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Physics

Sensing Magnetic Fields with a Giant Quantum Wave

József Fortágh, Andreas Günther

Published Mar 27, 2017• 0 citations
Publisher

Abstract

Microscopic imaging of local magnetic fields provides a window into the organizing principles of complex and technologically relevant condensed-matter materials.However, a wide variety of intriguing strongly correlated and topologically nontrivial materials exhibit poorly understood phenomena outside the detection capability of state-of-the-art high-sensitivity high-resolution scanning probe magnetometers.We introduce a quantum-noise-limited scanning probe magnetometer that can operate from room-to-cryogenic temperatures with unprecedented dc-field sensitivity and micron-scale resolution.The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) employs a magnetically levitated atomic Bose-Einstein condensate (BEC), thereby providing immunity to conductive and blackbody radiative heating.The SQCRAMscope has a field sensitivity of 1.4 nT per resolution-limited point (approximately 2 μm) or 6 nT= ffiffiffiffiffiffi Hz p per point at its duty cycle.Compared to point-by-point sensors, the long length of the BEC provides a naturally parallel measurement, allowing one to measure nearly 100 points with an effective field sensitivity of 600 pT= ffiffiffiffiffiffi Hz p for each point during the same time as a point-by-point scanner measures these points sequentially.Moreover, it has a noise floor of 300 pT and provides nearly 2 orders of magnitude improvement in magnetic flux sensitivity (down to 10 -6 Φ 0 = ffiffiffiffiffiffi Hz p ) over previous atomic probe magnetometers capable of scanning near samples.These capabilities are carefully benchmarked by imaging magnetic fields arising from microfabricated wire patterns in a system where samples may be scanned, cryogenically cooled, and easily exchanged.We anticipate the SQCRAMscope will provide charge-transport images at temperatures from room temperature to 4 K in unconventional superconductors and topologically nontrivial materials.

DOI
10.1103/physics.10.30

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Microscopic imaging of local magnetic fields provides a window into the organizing principles of complex and technologically relevant condensed-matter materials.However, a wide variety of intriguing strongly correlated and topologically nontrivial materials exhibit poorly understood phenomena outside the detection capability of state-of-the-art high-sensitivity high-resolution scanning probe magnetometers.We introduce a quantum-noise-limited scanning probe magnetometer that can operate from room-to-cryogenic temperatures with unprecedented dc-field sensitivity and micron-scale resolution.The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) employs a magnetically levitated atomic Bose-Einstein condensate (BEC), thereby providing immunity to conductive and blackbody radiative heating.The SQCRAMscope has a field sensitivity of 1.4 nT per resolution-limited point (approximately 2 μm) or 6 nT= ffiffiffiffiffiffi Hz p per point at its duty cycle.Compared to point-by-point sensors, the long length of the BEC provides a naturally parallel measurement, allowing one to measure nearly 100 points with an effective field sensitivity of 600 pT= ffiffiffiffiffiffi Hz p for each point during the same time as a point-by-point scanner measures these points sequentially.Moreover, it has a noise floor of 300 pT and provides nearly 2 orders of magnitude improvement in magnetic flux sensitivity (down to 10 -6 Φ 0 = ffiffiffiffiffiffi Hz p ) over previous atomic probe magnetometers capable of scanning near samples.These capabilities are carefully benchmarked by imaging magnetic fields arising from microfabricated wire patterns in a system where samples may be scanned, cryogenically cooled, and easily exchanged.We anticipate the SQCRAMscope will provide charge-transport images at temperatures from room temperature to 4 K in unconventional superconductors and topologically nontrivial materials.
The SQCRAMscope is a recently realized Scanning Quantum CRyogenic Atom Microscope that utilizes an atomic Bose-Einstein condensate to measure magnetic fields emanating from solid-state samples. The quantum sensor does so with unprecedented DC sensitivity at micron resolution from room-to-cryogenic temperatures. An additional advantage of the SQCRAMscope is the preservation of optical access to the sample: Magnetometry imaging of, e.g., electron transport may be performed in concert with other imaging techniques. This multimodal imaging capability can be brought to bear with great effect in the study of nematicity in iron-pnictide high-temperature superconductors, where the relationship between electronic and structural symmetry-breaking resulting in a nematic phase is under debate. Here, we combine the SQCRAMscope with an in situ microscope that measures optical birefringence near the surface. This enables simultaneous and spatially resolved detection of both bulk and near-surface manifestations of nematicity via transport and structural deformation channels, respectively. By performing the first local measurement of emergent resistivity anisotropy in iron pnictides, we observe sharp, nearly concurrent transport and structural transitions. More broadly, these measurements demonstrate the SQCRAMscope's ability to reveal important insights into the physics of complex quantum materials.
Microscopic imaging of local magnetic fields provides a window into the inner workings of complex and technologically relevant materials. The authors present an extremely sensitive scanning-probe microscope for imaging charge transport in strongly correlated and topologically nontrivial systems, from ambient down to liquid-helium temperature. This scanning quantum cryogenic atom microscope (SQCRAMscope) will change research spanning disciplines from basic condensed matter physics to the engineering of hybrid quantum systems.
The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) is a quantum sensor in which a quasi-1D quantum gas images electromagnetic fields emitted from a nearby sample. We report improvements to the microscope. Cryogen usage is reduced by replacing the liquid cryostat with a closed-cycle system and modified cold finger, and cryogenic cooling is enhanced by adding a radiation shield. The minimum accessible sample temperature is reduced from 35~K to 5.7~K while maintaining low sample vibrations. A new sample mount is easier to exchange, and quantum gas preparation is streamlined.
We report on the design and performance of a cryogenic (300 mK) near-field scanning microwave microscope. It uses a microwave resonator as the near-field sensor, operating at a frequency of 6 GHz and microwave probing amplitudes down to 100 μV, approaching low enough photon population (N ∼ 1000) of the resonator such that coherent quantum manipulation becomes feasible. The resonator is made out of a miniaturized distributed fractal superconducting circuit that is integrated with the probing tip, micromachined to be compact enough such that it can be mounted directly on a quartz tuning-fork, and used for parallel operation as an atomic force microscope (AFM). The resonator is magnetically coupled to a transmission line for readout, and to achieve enhanced sensitivity we employ a Pound-Drever-Hall measurement scheme to lock to the resonance frequency. We achieve a well localized near-field around the tip such that the microwave resolution is comparable to the AFM resolution, and a capacitive sensitivity down to 6.4 × 10(-20) F/Hz, limited by mechanical noise. We believe that the results presented here are a significant step towards probing quantum systems at the nanoscale using near-field scanning microwave microscopy.
People have been measuring magnetic fields since 200 BC, giving rise to the field of magnetometry. Recently there has been a drive to measure smaller fields with better resolution, resulting in the production of many different types of magnetometers, each with their own unique features. These magnetometers can have a diverse range of applications such as, GNSS free navigation, biomedical sensing, space and weather measurements, and material physics. When designing a magnetomoter there is a trade off between high sensitivity to magnetic fields and high spatial resolution. Currently, there is a unoccupied niche in direct current (DC) magnetometry, that requires a magnetic field sensitivity in the picotesla range and micron scale spatial resolution. Here, I introduce the Bose-Einstein condensate (BEC), which is a macroscopic quantum object, ideal for probing magnetic fields on the nanotesla to picotesla range, with micron scale resolution. This thesis discusses the use of a BEC microscope (BEC-M) to characterise mate- rials with novel applications in nanotechnology by producing 2D current density maps. To produce the atomic probe for microscopy, a BEC in the quasi-1D regime is carefully prepared, requiring an ultra high vacuum (UHV) environment along with custom designed trapping structures, to optically and magnetically confine the atoms. The sensitivity and resolution of the BEC-M makes it an ideal tool for characterising electrical properties of structures on the micron scale such as carbon nanotube (CNT) bundles and biological samples. Current network configuration in samples such as these, can be mapped via a raster scanning procedure. A measurement was made to identify current pathways in CNTs by measuring the atomic distribution of the ultra cold cloud and converting these images to magnetic field and current density maps.
Wide-field imaging of magnetic signals using ensembles of nitrogen-vacancy (NV) centers in diamond has garnered increasing interest due to its combination of micron-scale resolution, millimeter-scale field of view, and compatibility with diverse samples from across the physical and life sciences. Recently, wide-field NV magnetic imaging based on the Ramsey protocol has achieved uniform and enhanced sensitivity compared to conventional measurements. Here, we integrate the Ramsey-based protocol with spin-bath driving to extend the NV spin dephasing time and improve magnetic sensitivity. We also employ a high-speed camera to enable dynamic wide-field magnetic imaging. We benchmark the utility of this quantum diamond microscope (QDM) by imaging magnetic fields produced from a fabricated wire phantom. Over a 270 × 270 μm2 field of view, a median per-pixel magnetic sensitivity of 4.1(1) nT /Hz is realized with a spatial resolution ≲ 10 μm and sub-millisecond temporal resolution. Importantly, the spatial magnetic noise floor can be reduced to the picotesla scale by time-averaging and signal modulation, which enables imaging of a magnetic-field pattern with a peak-to-peak amplitude difference of about 300 pT. Finally, we discuss potential new applications of this dynamic QDM in studying biomineralization and electrically active cells.