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Dynamics of atoms in a pulsed evanescent wave

Pasi Ryytty, M. Kaivola, C.G. Aminoff

Published Jan 1, 1996• 0 citations
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Reflection of atoms from a pulsed evanescent wave

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Atomic motion in a pulsed evanescent wave, with a pulse duration on the order of the lifetime of the excited state, is calculated using the semiclassical Bloch-equation approach. The equations for the internal atomic motion are solved using two approximations based on high laser intensity and on slow atomic velocity. The center-of-mass motion in the field under the effect of the dipole force is subsequently determined by numerical integration. As an example, the calculations show that the maximum normally incident velocity allowing a sodium atom to be reflected is approximately 35 m/s when using a 10 MW/cm 2 laser pulse of 7 ns duration. Our results also demonstrate that the velocity distribution of the reflected atoms may considerably differ from the distribution of the incident atoms due to different deceleration and acceleration times in a short laser pulse. This effect may lead to an average slowing-down of the reflected part of a thermal particle beam.

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Time-Resolved Measurements of the Adsorption/Desorption of Rb Atoms on Octadecyltrichlorosilane Coated Surfaces

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We carry out the first time-resolved measurement of Rb atoms desorbing from octadecyltrichlorosilane coated surfaces by polarizing the atoms near the surface using an evanescent wave pump pulse and watching the subsequent intensity change of another evanescent wave probe beam, and find the mean adsorption (dwell) time to be about 400 ns at a cell body temperature of 112°C. The adsorption energy is found to be 0.19 eV from the surface temperature dependence of the adsorption time. This method can be extended to study the adsorption/desorption process of other alkali atoms on other surfaces of transparent substrates with an ultimate time resolution limited by the flight time of atoms in the evanescent wave which is of the order of nanoseconds.

Chinese Physics Letters•Jul 1, 2015•7 citations
Abstract\nnumbers: 03.75.-b Matter Waves 03.75.Be Atom and Neutron Optics 37.10.Gh Atom Traps and Guides 42.25.-p Wave Optics ABSTRACT Semi-evanescent and evanescent matter-waves produced by an atom wave packet impinging a repulsive barrier can be back-refracted and reconstructed by the application of negative-index " comoving " potential pulses. One shows that those collapses and revivals generate a matter wave confined on both sides of the barrier border (" surface matter wave ") and should be observable via the retardation of atom reflection from the barrier interface. This property, joined to the possibility recently demonstrated of inducing negative refraction of atom waves, makes such potentials a matter-wave counterpart of negative-index materials or " meta materials " well-known in light optics.
Atomic motion in a pulsed evanescent wave, with a pulse duration on the order of the lifetime of the excited state, is calculated using the semiclassical Bloch-equation approach. The equations for the internal atomic motion are solved using two approximations based on high laser intensity and on slow atomic velocity. The center-of-mass motion in the field under the effect of the dipole force is subsequently determined by numerical integration. As an example, the calculations show that the maximum normally incident velocity allowing a sodium atom to be reflected is approximately 35 m/s when using a 10 MW/cm 2 laser pulse of 7 ns duration. Our results also demonstrate that the velocity distribution of the reflected atoms may considerably differ from the distribution of the incident atoms due to different deceleration and acceleration times in a short laser pulse. This effect may lead to an average slowing-down of the reflected part of a thermal particle beam.
We carry out the first time-resolved measurement of Rb atoms desorbing from octadecyltrichlorosilane coated surfaces by polarizing the atoms near the surface using an evanescent wave pump pulse and watching the subsequent intensity change of another evanescent wave probe beam, and find the mean adsorption (dwell) time to be about 400 ns at a cell body temperature of 112°C. The adsorption energy is found to be 0.19 eV from the surface temperature dependence of the adsorption time. This method can be extended to study the adsorption/desorption process of other alkali atoms on other surfaces of transparent substrates with an ultimate time resolution limited by the flight time of atoms in the evanescent wave which is of the order of nanoseconds.