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Bulletin of the American Physical Society

Electrically guided continuous supersonic beams of polar molecules from a cryogenic buffer-gas source

Xing Yang Wu, Christian Sommer, Sotir Chervenkov, Andreas Rohlfes, Martin Zeppenfeld, Laurens van Buuren, Gerhard Rempe

Published Jun 5, 2012• 0 citations
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Continuous guided beams of slow and internally cold polar molecules

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We describe the combination of buffer-gas cooling with electrostatic velocity filtering to produce a high-flux continuous guided beam of internally cold and slow polar molecules. In a previous paper (L.D. van Buuren et al., Phys. Rev. Lett., 2009, 102, 033001) we presented results on density and state purity for guided beams of ammonia and formaldehyde using an optimized set-up. Here we describe in more detail the technical aspects of the cryogenic source, its operation, and the optimization experiments that we performed to obtain the best performance. The versatility of the source is demonstrated by the production of guided beams of different molecular species.

arXiv:0812.1923•Faraday Discussions•Jan 1, 2009•44 citations
This thesis reports on the combination of buffer-gas cooling with electric velocity filtering to produce a high-density guided beam of slow and internally cold polar molecules. In the continuous source, warm molecules are first cooled by collisions with a cryogenic helium buffer gas. Cold molecules are then extracted by means of an electric quadrupole guide. For formaldehyde the population of individual rotational states in the guide is monitored by depletion spectroscopy, resulting in single-state populations up to 82 %. This thesis also reports on a technique to produce pulses of slow guided molecules. The pulses exhibit a narrow velocity distribution around a tunable velocity.
We describe the combination of buffer-gas cooling with electrostatic velocity filtering to produce a high-flux continuous guided beam of internally cold and slow polar molecules. In a previous paper (L.D. van Buuren et al., Phys. Rev. Lett., 2009, 102, 033001) we presented results on density and state purity for guided beams of ammonia and formaldehyde using an optimized set-up. Here we describe in more detail the technical aspects of the cryogenic source, its operation, and the optimization experiments that we performed to obtain the best performance. The versatility of the source is demonstrated by the production of guided beams of different molecular species.