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Journal of Low Temperature Physics

Inelastic Atom–Atom Collisions in an External Electromagnetic Field: Cooling of Dense Atomic Gases

Oleg Prepelita

Published May 15, 2015• 0 citations
Publisher
DOI
10.1007/s10909-015-1309-7

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Collisions of molecules in a thermal gas are difficult to control. Thermal motion randomizes molecular encounters and diminishes the effects of external radiation or static electromagnetic fields on intermolecular interactions. The effects of the thermal motion can be reduced by cooling molecular gases to low temperatures. At temperatures near or below 1 K, the collision energy of molecules becomes less significant than perturbations due to external fields. At the same time, inelastic scattering and chemical reactions may be very efficient in low-temperature molecular gases. The purpose of this article is to demonstrate that collisions of molecules at temperatures below 1 K can be manipulated by external electromagnetic fields and to discuss possible applications of cold controlled chemistry. The discussion focuses on molecular interactions at cold (0.001-2 K) and ultracold (<0.001 K) temperatures and is based on both recent theoretical and experimental work. The article concludes with a summary of current challenges for theory and experiment in the research of cold molecules and cold chemistry.
Collisions of molecules in a thermal gas are difficult to control. Thermal motion randomizes molecular encounters and diminishes the effects of external radiation or static electromagnetic fields on intermolecular interactions. The effects of the thermal motion can be reduced by cooling molecular gases to low temperatures. At temperatures near or below 1 K, the collision energy of molecules becomes less significant than perturbations due to external fields. At the same time, inelastic scattering and chemical reactions may be very efficient in low-temperature molecular gases. The purpose of this article is to demonstrate that collisions of molecules at temperatures below 1 K can be manipulated by external electromagnetic fields and to discuss possible applications of cold controlled chemistry. The discussion focuses on molecular interactions at cold (0.001-2 K) and ultracold (<0.001 K) temperatures and is based on both recent theoretical and experimental work. The article concludes with a summary of current challenges for theory and experiment in the research of cold molecules and cold chemistry.
We show that cross sections for inelastic collisions of ultracold atoms or molecules confined by a harmonic potential have the same energy dependence as in pure 2D geometry. This indicates that chemical reactions and inelastic collisions may be suppressed in an ultracold gas under strong confinement in one dimension. We present a numerical proof of the threshold collision laws in 2D. Our results indicate that inelastic collisions in weak electromagnetic fields may be controlled by varying the orientation of the external field axis with respect to the plane of confinement.