Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Bulletin of the American Physical Society

Spectral hole burning and its application in microwave photonics

Stefan Putz, Andreas Angerer, Dmitry O. Krimer, Ralph Glattauer, William J. Munro, Stefan Rotter, Jörg Schmiedmayer, Johannes Majer

Published Mar 14, 2017• 1 citation
OpenAlex

Abstract

Rabi oscillations with a decay time of 26.7 μs are observed in a system comprising the electron spins in a diamond nitrogen–vacancy centre and a superconducting microwave cavity. Such oscillations are achieved by engineering the spectral hole burning of the spin ensemble. Spectral hole burning, used in inhomogeneously broadened emitters, is a well-established optical1 technique, with applications from spectroscopy to slow light2 and frequency combs3. In microwave photonics4, electron spin ensembles5,6 are candidates for use as quantum memories7 with potentially long storage times8. Here, we demonstrate long-lived collective dark states9 by spectral hole burning in the microwave regime10. The coherence time in our hybrid quantum system (nitrogen–vacancy centres strongly coupled to a superconducting microwave cavity) becomes longer than both the ensemble's free-induction decay and the bare cavity dissipation rate. The hybrid quantum system thus performs better than its individual subcomponents. This opens the way for long-lived quantum multimode memories, solid-state microwave frequency combs, spin squeezed states11, optical-to-microwave quantum transducers12 and novel metamaterials13. Beyond these, new cavity quantum electrodynamics experiments will be possible where spin–spin interactions and many-body phenomena14 are directly accessible.

Related papers

Hybrid quantum systems in the microwave regime (Conference Presentation)

William J. Munro, Andreas Angerer, Thomas Astner +4 more

The efficient generation, coherent control, manipulation and measurement of quantum states of light and matter is at the core of quantum technologies. Hybrid quantum systems, where one combines the best parts of multiple individual quantum systems together without their weaknesses, are now seen as a way to engineer composite quantum systems with the properties one requires. This would in principle allow one to probe new physical regimes. However, the issue until recently has been that hybridization has not resulted in systems with superior properties. Recently however we [Nature Photonics 11, 3639 (2016)] have shown an increased coherence times in hybrid system is of composed nitrogen-vacancy centers strongly coupled to a superconducting microwave resonator. This demonstration has enabled this kind of hybrid system to enter the regime where quantum nonlinearities are present. We discuss several types of nonlinearity effects that can be naturally explored (bistability and superradiance). Our work paves the way for the creation of spin squeezed states, novel metamaterials, long-lived quantum multimode memories and solid-state microwave frequency combs. Further in the longer term it may enable the exploration of many-body phenomena in new cavity quantum electrodynamics experiments.

Quantum Photonic Devices•Sep 18, 2018•0 citations

Sustained photon pulse revivals from inhomogeneously broadened spin ensembles

Dmitry O. Krimer, Matthias Zens, Stefan Putz +1 more

Abstract A very promising recent trend in applied quantum physics is to combine the advantageous features of different quantum systems into what is called “hybrid quantum technology”. One of the key elements in this new field will have to be a quantum memory enabling to store quanta over extended periods of time. Systems that may fulfill the demands of such applications are comb‐shaped spin ensembles coupled to a cavity. Due to the decoherence induced by the inhomogeneous ensemble broadening, the storage time of these quantum memories is, however, still rather limited. Here we demonstrate how to overcome this problem by burning well‐placed holes into the spectral spin density leading to spectacular performance in the multimode regime. Specifically, we show how an initial excitation of the ensemble leads to the emission of more than a hundred well‐separated photon pulses with a decay rate significantly below the fundamental limit of the recently proposed “cavity protection effect”. image

arXiv:1701.01852•Laser & Photonics Review•Oct 14, 2016•17 citations

Observation of dark states in a superconductor diamond quantum hybrid system

Xiaobo Zhu, Yuichiro Matsuzaki, Robert Amsüss +7 more

The hybridization of distinct quantum systems has opened new avenues to exploit the best properties of these individual systems. Superconducting circuits and electron spin ensembles are one such example. Strong coupling and the coherent transfer and storage of quantum information has been achieved with nitrogen vacancy centres in diamond. Recently, we have observed a remarkably sharp resonance (~1 MHz) at 2.878 GHz in the spectrum of flux qubit negatively charged nitrogen vacancy diamond hybrid quantum system under zero external magnetic field. This width is much narrower than that of both the flux qubit and spin ensemble. Here we show that this resonance is evidence of a collective dark state in the ensemble, which is coherently driven by the superposition of clockwise and counter-clockwise macroscopic persistent supercurrents flowing in the flux qubit. The collective dark state is a unique physical system and could provide a long-lived quantum memory. Recently, a sharp resonance was observed in the spectrum of a flux-qubit nitrogen-vacancy-centre hybrid quantum system that is much narrower than that of either the flux qubit or the spin ensemble. Zhu et al.investigate this resonance and find evidence of a coherently driven collective dark state.

Nature Communications•Apr 8, 2014•64 citations

Multi-mode storage and retrieval of microwave fields in a spin ensemble

Cécile Grèzes, Brian Julsgaard, Yuimaru Kubo +13 more

A quantum memory at microwave frequencies, able to store the state of multiple superconducting qubits for long times, is a key element for quantum information processing. Electronic and nuclear spins are natural candidates for the storage medium as their coherence time can be well above one second. Benefiting from these long coherence times requires to apply the refocusing techniques used in magnetic resonance, a major challenge in the context of hybrid quantum circuits. Here we report the first implementation of such a scheme, using ensembles of nitrogen-vacancy (NV) centres in diamond coupled to a superconducting resonator, in a setup compatible with superconducting qubit technology. We implement the active reset of the NV spins into their ground state by optical pumping and their refocusing by Hahn echo sequences. This enables the storage of multiple microwave pulses at the picoWatt level and their retrieval after up to $35 μ$s, a three orders of magnitude improvement compared to previous experiments.

arXiv:1401.7939•Jan 30, 2014•21 citations

Non-Markovian decoherence dynamics of strong-coupling hybrid quantum systems: A master equation approach

Kai-Ting Chiang, Wei-Min Zhang

Based on the experiments [S. Putz et al., Nat. Phys. 10, 720 (2014); Nat. Photonics 11, 36 (2017)] on the hybrid quantum system of a superconducting microwave cavity coupled strongly to an inhomogeneous broadening spin ensemble, we use the exact master equation theory to investigate its non-Markovian decoherence dynamics under external driving fields. In the experiments, the spin ensemble is made of negatively charged nitrogen-vacancy defects in diamond. The exact master equation theory generalizes the fluctuation-dissipation relation and depicts in details the transient non-Markovian decoherence, in which the dissipation (relaxation) and fluctuations (noise or dephasing) dynamics is well described and the non-Markovian memory effect can be well characterized. We study the physical picture of the transient non-Markovian decoherence dynamics and explore how the non-Markovian decoherence induced by the inhomogeneous broadening of the spin ensemble is suppressed in the strong-coupling regime. We also show how the spectral hole burning generates localized bound states for the further decoherence suppression. Furthermore, we investigate the two-time correlations to show the relationships between quantum fluctuations and quantum memory.

arXiv:2006.16064•Physical Review A•Jan 11, 2021•21 citations

Hybrid Quantum Systems with Collectively Coupled Spin States: Suppression of Decoherence through Spectral Hole Burning

Dmitry O. Krimer, Benedikt Hartl, Stefan Rotter

Spin ensemble based hybrid quantum systems suffer from a significant degree of decoherence resulting from the inhomogeneous broadening of the spin transition frequencies in the ensemble. We demonstrate that this strongly restrictive drawback can be overcome simply by burning two narrow spectral holes in the spin spectral density at judiciously chosen frequencies. Using this procedure we find an increase of the coherence time by more than an order of magnitude as compared to the case without hole burning. Our findings pave the way for the practical use of these hybrid quantum systems for the processing of quantum information.

arXiv:1501.03487•Physical Review Letters•Jul 14, 2015•24 citations
Rabi oscillations with a decay time of 26.7 μs are observed in a system comprising the electron spins in a diamond nitrogen–vacancy centre and a superconducting microwave cavity. Such oscillations are achieved by engineering the spectral hole burning of the spin ensemble. Spectral hole burning, used in inhomogeneously broadened emitters, is a well-established optical1 technique, with applications from spectroscopy to slow light2 and frequency combs3. In microwave photonics4, electron spin ensembles5,6 are candidates for use as quantum memories7 with potentially long storage times8. Here, we demonstrate long-lived collective dark states9 by spectral hole burning in the microwave regime10. The coherence time in our hybrid quantum system (nitrogen–vacancy centres strongly coupled to a superconducting microwave cavity) becomes longer than both the ensemble's free-induction decay and the bare cavity dissipation rate. The hybrid quantum system thus performs better than its individual subcomponents. This opens the way for long-lived quantum multimode memories, solid-state microwave frequency combs, spin squeezed states11, optical-to-microwave quantum transducers12 and novel metamaterials13. Beyond these, new cavity quantum electrodynamics experiments will be possible where spin–spin interactions and many-body phenomena14 are directly accessible.
The efficient generation, coherent control, manipulation and measurement of quantum states of light and matter is at the core of quantum technologies. Hybrid quantum systems, where one combines the best parts of multiple individual quantum systems together without their weaknesses, are now seen as a way to engineer composite quantum systems with the properties one requires. This would in principle allow one to probe new physical regimes. However, the issue until recently has been that hybridization has not resulted in systems with superior properties. Recently however we [Nature Photonics 11, 3639 (2016)] have shown an increased coherence times in hybrid system is of composed nitrogen-vacancy centers strongly coupled to a superconducting microwave resonator. This demonstration has enabled this kind of hybrid system to enter the regime where quantum nonlinearities are present. We discuss several types of nonlinearity effects that can be naturally explored (bistability and superradiance). Our work paves the way for the creation of spin squeezed states, novel metamaterials, long-lived quantum multimode memories and solid-state microwave frequency combs. Further in the longer term it may enable the exploration of many-body phenomena in new cavity quantum electrodynamics experiments.
Abstract A very promising recent trend in applied quantum physics is to combine the advantageous features of different quantum systems into what is called “hybrid quantum technology”. One of the key elements in this new field will have to be a quantum memory enabling to store quanta over extended periods of time. Systems that may fulfill the demands of such applications are comb‐shaped spin ensembles coupled to a cavity. Due to the decoherence induced by the inhomogeneous ensemble broadening, the storage time of these quantum memories is, however, still rather limited. Here we demonstrate how to overcome this problem by burning well‐placed holes into the spectral spin density leading to spectacular performance in the multimode regime. Specifically, we show how an initial excitation of the ensemble leads to the emission of more than a hundred well‐separated photon pulses with a decay rate significantly below the fundamental limit of the recently proposed “cavity protection effect”. image
The hybridization of distinct quantum systems has opened new avenues to exploit the best properties of these individual systems. Superconducting circuits and electron spin ensembles are one such example. Strong coupling and the coherent transfer and storage of quantum information has been achieved with nitrogen vacancy centres in diamond. Recently, we have observed a remarkably sharp resonance (~1 MHz) at 2.878 GHz in the spectrum of flux qubit negatively charged nitrogen vacancy diamond hybrid quantum system under zero external magnetic field. This width is much narrower than that of both the flux qubit and spin ensemble. Here we show that this resonance is evidence of a collective dark state in the ensemble, which is coherently driven by the superposition of clockwise and counter-clockwise macroscopic persistent supercurrents flowing in the flux qubit. The collective dark state is a unique physical system and could provide a long-lived quantum memory. Recently, a sharp resonance was observed in the spectrum of a flux-qubit nitrogen-vacancy-centre hybrid quantum system that is much narrower than that of either the flux qubit or the spin ensemble. Zhu et al.investigate this resonance and find evidence of a coherently driven collective dark state.
A quantum memory at microwave frequencies, able to store the state of multiple superconducting qubits for long times, is a key element for quantum information processing. Electronic and nuclear spins are natural candidates for the storage medium as their coherence time can be well above one second. Benefiting from these long coherence times requires to apply the refocusing techniques used in magnetic resonance, a major challenge in the context of hybrid quantum circuits. Here we report the first implementation of such a scheme, using ensembles of nitrogen-vacancy (NV) centres in diamond coupled to a superconducting resonator, in a setup compatible with superconducting qubit technology. We implement the active reset of the NV spins into their ground state by optical pumping and their refocusing by Hahn echo sequences. This enables the storage of multiple microwave pulses at the picoWatt level and their retrieval after up to 35μ35 μ35μs, a three orders of magnitude improvement compared to previous experiments.
Based on the experiments [S. Putz et al., Nat. Phys. 10, 720 (2014); Nat. Photonics 11, 36 (2017)] on the hybrid quantum system of a superconducting microwave cavity coupled strongly to an inhomogeneous broadening spin ensemble, we use the exact master equation theory to investigate its non-Markovian decoherence dynamics under external driving fields. In the experiments, the spin ensemble is made of negatively charged nitrogen-vacancy defects in diamond. The exact master equation theory generalizes the fluctuation-dissipation relation and depicts in details the transient non-Markovian decoherence, in which the dissipation (relaxation) and fluctuations (noise or dephasing) dynamics is well described and the non-Markovian memory effect can be well characterized. We study the physical picture of the transient non-Markovian decoherence dynamics and explore how the non-Markovian decoherence induced by the inhomogeneous broadening of the spin ensemble is suppressed in the strong-coupling regime. We also show how the spectral hole burning generates localized bound states for the further decoherence suppression. Furthermore, we investigate the two-time correlations to show the relationships between quantum fluctuations and quantum memory.
Spin ensemble based hybrid quantum systems suffer from a significant degree of decoherence resulting from the inhomogeneous broadening of the spin transition frequencies in the ensemble. We demonstrate that this strongly restrictive drawback can be overcome simply by burning two narrow spectral holes in the spin spectral density at judiciously chosen frequencies. Using this procedure we find an increase of the coherence time by more than an order of magnitude as compared to the case without hole burning. Our findings pave the way for the practical use of these hybrid quantum systems for the processing of quantum information.