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Prospect for bad cavity laser on large ion crystal

Georgy A. Kazakov, Justin Bohnet, Thorsten Schumm

Published Apr 26, 2017• 3 citations
OpenAlex

Abstract

Here we study the possibilities of creating a bad cavity laser on forbidden transition in cold ions forming large Coulomb crystal in linear Paul trap. We consider micromotion-induced shifts and coupling strengths, and perform quantitative estimations of the attainable laser power for lasing on the ${^3D_2} \rightarrow {^1S_0}$ transition in ${\rm ^{176}Lu^+}$ ions in a spherical-symmetric trap.

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Prospects for a bad-cavity laser using a large ion crystal

Georgy A. Kazakov, Justin Bohnet, Thorsten Schumm

We propose to build a bad-cavity laser using forbidden transitions in large ensembles of cold ions that form a Coulomb crystal in a linear Paul trap. This laser might realize an active optical frequency standard able to serve as a local oscillator in next-generation optical clock schemes. In passive optical clocks, large ensembles of ions appear less promising, as they suffer from inhomogeneous broadening due to quadrupole interactions and micromotion-related shifts. In bad-cavity lasers, however, the radiating dipoles can synchronize and generate stable and narrow-linewidth radiation. Furthermore, for specific ions, micromotion-induced shifts can be largely suppressed by operating the ion trap at a magic frequency. We discuss the output radiation properties and perform quantitative estimations for lasing on the ${}^{3}{D}_{2}\ensuremath{\rightarrow}{}^{1}{S}_{0}$ transition in $^{176}\mathrm{Lu}{}^{+}$ ions in a spherically symmetric trap.

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Superradiant lasers have emerged as a promising platform for optical frequency references due to their potential to achieve exceptionally narrow linewidths with reduced sensitivity to cavity noise. Trapped ion Coulomb crystals provide an attractive emitting medium due to their long coherence times, great environmental isolation and precise control over their motional dynamics. However, scaling trapped ion systems to the large ion numbers required for strong collective emission introduces new challenges, including crystal stability and position-dependent decoherence mechanisms. This work presents a numerical framework for modelling large Coulomb crystals confined within a linear Paul trap and assessing their suitability for superradiant lasing. A numerical simulation was developed to generate equilibrium crystal configurations, followed by a normal mode analysis to verify crystal’s dynamical stability and characterise the collective motional spectrum. The dependence of the crystal properties on the trapping parameters was examined, while the damping coefficient and integration timestep used in the numerical relaxation procedure were systematically optimised to obtain equilibrium configurations. The decoherence mechanisms expected to influence superradiant operation, including RF micromotion and electric quadrupole shifts, were also investigated as functions of ion number and trapping conditions. The simulations can produce accurate models of mechanically stable Coulomb crystals with up to 10,000 ions under appropriate relaxation conditions. They also show how the collective motional spectrum evolves across the trapping parameter space where they were also compared with the theoretical lasing threshold to assess the suitability of the trapping conditions for superradiant operation. Although the largest micromotion amplitudes increase with crystal size, a significant fraction of the ions remain confined close to the RF null, suggesting that large ion numbers may still be compatible with superradiant operation. The developed framework also provides a means of quantifying the quadrupole shift, indicating that the resulting frequency shifts are relatively small for the trapping parameters considered here, although further optimisation of the operating conditions is required to fully assess their influence on superradiant perfomance. Overall, the computational suite developed here establishes a versatile platform for studies of large Coulomb ion crystals and provides the tools to determine whether superradiant lasing thresholds can be reached with trapped ion crystals.

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Role of laser damping in trapped ion crystals

Ralph G. DeVoe, John A. Hoffnagle, Richard G. Brewer

It is currently thought that the laser cooling of an ordered ion array, an ion crystal, is qualitatively the same as that of a single ion. We show that this assumption is strongly violated in recent experiments in Paul traps, due to ion micromotion. Our analysis demonstrates an unexpected laser damping instability that induces an ion-crystal order-chaos transition and also explains why ion crystals in Paul traps have been limited to less than 100 ions. We directly observe the effects of ion micromotion on the laser cooling of a single trapped ${\mathrm{Ba}}^{+}$ ion by a new technique.

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The concept of an active optical frequency standard was proposed about 10 years ago. The idea was to use optically trapped alkaline-earth atoms as a gain medium to built an extremely narrow-line laser, whose frequency would be robust against fluctuations of the cavity length. The main challenge in the realization of this concept is the short trap lifetime of the atoms. Recently we showed, that in such a laser, neutral atoms may be replaced by charged ions in a radio-frequency (RF) Paul trap with much longer lifetime. This idea rests on two pillars: the effect of synchronization of radiating dipoles with moderate inhomogeneous broadening, and the possibility to compensate (in leading orders) micromotion-induced shifts for some ion species in specially designed traps.

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Inhibition of laser cooling in Paul traps

Ralph G. DeVoe, John A. Hoffnagle, Richard G. Brewer

Several groups have recently used laser cooling to produce ordered arrays of ions, ion crystals, in rf quadrupole ion traps (Paul traps). Laser cooling has been understood using previous theories which ignore ion micromotion and replace the oscillating rf trap potential with a static pseudopotential. We show that in recent experiments, ion micromotion can exceed one wavelength of the cooling radiation and that the resulting Doppler shifts can transform laser cooling into laser heating. Changes in trap voltage, ion position, and laser intensity can all reverse the sign of laser cooling. This, together with ideas of deterministic chaos, can lead to a reinterpretation of experiments on ion crystals. The recognition that effects previously attributed to an experimental artifact, rf heating, may actually be due to a failure of laser cooling opens the door, on the one hand, to precise theories of phase transitions and, on the other, to improved cooling techniques that can permit the creation of larger ion crystals.

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Radial Two-Dimensional Ion Crystals in a Linear Paul Trap

Marissa D’Onofrio, Yuanheng Xie, A. J. Rasmusson +3 more

We experimentally study two-dimensional (2D) Coulomb crystals in the "radial-2D" phase of a linear Paul trap. This phase is identified by a 2D ion lattice aligned entirely with the radial plane and is created by imposing a large ratio of axial to radial trapping potentials. Using arrays of up to 19 ^{171}Yb^{+} ions, we demonstrate that the structural phase boundaries of such crystals are well described by the pseudopotential approximation, despite the time-dependent ion positions driven by intrinsic micromotion. We further observe that micromotion-induced heating of the radial-2D crystal is confined to the radial plane. Finally, we verify that the transverse motional modes, which are used in most ion-trap quantum simulation schemes, are well-predictable numerically and remain decoupled and cold in this geometry. Our results establish radial-2D ion crystals as a robust experimental platform for realizing a variety of theoretical proposals in quantum simulation and computation.

arXiv:2012.12766•Physical Review Letters•Jul 9, 2021•40 citations
Here we study the possibilities of creating a bad cavity laser on forbidden transition in cold ions forming large Coulomb crystal in linear Paul trap. We consider micromotion-induced shifts and coupling strengths, and perform quantitative estimations of the attainable laser power for lasing on the 3D2→1S0{^3D_2} \rightarrow {^1S_0}3D2​→1S0​ transition in 176Lu+{\rm ^{176}Lu^+}176Lu+ ions in a spherical-symmetric trap.
We propose to build a bad-cavity laser using forbidden transitions in large ensembles of cold ions that form a Coulomb crystal in a linear Paul trap. This laser might realize an active optical frequency standard able to serve as a local oscillator in next-generation optical clock schemes. In passive optical clocks, large ensembles of ions appear less promising, as they suffer from inhomogeneous broadening due to quadrupole interactions and micromotion-related shifts. In bad-cavity lasers, however, the radiating dipoles can synchronize and generate stable and narrow-linewidth radiation. Furthermore, for specific ions, micromotion-induced shifts can be largely suppressed by operating the ion trap at a magic frequency. We discuss the output radiation properties and perform quantitative estimations for lasing on the ${}^{3}{D}_{2}\ensuremath{\rightarrow}{}^{1}{S}_{0}$ transition in 176Lu+^{176}\mathrm{Lu}{}^{+}176Lu+ ions in a spherically symmetric trap.
Superradiant lasers have emerged as a promising platform for optical frequency references due to their potential to achieve exceptionally narrow linewidths with reduced sensitivity to cavity noise. Trapped ion Coulomb crystals provide an attractive emitting medium due to their long coherence times, great environmental isolation and precise control over their motional dynamics. However, scaling trapped ion systems to the large ion numbers required for strong collective emission introduces new challenges, including crystal stability and position-dependent decoherence mechanisms. This work presents a numerical framework for modelling large Coulomb crystals confined within a linear Paul trap and assessing their suitability for superradiant lasing. A numerical simulation was developed to generate equilibrium crystal configurations, followed by a normal mode analysis to verify crystal’s dynamical stability and characterise the collective motional spectrum. The dependence of the crystal properties on the trapping parameters was examined, while the damping coefficient and integration timestep used in the numerical relaxation procedure were systematically optimised to obtain equilibrium configurations. The decoherence mechanisms expected to influence superradiant operation, including RF micromotion and electric quadrupole shifts, were also investigated as functions of ion number and trapping conditions. The simulations can produce accurate models of mechanically stable Coulomb crystals with up to 10,000 ions under appropriate relaxation conditions. They also show how the collective motional spectrum evolves across the trapping parameter space where they were also compared with the theoretical lasing threshold to assess the suitability of the trapping conditions for superradiant operation. Although the largest micromotion amplitudes increase with crystal size, a significant fraction of the ions remain confined close to the RF null, suggesting that large ion numbers may still be compatible with superradiant operation. The developed framework also provides a means of quantifying the quadrupole shift, indicating that the resulting frequency shifts are relatively small for the trapping parameters considered here, although further optimisation of the operating conditions is required to fully assess their influence on superradiant perfomance. Overall, the computational suite developed here establishes a versatile platform for studies of large Coulomb ion crystals and provides the tools to determine whether superradiant lasing thresholds can be reached with trapped ion crystals.
It is currently thought that the laser cooling of an ordered ion array, an ion crystal, is qualitatively the same as that of a single ion. We show that this assumption is strongly violated in recent experiments in Paul traps, due to ion micromotion. Our analysis demonstrates an unexpected laser damping instability that induces an ion-crystal order-chaos transition and also explains why ion crystals in Paul traps have been limited to less than 100 ions. We directly observe the effects of ion micromotion on the laser cooling of a single trapped Ba+{\mathrm{Ba}}^{+}Ba+ ion by a new technique.
The concept of an active optical frequency standard was proposed about 10 years ago. The idea was to use optically trapped alkaline-earth atoms as a gain medium to built an extremely narrow-line laser, whose frequency would be robust against fluctuations of the cavity length. The main challenge in the realization of this concept is the short trap lifetime of the atoms. Recently we showed, that in such a laser, neutral atoms may be replaced by charged ions in a radio-frequency (RF) Paul trap with much longer lifetime. This idea rests on two pillars: the effect of synchronization of radiating dipoles with moderate inhomogeneous broadening, and the possibility to compensate (in leading orders) micromotion-induced shifts for some ion species in specially designed traps.
Several groups have recently used laser cooling to produce ordered arrays of ions, ion crystals, in rf quadrupole ion traps (Paul traps). Laser cooling has been understood using previous theories which ignore ion micromotion and replace the oscillating rf trap potential with a static pseudopotential. We show that in recent experiments, ion micromotion can exceed one wavelength of the cooling radiation and that the resulting Doppler shifts can transform laser cooling into laser heating. Changes in trap voltage, ion position, and laser intensity can all reverse the sign of laser cooling. This, together with ideas of deterministic chaos, can lead to a reinterpretation of experiments on ion crystals. The recognition that effects previously attributed to an experimental artifact, rf heating, may actually be due to a failure of laser cooling opens the door, on the one hand, to precise theories of phase transitions and, on the other, to improved cooling techniques that can permit the creation of larger ion crystals.
We experimentally study two-dimensional (2D) Coulomb crystals in the "radial-2D" phase of a linear Paul trap. This phase is identified by a 2D ion lattice aligned entirely with the radial plane and is created by imposing a large ratio of axial to radial trapping potentials. Using arrays of up to 19 ^{171}Yb^{+} ions, we demonstrate that the structural phase boundaries of such crystals are well described by the pseudopotential approximation, despite the time-dependent ion positions driven by intrinsic micromotion. We further observe that micromotion-induced heating of the radial-2D crystal is confined to the radial plane. Finally, we verify that the transverse motional modes, which are used in most ion-trap quantum simulation schemes, are well-predictable numerically and remain decoupled and cold in this geometry. Our results establish radial-2D ion crystals as a robust experimental platform for realizing a variety of theoretical proposals in quantum simulation and computation.