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Ukrainian Journal of Physics

Application of the Generalized Absorptance for Accounting the Recoil and Doppler Effects

Андрій Сіжук, S. M. Yezhov

Published May 1, 2017• 0 citations
Publisher

Abstract

A method of calculation of the absorption coefficient in the terms of quantum optics with regard for the quantization of the electromagnetic field and the Doppler effect is presented. It is shown that the local value of the absorption coefficient non-linearly depends on the atomic density and initial intensity. The analytically derived results are demonstrated in graphs for the the local absorption coefficient as a function of the frequency. The relatively strong dependence of the absorptance on the path length of an optical light beam is caused by the interatomic coupling through the intermediary of an electromagnetic field. The splitting of the absorption line induced by the Doppler effect in the system placed between mirrors is demonstrated.

DOI
10.15407/ujpe62.04.0299

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A method of calculation of the absorption coefficient in the terms of quantum optics with regard for the quantization of the electromagnetic field and the Doppler effect is presented. It is shown that the local value of the absorption coefficient non-linearly depends on the atomic density and initial intensity. The analytically derived results are demonstrated in graphs for the the local absorption coefficient as a function of the frequency. The relatively strong dependence of the absorptance on the path length of an optical light beam is caused by the interatomic coupling through the intermediary of an electromagnetic field. The splitting of the absorption line induced by the Doppler effect in the system placed between mirrors is demonstrated.
The quantum optical theory of absorption/reemission properties of a system of interacting atoms is discussed. The calculation method of the absorption coefficient is developed with regard for the quantization of field, thermal atomic motion, Doppler effect, and the model interaction between atoms. It is shown that the formulation of the absorption coefficient in the quantum optical context is based on the commutation relation between the operators of electric field and intensity. The revealed non-linear dependence of the absorption coefficient on the atomic density, even in the case of negligible binary interaction, can be referred to a certain kind of quantum-optic collective effects.
The spatial inhomogeneity of absorption coefficient of the space between mirrors, filled by an optically active gas, is analyzed in quantum optical terms. It was theoretically shown, that the quantization of electromagnetic field in a cavity (optical resonator) can reveal the spatial inhomogeneity of absorption or re-emission ability of the optically active medium. It appears from the analytical calculations, the inhomogeneity is caused by the Doppler frequency shifts (including recoil effects) during the atom-photon collisions and the non-zero initial frequency width of the scanning signal. The proposed analytical representation of the absorption coefficient through the additive quantum optical terms gives deeper insight into intrinsic processes in the interacting with light matter.
Quantum optical theory of absorption properties of interacting atoms is developed. The concept of local absorptance is introduced as a derivative of the logarithm of intensity with respect to the distance in the vicinity of a given spatial point and a moment of time. The intensity is represented by the quantum and statistically averaged normal product of creation and annihilation operators of the electromagnetic field. The development of an analytical method of the estimation for the kinetic and optical parameters for the system is proposed here. The calculation method of the absorption coefficient includes thermal atomic motion, Doppler effect, and the short-range interaction between atoms. The absorption coefficient explicitly takes into account the quantum nature of the optical field. The ability of the system to absorb or emit quanta is quantitatively expressed through the special form of interaction integrals. The specific form of integrals results from the structure of the quantum brackets. The interplay between the collective (virtual photon exchange) and binary (optically induced inter-particle bonding) processes determines the system behavior. The spectral profile of the local absorption coefficient for different atomic densities and time intervals is simulated for realistic parameters.
The recoil of a neutral atom irradiated by counter-propagating light with the same frequency and intensity is studied. The expectation value of the momentum transferred from the light to the atom with spherical symmetry at rest is usually zero because of symmetry. However, if the optical absorption coefficient of the atom depends on the incident light direction due to the magnetoelectric effect, as is the case in materials with nonreciprocal directional dichroism, the momentum transfer between the atom and photons depends on the incident direction. This allows even a standing electromagnetic wave to break the symmetry of the recoil of an atom.
A theoretical analysis is made of a resonant interaction of two-level atoms with the field of three strong spatially separated standing waves. It is shown that this interaction should give rise to a resonance of width equal to the reciprocal of the transit time between the fields and this resonance should be observed for all rational values of the ratio of the distances by which the waves are separated in space. Calculations are made of the corrections to the flux of particles excited in an atomic beam and to the power absorbed by a gas because of the interaction of atoms with the three fields. It is found that because of recoil a resonance of this kind splits into an infinite series of components separated by intervals of the order of the recoil frequency. The results are given of a numerical calculation of the strongest components of this resonance. The shift and deformation of lines due to quadratic Doppler effect are considered. The results of the calculations are compared with the available experimental data.
It is shown that, in general, the interaction between relaxing quantum systems and radiation is described by non-Markov transport equations for the density matrix ρ p and the relaxation matrix depends on the properties of the radiation. The usual Markov-type equations for ρ p are obtained from these equations if γτ c ≪1 and (∊ 2 +4 V 2 ) 1/2 τ c ≪1 (γ is the width of the investigated transition in a quantum system, rc is the correlation time of the perturbations causing relaxation, e is the frequency detuning, and V is the energy of the interaction between the system and the radiation field). When the second inequality is disobeyed, the relaxation process deviates strongly from the Markov type. In the case of small values of V , this results in a non-Lorentzian profile of the absorption lines characterized by a steep descent in the wings. In the range of high values of V , when 2 V τ c 1, the whole relaxation process becomes greatly modified: the dependence of the relaxation coefficients on V becomes strong and a coupling appears between the relaxations of the diagonal and the nondiagonal elements of the density matrix. This is manifested, in particular, in the saturation effect: the term describing saturation in the expression for the polarizability changes considerably and the expression for the line width loses the component due to the adiabatic (elastic) perturbation.