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Bulletin of the American Physical Society

Dynamical effects of Stark-shifted quantum dots strongly coupled to photonic crystal cavities

Kaushik Roy Choudhury, Ranojoy Bose, Edo Waks A

Published Mar 18, 2013• 0 citations
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arXiv:1107.3751•Jul 19, 2011•4 citations
Vacuum Rabi oscillation is a damped oscillation in which energy can transfer between an atomic excitation and a photon when an atom is strongly coupled to a photonic cavity. This process is challenging to be coherently controlled due to the fact that interaction between the atom and the electromagnetic resonator needs to be modulated in a quick manner compared to vacuum Rabi frequency. This control has been achieved at microwave frequencies, but has remained challenging to be implemented in the optical domain. Here we demonstrated coherent control of energy transfer in a semiconductor quantum dot strongly coupled to a photonic crystal molecule by manipulating the vacuum Rabi oscillation of the system. Instead of using a single photonic crystal cavity, we utilized a photonic crystal molecule consisting two coupled photonic crystal defect cavities to obtain both strong quantum dot-cavity coupling and cavityenhanced AC stark shift. In our system the AC stark shift modulates the coupling interaction between the quantum dot and the cavity by shifting the quantum dot resonance, on timescales (picosecond) shorter than the vacuum Rabi period. We demonstrated the ability to transfer excitation between a quantum dot and cavity, and performed coherent control of light-matter states. Our results provides an ultra-fast approach for probing and controlling light-matter interactions in an integrated nanophotonic device, and could pave the way for gigahertz rate synthesis of arbitrary quantum states of light at optical frequencies.
We experimentally investigate the dynamic nonlinear response of a single quantum dot (QD) strongly coupled to a photonic crystal cavity-waveguide structure. The temporal response is measured by pump-probe excitation where a control pulse propagating through the waveguide is used to create an optical Stark shift on the QD, resulting in a large modification of the cavity reflectivity. This optically induced cavity reflectivity modification switches the propagation direction of a detuned signal pulse. Using this device we demonstrate all-optical switching with only 14 attojoules of control pulse energy. The response time of the switch is measured to be up to 8.4 GHz, which is primarily limited by the cavity-QD interaction strength.