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Quantum correlations between single telecom photons and a multimode on-demand solid-state quantum memory

Alessandro Seri, Andreas Lenhard, Daniel Rieländer, Mustafa Gündoğan, Patrick M. Ledingham, Margherita Mazzera, Hugues de Riedmatten

Published May 24, 2017• 21 citations
Publisher

Abstract

Quantum correlations between long-lived quantum memories and telecom photons that can propagate with low loss in optical fibers are an essential resource for the realization of large-scale quantum information networks. Significant progress has been realized in this direction with atomic and solid-state systems. Here, we demonstrate quantum correlations between a telecom photon and a multimode ondemand solid state quantum memory. This is achieved by mapping a correlated single photon onto a spin collective excitation in a Pr 3+ :Y 2 SiO 5 crystal for a controllable time. The stored single photons are generated by cavity-enhanced spontaneous parametric down-conversion and heralded by their partner photons at telecom wavelength. These results represent the first demonstration of a multimode on-demand solid state quantum memory for external quantum states of light. They provide an important resource for quantum repeaters and pave the way for the implementation of quantum information networks with distant solid state quantum nodes.

DOI
10.17863/cam.10279

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Quantum correlations between long-lived quantum memories and telecom photons that can propagate with low loss in optical fibers are an essential resource for the realization of large-scale quantum information networks. Significant progress has been realized in this direction with atomic and solid-state systems. Here, we demonstrate quantum correlations between a telecom photon and a multimode ondemand solid state quantum memory. This is achieved by mapping a correlated single photon onto a spin collective excitation in a Pr 3+ :Y 2 SiO 5 crystal for a controllable time. The stored single photons are generated by cavity-enhanced spontaneous parametric down-conversion and heralded by their partner photons at telecom wavelength. These results represent the first demonstration of a multimode on-demand solid state quantum memory for external quantum states of light. They provide an important resource for quantum repeaters and pave the way for the implementation of quantum information networks with distant solid state quantum nodes.
Quantum correlations between long-lived quantum memories and telecom photons that can propagate with low loss in optical fibers are an essential resource for the realization of large-scale quantum information networks.Significant progress has been realized in this direction with atomic and solid-state systems.Here, we demonstrate quantum correlations between a telecom photon and a multimode ondemand solid state quantum memory.This is achieved by mapping a correlated single photon onto a spin collective excitation in a Pr 3þ ∶Y 2 SiO 5 crystal for a controllable time.The stored single photons are generated by cavity-enhanced spontaneous parametric down-conversion and heralded by their partner photons at telecom wavelength.These results represent the first demonstration of a multimode on-demand solid state quantum memory for external quantum states of light.They provide an important resource for quantum repeaters and pave the way for the implementation of quantum information networks with distant solid state quantum nodes.
Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand readout and multimode operation are additional precious assets that will benefit the communication rate. In this Letter, we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely nondegenerate parametric down-conversion, featuring energy-time entanglement between the telecom-wavelength idler and a visible signal photon. The latter is stored in a Pr^{3+}:Y_{2}SiO_{5} crystal as a spin wave using the full atomic frequency comb scheme. We then recall the stored signal photon and analyze the entanglement using the Franson scheme. We measure conditional fidelities of 92(2)% for excited-state storage, enough to violate a Clauser-Horne-Shimony-Holt inequality, and 77(2)% for spin-wave storage. Taking advantage of the on-demand readout from the spin state, we extend the entanglement storage in the quantum memory for up to 47.7 μs, which could allow for the distribution of entanglement between quantum nodes separated by distances of up to 10 km.
Multiplexed quantum memories increase the entanglement distribution rate in long-distance quantum repeater architectures by harnessing storage in several degrees of freedom. Here, we report on the distribution of light-matter quantum correlations using an array of time-multiplexed solid-state quantum memories. We store telecom-heralded single photons sequentially in up to ten memory cells using the full atomic frequency comb protocol with on-demand read-out in a Pr3+^{3+}3+:Y2_22​SiO5_55​ crystal. Leveraging both spatial and temporal multiplexing, we demonstrate quantum correlations between the telecom photon and up to 60 spatio-temporal modes of the quantum memory array. We then transmit the heralding telecom photon over 39.1 km of deployed optical fiber in the Metropolitan Area of Barcelona. In a realistic scenario where the generation rate is limited by the two-way communication time, we show that up to 15 % of the 393μs393 μs393μs round-trip communication time is filled with communication trials, leading to a 60-fold enhancement in the rate of detected telecom photons correlated with the quantum memory array, compared to a single-mode memory. With increased storage times and efficiencies, our multiplexed quantum memory array will constitute the backbone of a long-distance quantum network, establishing remote entanglement at high rates.
As the reach of quantum technologies extends ever further in communication and information science, a reliable way of transferring quantum information between distant locations becomes ever more crucial. While photons are widely accepted as excellent carriers due to their speed and low decoherence, losses of transmission (in free space or fibre) and the impossibility of cloning quantum information still pose a great challenge. The quantum repeater architecture was suggested as a solution to both problems [1]. In a quantum repeater the information encoded in an input state is transferred to a new one through entanglement swapping, that is then sent on along the channel. In this work we present our advances towards the realisation of a quantum repeater. Our system of choice combines a solid-state quantum memory with a source of photon pairs. The memory is based on a Rare-Earth Doped crystal, where quantum information can be stored in Pr3+ ions as a collective excitation using the Atomic Frequency Comb technique. On demand retrieval of the information is realised by transferring the excitation to a long-lived spin state. Record values of storage times and retrieval efficiencies have been demonstrated in this system [2]. Entangled pairs of single photons are generated by parametric down conversion in a periodically poled crystal placed inside a bow-tie cavity. This allows us to generate narrow band photons pairs, where the signal is spectrally matched to the memory (606nm), while the idler is in the telecom band [3]. Such a configuration allows us to benefit from the high performance of the memory, that also allows for temporal [2] and frequency [4] multimodality, while at the same time overcoming the high optical losses of 606nm photons by pair generation of a telecom photon. The first stepping stone, progress towards which is presented in this work, is the successful demonstration of energy-time entanglement between the telecom idler photon and the signal photon, stored as spin-wave excitation. The entanglement of the original pair is maintained by the memory temporal multimodality. The entanglement analysis will be made through time-bin qubit analysers made of a fibre-based Mach-Zehnder interferometer, for the former, and a solid-state equivalent based on two AFC with different storage times, for the latter [5]. In this direction we have already doubled the efficiency of the AFC storage protocols, that will be beneficial to count rates and signal-to-noise ratio. With respect to [2], we also increased the spectral-matching between the source and the memory [4]. Our experiment will provide an increase in storage time of 3 orders of magnitude with respect to previous demonstrations, as well as introducing for the first time on-demand read-out in a highly multi-mode memory. Demonstration of the successful transfer of quantum information between the signal photon and the long-lived solid-state excitation will open the way to the demonstration of long-distance entanglement between individual nodes in a quantum network.
In this talk, we report on recent progress towards the realization of quantum repeaters based on rare-earth doped crystal quantum memories (QM) and cavity-enhanced SPDC photon-pair sources. We first present our demonstration of on-demand telecom-heralded entanglement between multimode solid-state quantum memories with high rate and fully adjustable recall time. Then, we show how we successfully established long-distance non-classical correlations between a telecom photon and a QM in a field-deployed experiment in the city of Barcelona.
Long-lived storage of single photons under the form of atomic excitations is at the foundation of long-distance entanglement distribution in quantum networks. To mitigate decoherence effects induced by the environment, rephasing of the hyperfine coherences using microwave pulses have been implemented in a variety of single-emitter and ensemble-based solid-state systems. However, the demonstration of storage of single photons in an absorptive quantum memory including such spin rephasing mechanism remains elusive. In this work, we show non-classical storage of telecom-heralded single photons in a Pr3+^{3+}3+:Y2_22​SiO5_55​ rare-earth ion doped crystal quantum memory using the atomic frequency comb (AFC) spin-wave protocol combined with a XY4 spin rephasing sequence. Long-lived AFC photon echoes are first observed in the classical regime for storage times of up to approximately 3 ms. We then demonstrate non-classical correlations between heralding photons and stored signal photons generated by a cavity-enhanced parametric photon-pair source for storage times of up to 180 μμμs and with measured cross-correlation values as high as 4.6(4). Together with the capacity of Pr3+^{3+}3+:Y2_22​SiO5_55​ QMs to support highly efficient and multiplexed storage, this result represents a significant step towards scalable long-distance quantum repeater links.