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Bulletin of the American Physical Society

Absolute frequency measurement of the $^{1}$S$_{0}$$\leftrightarrow$$^{3}$P$_{0}$ clock transition at 578.4 nm in ytterbium

Chad Hoyt, Zeb W. Barber, Chris W. Oates, Tara M. Fortier, Scott A. Diddams, Leo W. Hollberg

Published May 18, 2005• 0 citations
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Absolute frequency measurement of the 1^{1}1S0_{0}0​↔\leftrightarrow↔3^{3}3P0_{0}0​ clock transition at 578.4 nm in ytterbium
Observation of the 1^{1}1S0_{0}0​ -- 3^33P0_00​ clock transition at 578 nm in atomic Yb
A cavity-stabilized 578 nm laser is used to probe the clock transition of ytterbium atoms trapped in optical lattice sites. We obtain a Fourier-limited 4.2-Hz-linewidth Rabi spectrum and a Ramsey spectrum with fringe linewidth of 3.3 Hz. Based on one of the spectra, the 578 nm laser light is frequency-stabilized to the center of the transition to achieve a closed-loop operation of an optical clock. Based on interleaved measurement, the frequency instability of a single optical clock is demonstrated to be 5.4 × 10-16/√τ.
Clock transition at 1.14μm1.14 \mu \mathrm{m}1.14μm in neutral thulium is a promising candidate for compact and robust transportable optical clock due to its extremely low sensitivity to external electric and magnetic fields. Cold Tm atoms are now used in optical lattice clocks, quantum simulators and for the study of Bose-Einstein condensation and cold collision physics. In this work, we discuss experimentally measured absolute frequencies of the two transitions at 410.6 nm and 530.7 nm, used for laser cooling of thulium atoms, transition at 418.8 nm used for optical pumping and clock transition at 1140 nm. Using accurate laser spectroscopy in an ensemble of cold thulium atoms, we measured frequencies of these transitions using an optical frequency comb, which was referenced to an active hydrogen maser. Transition frequencies were measured with an uncertainty at one tenth of their natural linewidth, which is sufficient for cooling and pumping of thulium atoms. The uncertainty of the clock transition frequency is 30 Hz, which was limited by the maser frequency calibration with GNSS. Our results can find application in existing experiments with cold thulium atoms and especially in new projects.