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Bulletin of the American Physical Society

Crystallization of photons via light storage in Rydberg gases

Matthias Moos, Johannes Otterbach, Dominik Muth, Michael Fleischhauer

Published Jun 5, 2013• 0 citations
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Physics Photons are ideal carriers of information. They are fast and coherent, and because they don't interact much with each other they can have very long lifetimes. However, stopping, processing, and manipulating the photons requires them to be stored in a memory, where doing so can damage their fragile quantum properties, which leads to a loss of coherence. Although photons have been coherently stored in and retrieved from ensembles of atom gases, both warm and cold atom clouds, for practical applications a solid-state memory would be desired. Heinze et al. have developed a method to enhance the storage time of photons in a rare-earth–ion—doped crystal. They use a series of laser pulses to initialize the crystal for photon storage and then load it with their “information photons.” By iteratively optimizing the experimental parameters, they show that they can store light pulses and even entire images in the crystal and then retrieve them up to a minute later with their coherent properties intact. The results present an important step toward building a viable quantum network. Phys. Rev. Lett. 111 , 033601(2013).

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We propose a new method to create two-photon states in a controllable way using interaction between the Rydberg atoms during the storage and retrieval of slow light. A distinctive feature of the suggested procedure is that the slow light is stored into a superposition of two atomic coherences under conditions of electromagnetically induced transparency (EIT). Interaction between the atoms during the storage period creates entangled pairs of atoms in a superposition state that is orthogonal to the initially stored state. Restoring the slow light from this new atomic state one can produce a two photon state with a second-order correlation function determined by the atom-atom interaction and the storage time. Therefore the measurement of the restored light allows one to probe the atom-atom coupling by optical means with a sensitivity that can be increased by extending the storage time. As a realization of this idea we consider a many-body Ramsey-type technique which involves pi/2 pulses creating a superposition of Rydberg states at the beginning and the end of the storage period. In that case the regenerated light is due to the resonance dipole-dipole interaction between the atoms in the Rydberg states.

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We present an improved version of the superatom (SA) model to examine the slow-light dynamics of a few-photons signal field in cold Rydberg atoms with van der Waals (vdW) interactions. A main feature of this version is that it promises consistent estimations on total Rydberg excitations based on dynamic equations of SAs or atoms. We consider two specific cases in which the incident signal field contains more photons with a smaller detuning or less photons with a larger detuning so as to realize the single-photon-level light storage. It is found that vdW interactions play a significant role even for the slow-light dynamics of a single-photon signal field as distributed Rydberg excitations are inevitable in the picture of dark-state polariton. Moreover, the stored (retrieved) signal field exhibits a clearly asymmetric (more symmetric) profile because its leading and trailing edges undergo different (identical) traveling journeys, and higher storage/retrieval efficiencies with well preserved profiles apply only to weaker and well detuned signal fields. These findings are crucial to understand the nontrivial interplay of single-photon-level light storage and distributed Rydberg excitations.

Frontiers of Physics•Aug 27, 2021•8 citations
Physics Photons are ideal carriers of information. They are fast and coherent, and because they don't interact much with each other they can have very long lifetimes. However, stopping, processing, and manipulating the photons requires them to be stored in a memory, where doing so can damage their fragile quantum properties, which leads to a loss of coherence. Although photons have been coherently stored in and retrieved from ensembles of atom gases, both warm and cold atom clouds, for practical applications a solid-state memory would be desired. Heinze et al. have developed a method to enhance the storage time of photons in a rare-earth–ion—doped crystal. They use a series of laser pulses to initialize the crystal for photon storage and then load it with their “information photons.” By iteratively optimizing the experimental parameters, they show that they can store light pulses and even entire images in the crystal and then retrieve them up to a minute later with their coherent properties intact. The results present an important step toward building a viable quantum network. Phys. Rev. Lett. 111 , 033601(2013).
We propose a new method to create two-photon states in a controllable way using interaction between the Rydberg atoms during the storage and retrieval of slow light. A distinctive feature of the suggested procedure is that the slow light is stored into a superposition of two atomic coherences under conditions of electromagnetically induced transparency (EIT). Interaction between the atoms during the storage period creates entangled pairs of atoms in a superposition state that is orthogonal to the initially stored state. Restoring the slow light from this new atomic state one can produce a two photon state with a second-order correlation function determined by the atom-atom interaction and the storage time. Therefore the measurement of the restored light allows one to probe the atom-atom coupling by optical means with a sensitivity that can be increased by extending the storage time. As a realization of this idea we consider a many-body Ramsey-type technique which involves pi/2 pulses creating a superposition of Rydberg states at the beginning and the end of the storage period. In that case the regenerated light is due to the resonance dipole-dipole interaction between the atoms in the Rydberg states.
We present an improved version of the superatom (SA) model to examine the slow-light dynamics of a few-photons signal field in cold Rydberg atoms with van der Waals (vdW) interactions. A main feature of this version is that it promises consistent estimations on total Rydberg excitations based on dynamic equations of SAs or atoms. We consider two specific cases in which the incident signal field contains more photons with a smaller detuning or less photons with a larger detuning so as to realize the single-photon-level light storage. It is found that vdW interactions play a significant role even for the slow-light dynamics of a single-photon signal field as distributed Rydberg excitations are inevitable in the picture of dark-state polariton. Moreover, the stored (retrieved) signal field exhibits a clearly asymmetric (more symmetric) profile because its leading and trailing edges undergo different (identical) traveling journeys, and higher storage/retrieval efficiencies with well preserved profiles apply only to weaker and well detuned signal fields. These findings are crucial to understand the nontrivial interplay of single-photon-level light storage and distributed Rydberg excitations.