Interaction of intense laser pulses with ultra-cold atomic samples

Mihaela Vatasescu

Michelle Stephens, Kyle Taylor, Jacob Berg +3 more

D. Ciampini, F. Fuso, Jörg Helge Müller +3 more

The recent development of laser cooling and trapping techniques has made possible the controlled realization of dense and cold atomic samples, thus opening the way for spectroscopic investigations in the low and ultra-low temperature regimes not accessible with conventional techniques. In our lab, an apparatus for laser cooling and Bose-Einstein condensation of rubidium atoms is in operation, producing a sample large enough to perform reliable investigations by absorption or emission techniques. Moving from previous photoionization experiments of laser-cooled atoms in a magneto-optical trap irradiated by cw-laser radiation [1] and stimulated by the interest grown recently on ultra-cold plasma [2], we have started a series of experiments aimed at investigating the interaction of intense laser pulses with the ultra-cold neutral sample, boty aboeand below the condensation temperature. Radiation from an excimer-pumped dye laser was used at a wavelength close to 594 nm, corresponding to the ionization threshold of rubidium for two photon non-resonant absorption from the ground state, with intensities in the tens of MW/cm^2 range and a pulse duration of 16 ns. Preliminary results, attained through the dynamical analysis (atom number, temperature) of the cold atom sample after the arrival of the laser pulse, suggest the occurrence of different processes, initiated by multi-photon ionization, involving collisions between cold electrons and ultra-cold neutrals, recombination at low temperatures and collective processes in the weak and cold plasma. Interpretation of those results demonstrates that this class of experiments, based on a variety of topics typical of atomic, plasma and statistical physics, can open the way for novel and intriguing investigations of laser-matter interaction. Further experimental developments will include duplication of the laser pulse frequency and one photon ionization of ground state rubidium laser-cooled atoms. [1] O. Maragò et al., Phys. Rev. A 57 R4110 (1998); E., Arimondo et al., Appl. Surf. Sci. 154-155 527 (2000); F. Fuso et al., Opt. Commun. 173 223 (2000). [2] T.C. Killian et al., Phys. Rev. Lett. 83 4776 (1999); S. Kulin et al., Phys. Rev. Lett. 85 318 (2000).

Karen Chamberlin, Derek Lilla, Kyle Taylor +3 more

Jack Saywell

Atom interferometric sensors can enable extremely precise measurements of inertial motion and external fields by manipulating and interfering atomic states using pulses of laser light. However, like many experiments that require the coherent control of a quantum system, the interaction fidelity is limited by inhomogeneities in the control fields. Variations in atomic velocity and laser intensity lead different atoms to experience different interactions under the same pulse, reducing the interference fringe contrast, introducing bias, and limiting the sensitivity. We present the theoretical design and experimental demonstration of pulses for atom interferometry which compensate inhomogeneities in atomic velocity and laser intensity. By varying the laser phase throughout a pulse and choosing an appropriate fidelity measure to be maximised, pulses are optimised by adapting optimal control techniques originally designed for nuclear magnetic resonance applications. We show using simulations that optimised pulses significantly improve the fidelity of interferometer operations and verify this experimentally using Raman transitions within a cold sample of 85Rb atoms. We demonstrate a robust state-transfer pulse that achieves a fidelity of 99.8(3)% in a ∼ 35 µK sample and obtain a threefold increase in the fringe contrast using a full sequence of optimised pulses. Many of the pulse shapes found by optimal control are simple and symmetrical, and we show that certain symmetries are integral to error compensation. By systematically exploring the dependence of these solutions on the model and optimisation parameters, we demonstrate a stability which underlines the general applicability of optimised pulses to a range of interferometer configurations. Finally, we introduce and computationally analyse a novel theoretical approach to improve the sensitivity of large-momentum-transfer (LMT) interferometers, whereby “biselective” pulses are optimised to track the changing resonance conditions encountered in extended pulse sequences that are designed to increase the measurement sensitivity. When conventional pulses of steady phase are used, the interference contrast decays rapidly as extra pulses are added because of the change in resonance. Using numerical simulations, we show that bi-selective pulses maintain interaction fidelity throughout extended pulse sequences, allowing significant increases in the sensitivity that may be obtained using LMT.

Duncan Tate, R.E. Wilson, Margaret S. Martei +1 more

We discuss our progress towards achieving external control of the electron temperature and the Coulomb coupling parameter of ultra-cold plasmas. Using a Littman dye laser, we create the plasma by partially photoionizing a dense, cold sample of rubidium atoms in a magneto-optical trap (MOT). At a controllable time delay, we excite neutral atoms in the plasma to a specific Rydberg state using a narrow bandwidth pulsed laser. We have made very qualitative measurements of the electron temperature as a function of delay from the exciting laser pulses. Some of our results suggest that the plasma is stabilized by the presence of the Rydberg atoms, with a longer lifetime and slower expansion rate than a plasma that evolves directly from a dense Rydberg sample.