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Bulletin of the American Physical Society

Intensity-modulated polarizabilities and magic trapping of alkali-metal and divalent atoms in infrared optical lattices

Türker Topçu, Andrei Derevianko

Published Jun 4, 2014• 0 citations
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Intensity landscape and the possibility of magic trapping of alkali-metal Rydberg atoms in infrared optical lattices

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Motivated by compelling advances in manipulating cold Rydberg (Ry) atoms in optical traps, we consider the effect of the large extent of a Ry electron wave function on trapping potentials. We find that, when the Ry orbit lies outside inflection points in the laser intensity landscape, the atom can stably reside in laser intensity maxima. Effectively, the free-electron ac polarizability of the Ry electron is modulated by the intensity landscape and can accept both positive and negative values. We apply these insights to determining the magic wavelengths for Ry-ground-state transitions for alkali-metal atoms trapped in infrared optical lattices. We find magic wavelengths to be around $10\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{m}$ with exact values that depend on Ry-state quantum numbers.

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We develop a theoretical understanding of the trapping of divalent Rydberg atoms in optical lattices. Because the size of the Rydberg electron cloud can be comparable to the scale of spatial variations of laser intensity, we pay special attention to averaging optical fields over the atomic wave functions. The optical potential is proportional to the ac Stark polarizability. We find that in the independent-particle approximation for the valence electrons, this polarizability breaks into two contributions: the singly ionized core polarizability and the contribution from the Rydberg electron. Unlike the usually employed free-electron polarizability, the Rydberg contribution depends both on the laser intensity profile and on the rotational symmetry of the total electronic wave function. We focus on the $J=0$ Rydberg states of Sr and evaluate the dynamic polarizabilities of the $5sns$(${}^{1}{S}_{0}$) and $5snp$(${}^{3}{P}_{0}$) Rydberg states. We specifically chose the Sr atom for its optical-lattice clock applications. We find that there are several magic wavelengths in the infrared region of the spectrum at which the differential Stark shift between the clock states [$5{s}^{2}$(${}^{1}{S}_{0}$) and $5s5p$(${}^{3}{P}_{0}$)] and the $J=0$ Rydberg states [$5sns$(${}^{1}{S}_{0}$) and $5snp$(${}^{3}{P}_{0}$)] vanishes. We tabulate these wavelengths as a function of the principal quantum number $n$ of the Rydberg electron. We find that because the contribution to the total polarizability from the Rydberg electron vanishes at short wavelengths, magic wavelengths below $\ensuremath{\sim}$1000 nm are ``universal'' as they do not depend on the principal quantum number $n$.

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Tune-out wavelengths and landscape-modulated polarizabilities of alkali-metal Rydberg atoms in infrared optical lattices

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Intensity-modulated optical lattice potentials can change sign for an alkali-metal Rydberg atom, and the atoms are not always attracted to intensity minima in optical lattices with wavelengths near the CO${}_{2}$ laser band. Here we demonstrate that such IR lattices can be tuned so that the trapping potential experienced by the Rydberg atom can be made to vanish for atoms in ``targeted'' Rydberg states. Such state-selective trapping of Rydberg atoms can be useful in controlled cold Rydberg collisions, cooling Rydberg states, and species-selective trapping and transport of Rydberg atoms in optical lattices. We tabulate wavelengths at which the trapping potential vanishes for the $ns$, $np$, and $nd$ Rydberg states of Na and Rb atoms and discuss advantages of using such optical lattices for state-selective trapping of Rydberg atoms. We also develop exact analytical expressions for the lattice-induced polarizability for the ${m}_{z}=0$ Rydberg states and derive an accurate formula predicting tune-out wavelengths at which the optical trapping potential becomes invisible to Rydberg atoms in targeted $l=0$ states.

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Magic wavelengths for optically trapped atoms

Bindiya Arora, Marianna S. Safronova, Charles W. Clark

Bulletin of the American Physical Society•Mar 24, 2011•0 citations
Motivated by compelling advances in manipulating cold Rydberg (Ry) atoms in optical traps, we consider the effect of the large extent of a Ry electron wave function on trapping potentials. We find that, when the Ry orbit lies outside inflection points in the laser intensity landscape, the atom can stably reside in laser intensity maxima. Effectively, the free-electron ac polarizability of the Ry electron is modulated by the intensity landscape and can accept both positive and negative values. We apply these insights to determining the magic wavelengths for Ry-ground-state transitions for alkali-metal atoms trapped in infrared optical lattices. We find magic wavelengths to be around $10\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{m}$ with exact values that depend on Ry-state quantum numbers.
We develop a theoretical understanding of the trapping of divalent Rydberg atoms in optical lattices. Because the size of the Rydberg electron cloud can be comparable to the scale of spatial variations of laser intensity, we pay special attention to averaging optical fields over the atomic wave functions. The optical potential is proportional to the ac Stark polarizability. We find that in the independent-particle approximation for the valence electrons, this polarizability breaks into two contributions: the singly ionized core polarizability and the contribution from the Rydberg electron. Unlike the usually employed free-electron polarizability, the Rydberg contribution depends both on the laser intensity profile and on the rotational symmetry of the total electronic wave function. We focus on the J=0J=0J=0 Rydberg states of Sr and evaluate the dynamic polarizabilities of the 5sns5sns5sns(1S0{}^{1}{S}_{0}1S0​) and 5snp5snp5snp(3P0{}^{3}{P}_{0}3P0​) Rydberg states. We specifically chose the Sr atom for its optical-lattice clock applications. We find that there are several magic wavelengths in the infrared region of the spectrum at which the differential Stark shift between the clock states [5s25{s}^{2}5s2(1S0{}^{1}{S}_{0}1S0​) and 5s5p5s5p5s5p(3P0{}^{3}{P}_{0}3P0​)] and the J=0J=0J=0 Rydberg states [5sns5sns5sns(1S0{}^{1}{S}_{0}1S0​) and 5snp5snp5snp(3P0{}^{3}{P}_{0}3P0​)] vanishes. We tabulate these wavelengths as a function of the principal quantum number nnn of the Rydberg electron. We find that because the contribution to the total polarizability from the Rydberg electron vanishes at short wavelengths, magic wavelengths below $\ensuremath{\sim}$1000 nm are ``universal'' as they do not depend on the principal quantum number nnn.
Intensity-modulated optical lattice potentials can change sign for an alkali-metal Rydberg atom, and the atoms are not always attracted to intensity minima in optical lattices with wavelengths near the CO2{}_{2}2​ laser band. Here we demonstrate that such IR lattices can be tuned so that the trapping potential experienced by the Rydberg atom can be made to vanish for atoms in ``targeted'' Rydberg states. Such state-selective trapping of Rydberg atoms can be useful in controlled cold Rydberg collisions, cooling Rydberg states, and species-selective trapping and transport of Rydberg atoms in optical lattices. We tabulate wavelengths at which the trapping potential vanishes for the nsnsns, npnpnp, and ndndnd Rydberg states of Na and Rb atoms and discuss advantages of using such optical lattices for state-selective trapping of Rydberg atoms. We also develop exact analytical expressions for the lattice-induced polarizability for the mz=0{m}_{z}=0mz​=0 Rydberg states and derive an accurate formula predicting tune-out wavelengths at which the optical trapping potential becomes invisible to Rydberg atoms in targeted l=0l=0l=0 states.