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Bulletin of the American Physical Society

Probing Floquet State Dynamics of a Strong Field Dressed He Atom Using Attosecond Pulse Trains

Niranjan Shivaram, Henry R. Timmers, Xiao‐Min Tong, Arvinder S. Sandhu

Published Jun 16, 2011• 0 citations
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We present the first measurement of the vectorial response of strongly dressed helium atoms probed by an attosecond pulse train (APT) polarised either parallel or perpendicular to the dressing field polarisation. The transient absorption is probed as a function of delay between the APT and the linearly polarised 800 nm field of peak intensity . The APT spans the photon energy range 16–42 eV, covering the first ionisation energy of helium (24.59 eV). With parallel polarised dressing and probing fields, we observe modulations with periods of one half and one quarter of the dressing field period. When the polarisation of the dressing field is altered from parallel to perpendicular with respect to the APT polarisation we observe a large suppression in the modulation depth of the above ionisation threshold absorption. In addition to this we present the intensity dependence of the harmonic modulation depth as a function of delay between the dressing and probe fields, with dressing field peak intensities ranging from 2 × 10 12 to 2 × 10 14 . We compare our experimental results with a full-dimensional solution of the single-atom time-dependent (TD) Schrödinger equation obtained using the recently developed abinitio TD B-spline ADC method and find good qualitative agreement for the above threshold harmonics.
Using high-order harmonic attosecond pulse trains, we investigate the photoionization dynamics and transient electronic structure of a helium atom in the presence of moderately strong (∼10(12) W cm(-2)) femtosecond laser pulses. We observe quantum interferences between photoexcitation paths from the ground state to different laser-dressed Floquet state components. As the intensity ramps on femtosecond time scales, we observe switching between ionization channels mediated by different atomic resonances. Using precision measurements of ion yields and photoelectron distributions, the quantum phase difference between interfering paths is extracted for each ionization channel and compared with simulations. Our results elucidate photoionization mechanisms in strong fields and open the doors for photoabsorption or photoionization control schemes.