The quantum nature of light makes it a basic component for models of quantum measurement and information exchange between disparate quantum modes, pioneered in the field of cavity quantum electrodynamics. The interaction of atomic ensembles with the mode of an optical cavity provides a flexible platform for exploring the coherent interaction of light with diverse macroscopic dynamics, such as collective motion and spin. This dissertation presents experimental results and theoretical models for continuous measurement and control of the center of mass motion and collective spin precession of an atomic ensemble, mediated by coupling to a high-finesse optical cavity. First, the theory of dispersive coupling between the cavity mode and the collective motion and spin of an atomic ensemble is derived, and then a general time-domain formalism is developed for theoretical analysis of multi-mode optodynamical systems. Single-mode optodynamical effects are introduced through experimental demonstrations of measurement and control of the collective atomic spin, providing a close analogy to cavity optomechanics.Next, multiple collective atomic modes are considered within a single cavity, in order to assemble optically mediated interactions within multi-mode optodynamical systems. A demonstration of optodynamical interactions between the center of mass motion of two atomic ensembles is presented, coupled through an optical spring mediated by the cavity mode. Then simultaneous coupling of the center of mass motion and total spin precession of a single ensemble of atoms is described, yielding an experimental realization of a negative-mass instability, facilitated by the novel resource of the spin ensembles inverted state. A theoretical analysis of the negative-mass instability is presented, which indicates the possibility of generating two-mode squeezed states in the absence of excess incoherent noise. Finally, linear state retrodiction from the optodynamical signals is discussed, providing background and supplemental material for a forthcoming manuscript.
We analyze the dynamics of spin-mixing interactions generated by coupling spin-1 atoms to the mode of a high-finesse optical cavity. We show that the dynamics can be understood in terms of generators of the noncompact Lie group SU(1, 1) and introduce a set of SU(1, 1) coherent states which are preserved under Hamiltonian evolution. In terms of these coherent states the resulting dynamics may be interpreted as classical motion on the unit disk. We explicitly compute the trajectories of this classical motion and show that the motion is equivalent to spin-nematic squeezing in the atomic ensemble. Non-uniform coupling between the atomic ensemble and the cavity mode leads to departures from this simple behavior; we introduce a toy model that captures this non-uniformity and solve it exactly.
We realize a spin-orbit interaction between the collective spin precession and center-of-mass motion of a trapped ultracold atomic gas, mediated by spin- and position-dependent dispersive coupling to a driven optical cavity. The collective spin, precessing near its highest-energy state in an applied magnetic field, can be approximated as a negative-mass harmonic oscillator. When the Larmor precession and mechanical motion are nearly resonant, cavity mediated coupling leads to a negative-mass instability, driving exponential growth of a correlated mode of the hybrid system. We observe this growth imprinted on modulations of the cavity field and estimate the full covariance of the resulting two-mode state by observing its transient decay during subsequent free evolution.
We present a cross-cavity system in which steady-state superradiance is achieved using solely collective dissipative dynamics. Two cavities symmetrically couple an ensemble of four-level atoms by driving transitions between two electronic states and two motional states along perpendicular cavity axes. Both cavities operate in the bad-cavity regime: one cavity mediates collective atomic decay, while the other cavity, together with a coherent drive, mediates collective pumping via an off-resonant Raman transition. With this, we find steady-state superradiant states that possess nonclassical properties, such as super-Poissonian photon statistics. The system thus requires a beyond mean-field description, and so we develop an exact master equation simulation technique utilizing strong symmetries of the system's jump operators. Because superradiant decay is accompanied by a momentum impulse along the corresponding cavity axis, the system exhibits substantial hybrid entanglement between the atoms' spin and motional degrees of freedom at steady state. We also demonstrate that heralded measurements of the two cavity outputs prepare a state with significant particle-particle entanglement with prospects for quantum-enhanced acceleration sensing.