects a 30um void that has been laser etched through the single-mode fibre. Thus, the optically trapped atoms are tightly confined in the path of fibre-guided photons for maximum overlap. Such a system is capable of writing, reading and storing quantum information and clearly has massive implications for quantum information technologies. The device presented is adaptable, scalable and highly integrated making it the ideal building block for quantum computing. Developments and modifications made to a system for producing ultracold samples of lithium-6, caesium-133 and mixtures thereof is also presented. Feshbach molecules have major applications in quantum computing, particularly in the modelling of complex many-body quantum systems. The large dipolar moment of the lithium-caesium Feshbach molecule is the largest of all the alkali dimers producing rich long-range anisotropic dipole-dipole interactions. By use of the broad Feshbach resonance situated at 834G we associate fermionic lithium-6 atoms into bosonic lithium-6-2 Feshbach molecules. Subsequent evaporative cooling drives a phase transition in the diffuse lithium gas to produce a molecular Bose-Einstein Condensate containing up to 1e4 atoms, the first to be produced in the UK. This thesis documents the construction of the quantum integrated light and matter interface (QuILMI) in its entirety from inception to realisation. An enormous amount of work has gone into the design and subsequent development of various vacuum, laser and magnetic systems that work seamlessly in tandem via a programmable control system. The system is now in a position to demonstrate to the world that atom-photon coupling on a chip is the way forward. For the lithium-caesium mixture experiment, a versatile dual-species oven has been meticulously designed, constructed and thoroughly characterised to replace one that significantly malfunctioned and harmed the experiment. The oven is capable of tuning the axial fluxes of lithium and caesium through several orders of magnitude via PID temperature controlled reservoirs. An array of fifteen 0.51mm diameter microtubes highly collimate the dual-species atomic beam such that little flux is wasted prolonging the life of both the source and the vacuum ion pumps. This source will return the system to its former glory such that the ultimate goal of realising ultracold lihtium-caesium Feshbach molecules can once again be pursued.
A highly integrated device capable of interfacing light and matter on a chip is presented. 1e7 caesium-133 atoms are captured from a hot vapour into a magneto-optical trap held close to a chip-mounted single-mode fibre. Sub-Doppler optical molasses cools the atoms and transfers them into a tightly focused 18W vertical optical dipole trap which intersects a 30um void that has been laser etched through the single-mode fibre. Thus, the optically trapped atoms are tightly confined in the path of fibre-guided photons for maximum overlap. Such a system is capable of writing, reading and storing quantum information and clearly has massive implications for quantum information technologies. The device presented is adaptable, scalable and highly integrated making it the ideal building block for quantum computing. Developments and modifications made to a system for producing ultracold samples of lithium-6, caesium-133 and mixtures thereof is also presented. Feshbach molecules have major applications in quantum computing, particularly in the modelling of complex many-body quantum systems. The large dipolar moment of the lithium-caesium Feshbach molecule is the largest of all the alkali dimers producing rich long-range anisotropic dipole-dipole interactions. By use of the broad Feshbach resonance situated at 834G we associate fermionic lithium-6 atoms into bosonic lithium-6-2 Feshbach molecules. Subsequent evaporative cooling drives a phase transition in the diffuse lithium gas to produce a molecular Bose-Einstein Condensate containing up to 1e4 atoms, the first to be produced in the UK. This thesis documents the construction of the quantum integrated light and matter interface (QuILMI) in its entirety from inception to realisation. An enormous amount of work has gone into the design and subsequent development of various vacuum, laser and magnetic systems that work seamlessly in tandem via a programmable control system. The system is now in a position to demonstrate to the world that atom-photon coupling on a chip is the way forward. For the lithium-caesium mixture experiment, a versatile dual-species oven has been meticulously designed, constructed and thoroughly characterised to replace one that significantly malfunctioned and harmed the experiment. The oven is capable of tuning the axial fluxes of lithium and caesium through several orders of magnitude via PID temperature controlled reservoirs. An array of fifteen 0.51mm diameter microtubes highly collimate the dual-species atomic beam such that little flux is wasted prolonging the life of both the source and the vacuum ion pumps. This source will return the system to its former glory such that the ultimate goal of realising ultracold lihtium-caesium Feshbach molecules can once again be pursued.
Ultracold mixture experiments hold the promise of providing new insights into many-body quantum systems as well as ultracold chemistry and few-body phenomena. The work presented in this thesis dealt with the construction of a new apparatus for the production and study of ultracold gases of fermionic lithium-6 and bosonic caesium-133. These isotopes offer a wide tunability in their interaction strength, both in inter-species and intra-species collisions, through magnetic Feshbach resonances. Additionally, the widely different resonance frequencies of lithium and caesium enables independent control of each of the species. With this apparatus, Bose-Einstein condensates (BEC) containing 10^4 lithium Feshbach molecules are routinely produced. The cooling system for caesium has been developed in parallel and important steps towards producing ultracold caesium gases have been made. An optical dipole trap has been loaded with 2x10^6 caesium atoms and evaporative cooling towards quantum degeneracy can now be pursued. Laser, vacuum, magnetic and control systems have been developed for the implementation of this experiment. Light produced with this laser system was used to laser cool atoms, create conservative dipole traps as well as to provide means of imaging atomic clouds. Additionally, a system to produce strong magnetic fields of up to 1400 G has been established in order to exploit the wide tunability in the atomic interactions. Software that was developed for the computerised control system facilitated the coordination of all the components involved in the experimental sequence. Measurements and calculations that showcase the functionality of relevant parts of the setup are presented in this thesis. In this experiment, lithium and caesium atoms are obtained from a novel type of Zeeman slower and are loaded into a magneto-optical trap (MOT). The system is capable of doing this independently for each of the atomic species as well as sequentially. After the MOT has been loaded with atoms, they are transferred into a conservative far-off-resonance optical dipole trap. By adjusting the interactions between atoms and lowering the depth of the dipole trap, efficient evaporative cooling of lithium was carried out from which a molecular BEC was obtained. Time-of-flight measurements were used to characterise the condensate and study its expansion dynamics.
Atom chips are an excellent tool for studying ultracold degenerate quantum gases, due to the high degree of controllability afforded by the precise potentials generated from the current-carrying microfabricated wires on the chip surface. The geometries of the trapping potentials are inherently capable of realising extreme aspect ratios, and therefore creating model systems with effectively reduced dimensionality, particularly the theoretically-tractable one-dimensional Bose gas. In addition, the temporal tunability makes it possible to impart non-adiabatic changes on the trapping potentials, allowing experimental investigation of samples which have been brought out of equilibrium - a situation which is not fully theoretically understood. This thesis describes the implementation, development and characterisation of an experimental system for producing the first Bose-Einstein condensates of atomic rubidium 87 gas trapped on the surface of an atom chip in Nottingham. Such an apparatus is very complex and requires careful characterisation in order to run in a stable and reliable way. Details of the experimental setup are thoroughly outlined, including the vacuum system, lasers, electronics, computer control and timing, and the optical imaging system. A newly installed compact two-dimensional magneto-optical trap provides an loading rate of 5e7 atoms per second for loading a three-dimensional mirror-magneto-optical trap with 1.5e8 atoms, at a temperature of 300uK within 10s. The cloud is then sub-Doppler cooled to 50uK, and spin-polarised with 96% purity into the |F=2,mF=+2> ground state within 5ms, in preparation for loading a purely magnetic trap. A millimeter sized copper Z-shaped conductor located beneath the atom chip surface creates a Ioffe-Pritchard magnetic trap, into which the laser cooled cloud is loaded with 70% efficiency, and can be held with a vacuum-limited lifetime of 40s. Evaporative cooling then pre-cools the sample to below 20uK within 10s, to allow the subsequent loading into potentials created by the atom chip with 100% efficiency. A final evaporation stage then cools the cloud below the phase transition temperature of 800nK, resulting finally in pure BECs with 105 atoms confined using the atom chip. Key measurements of various properties of the trapped condensates are presented, which are important in order to characterise the system fully, and to compare with theoretical expectations. In particular, included are the variation of condensate fraction with temperature, the BEC expansion dynamics, and the condensate lifetime in the trap, for example. Finally, it is demonstrated how BECs can be produced on the atom chip without the use of external macroscopic coils, achieved by using novel, integrated sheet structures located beneath the chip surface - unique to this experimental system - to create the necessary bias fields.
This thesis describes the production of molecular Bose-Einstein condensates (BEC) of 6Li2 dimers and binding energy measurements of p-wave Feshbach molecules. A σ− Zeeman slower is used to produce a continuous beam of isotopically enriched 6Li atoms at speeds low enough to load a magneto-optical trap (MOT). We currently have a flux of slowed atoms of ~ 5 · 106 atoms/s loading the MOT with more than 108 atoms. We then transfer up to 106 atoms in an almost equal spin mixture of the two lowest hyperfine states into an optical dipole trap. We achieved condensates in three different crossed optical dipole trap geometries. The initial low power optical dipole trap was formed using light from a 25WVersaDisk Yb:YAG laser at 1030 nm. It consisted of a 15 W beam crossed with a 13 W beam at about 80 degrees with a waist of approximately 30 μm in each beam. By translating the focus of the second beam we could change the trap geometry from near symmetric to elongated. Nowadays, we produce condensates in a crossed dipole trap formed by a 100 W fibre laser. Both arms are focussed to a waist of 40 μm, cross each other at 14 degrees and have laser powers of ~80 W and ~70 W, respectively. Evaporative cooling is achieved by reducing the laser power near the broad s-wave Feshbach resonance at 834 G. By tuning to the low magnetic field side (770 G) of the Feshbach resonance molecules are formed through three-body recombination at sufficiently low temperatures. Further evaporation leads to the creation of a molecular BEC. After reducing the laser power by a factor of about 1000 in approximately 3 s we have observed more than 30 000 condensed molecules. During the evaporation the temperature decreases from about 100 μK to below 100 nK. We present measurements of the binding energies of 6Li p-wave Feshbach molecules formed in combinations of the |F = 1/2,mF = +1/2i (|1i) and |F = 1/2,mF = −1/2i (|2i) states. The binding energies scale linearly with magnetic field detuning for all three resonances. The relative molecular magnetic moments are found to be 113 ± 7 μK/G, 111 ± 6 μK/G and 118 ± 8 μK/G for the |1i − |1i, |1i − |2i and |2i − |2i resonances, respectively, in good agreement with theoretical predictions.
The field of ultracold matter has developed rapidly over the course of the past twenty to thirty years. One outstanding achievement has been the realisation of Bose-Einstein condensation (BEC) only 23 years ago. Many other fascinating observations of quantum phenomena have been made at an incredibly fast pace using ultracold atomic samples with contact force interactions as a testbed. Due to the rapid successes of all these experiments on atomic ensembles, researchers began to aim for more elaborate inter-particle interactions. A possible additional one is the dipole-dipole interaction (DDI), the long-range character of which stands out in comparison to the contact interactions. Moreover, DDI is anisotropic and the possibility to tune the direction of the dipoles in the experiment as well as the interaction strength promises the possibility to study a plethora of new quantum phenomena. In recent years, several experiments using different combinations of alkali atoms to create ground-state hetero-nuclear molecules in the ultracold regime have been set up, following the pioneering work on KRb molecules. Of all possible combinations of two alkali atoms, NaK combines the advantages of a high induced electric dipole moment of 2.72 Debye, chemical stability of the ground-state molecules, the possibility to realise bosonic as well as fermionic molecules and a large knowledge base for cooling and trapping of the two atomic species. This thesis reports on the development and construction of an experiment apparatus for the production of ultracold bosonic dipolar ground state 23Na39K molecules. This includes the setup of an ultra-high vacuum (UHV) system, several laser light sources, microwave (MW) and radio frequency (RF) antennas and electronics to control the various components of the experiment. The system pre-cools the atomic samples of 23Na and 39K and loads them into a dual-species three-dimensional magneto-optical trap (3D MOT). After a transfer to a magnetic quadrupole trap, the mixture is cooled by forced MW evaporation until three-body losses limit dual-species operation at high densities and zero magnetic field. Using the pure optical trapping potential of a crossed optical dipole trap (cODT) and RF- state-transfer, the scattering properties of the bosonic mixture of 23Na+39K are investigated in extensive atom loss measurements for a magnetic field range from 0 to 750 G. Several Feshbach resonances, zero crossings of the interspecies scattering length and inelastic loss features in many different scattering channels are identified. The results of this study are used to refine the molecular potentials of NaK and to produce a dual-species quantum-degenerate mixture of two BECs in the state (f = 1, mf = −1) of 23Na + (f = 1, mf = −1) of 39K. The measurements and refined molecular potentials will considerably aid in the future realisation of 23Na39K molecules in their absolute ground state.
Hybrid quantum devices, incorporating both atoms and photons, are able to exploit the benefits of both systems. Compact, robust atom-photon interfaces will enable scalable architectures for quantum computing and quantum communication, as well as chip-scale sensors and single-photon sources. We demonstrate a new type of interface and show the interaction of cold cesium atoms with resonant photons. For this atoms are cooled in a magneto-optical trap, transferred to an optical dipole trap and positioned inside a transverse, 30 µm diameter through-hole in an optical fibre, created via laser micromachining. The intersection is orthogonal to the propagation direction of the light mode. We trap about 300 atoms at a temperature of 120µK. When the guided light is on resonance with the caesium D2 line, up to 87% of it is absorbed by the atoms. Our technique can be applied in 2-dimensional systems, i.e. in optical waveguide chips and other existing photonic systems. We also discuss the influence of hole shapes on transmission and prospects of adding a micro-cavity.
This thesis reports on the tunability of interactions in ultracold Bose-Fermi mixtures of Cesium and Lithium. The \nfirst realization of an optically trapped \n6Li -133Cs mixture enabled to perform trap loss spectroscopy measurements to identify \nmagnetic Feshbach resonances. A total of 19 interspecies Feshbach resonances, all in the magnetic field range between 650 G and 950 G, were observed for the two energetically lowest spin states of each species. Two 5 G broad and especially two 60 G broad s-wave resonances give perspectives to produce a dipolar quantum gas of LiCs ground state molecules as well as to study the Efimov effect in highly mass imbalanced systems. In addition, a unique relative tunability of intra- and interspecies \nscattering lengths was found which makes the 6Li -133Cs system also well suited for the investigation of polarons. Evaporative cooling was performed on optically trapped samples which contained only one of the species. In this way, Bose-Einstein condensates of 6Li molecules as well as 133Cs samples at a phase-space density of p = 4 · 10^2 were prepared. All experiments were performed in a new apparatus, which has been designed and set up during this thesis.