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Generating non-classical light using Rydberg interactions

Valentina Parigi, Erwan Bimbard, Jovica Stanojevic, Alexei Ourjoumtsev, Philippe Grangier

Published Jul 19, 2012• 0 citations
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Rydberg ensembles have many diverse and important applications for quantum information and quantum optics. For example, Rydberg ensembles can generate non-classical states of light which would be useful in a quantum network, and they could be used as qubits in a future quantum computer. For this reason, this thesis will present investigations of light-matter interactions in Rydberg ensembles. Non-classical states of light, such as single-photon states, are important for many quantum communication protocols. We have performed an experiment that demonstrates the generation of single-photon states from a Rydberg ensemble. We then studied the second-order correlations between this single-photon state of light and an incident coherent field. Under these conditions, we observed Hanbury Brown Twiss interference between the emission from a driven super-atom and a coherent field in the absence of stimulated emission. For a universal quantum computing architecture, coherence times must be much longer than gate operations. We observe ground-Rydberg coherence times in excess of 20 microseconds by using a "magic-wavelength" optical lattice to confine the atoms. Using this coherence time, we measured the differential nuclear-spin-dependent light shifts for principal quantum numbers, n, between n = 30 and n = 65, which is relevant for future high-fidelity Rydberg qubits in optical potentials. Also, we measured the hyperfine constant for atomic Rb to be 35.71 GHz with an uncertainty of 0.18 GHz.

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Using electromagnetically induced transparency and photon storage, the strong dipolar interactions between Rydberg atoms and the resulting dipole blockade can be mapped onto light fields to realise optical non-linearities and interactions at the single photon level. We report on the realisation of an experimental apparatus designed to study interactions between single photons stored as Rydberg excitations in optically trapped microscopic ensembles of ultracold 87Rb atoms. A pair of in-vacuum high numerical aperture lenses focus excitation and trapping beams down to 1 μm, well below the Rydberg blockade. Thanks to efficient magneto-optical trap (MOT) loading from an atomic beam generated by a 2D MOT and the ability to recycle the microscopic ensembles more than 20000 times without significant atom loss, we achieve effective repetition rates exceeding 110 kHz to obtain good photon counting statistics on reasonable time scales. To demonstrate the functionality of the setup, we present evidence of strong photon interactions including saturation of photon storage and the retrieval of non-classical light. Using in-vacuum antennae operating at up to 40 GHz, we perform microwave spectroscopy on photons stored as Rydberg excitations and observe an interaction induced change in lineshape depending on the number of stored photons.

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Bulletin of the American Physical Society•Jun 5, 2012•0 citations
Realization of distributed quantum systems requires fast generation and long-term storage of quantum states. Ground atomic states enable memories with storage times in the range of a minute, however their relatively weak interactions do not allow fast creation of non-classical collective states. Rydberg atomic systems feature fast preparation of singly excited collective states and their efficient mapping into light, but storage times in these approaches have not yet exceeded a few microseconds. Here we demonstrate a system that combines fast quantum state generation and long-term storage. An initially prepared coherent state of an atomic memory is transformed into a non-classical collective atomic state by Rydberg-level interactions in less than a microsecond. By sheltering the quantum state in the ground atomic levels, the storage time is increased by almost two orders of magnitude. This advance opens a door to a number of quantum protocols for scalable generation and distribution of entanglement.
Rydberg ensembles have many diverse and important applications for quantum information and quantum optics. For example, Rydberg ensembles can generate non-classical states of light which would be useful in a quantum network, and they could be used as qubits in a future quantum computer. For this reason, this thesis will present investigations of light-matter interactions in Rydberg ensembles. Non-classical states of light, such as single-photon states, are important for many quantum communication protocols. We have performed an experiment that demonstrates the generation of single-photon states from a Rydberg ensemble. We then studied the second-order correlations between this single-photon state of light and an incident coherent field. Under these conditions, we observed Hanbury Brown Twiss interference between the emission from a driven super-atom and a coherent field in the absence of stimulated emission. For a universal quantum computing architecture, coherence times must be much longer than gate operations. We observe ground-Rydberg coherence times in excess of 20 microseconds by using a "magic-wavelength" optical lattice to confine the atoms. Using this coherence time, we measured the differential nuclear-spin-dependent light shifts for principal quantum numbers, n, between n = 30 and n = 65, which is relevant for future high-fidelity Rydberg qubits in optical potentials. Also, we measured the hyperfine constant for atomic Rb to be 35.71 GHz with an uncertainty of 0.18 GHz.
Using electromagnetically induced transparency and photon storage, the strong dipolar interactions between Rydberg atoms and the resulting dipole blockade can be mapped onto light fields to realise optical non-linearities and interactions at the single photon level. We report on the realisation of an experimental apparatus designed to study interactions between single photons stored as Rydberg excitations in optically trapped microscopic ensembles of ultracold 87Rb atoms. A pair of in-vacuum high numerical aperture lenses focus excitation and trapping beams down to 1 μm, well below the Rydberg blockade. Thanks to efficient magneto-optical trap (MOT) loading from an atomic beam generated by a 2D MOT and the ability to recycle the microscopic ensembles more than 20000 times without significant atom loss, we achieve effective repetition rates exceeding 110 kHz to obtain good photon counting statistics on reasonable time scales. To demonstrate the functionality of the setup, we present evidence of strong photon interactions including saturation of photon storage and the retrieval of non-classical light. Using in-vacuum antennae operating at up to 40 GHz, we perform microwave spectroscopy on photons stored as Rydberg excitations and observe an interaction induced change in lineshape depending on the number of stored photons.