I describe the theory and construction of a new bichromatic optical superlattice to study the pairing and thermodynamics of spin $\\frac{1}{2}$-up and spin $\\frac{1}{2}$-down atoms in periodic double well potentials. Our bichromatic lattice contains $\\lambda_1=1064$ nm and $\\lambda_2=532$ nm standing wave lattices. With tunable depth and relative phase between the two lattices, periodic double well potentials of arbitrary local symmetry can be constructed. I present the first systematic experimental study of a two-component ultracold $^6$Li atomic Fermi gas in a single color 1064 nm lattice, which is continuously tuned from 2D to quasi-2D. A system is 2D if it is free to move in two dimensions while tightly confined in the third direction, such that only the ground state is occupied. Conversely, it is quasi-2D if higher states in the tightly confined direction are also occupied. I describe both radio frequency spectra and radial cloud profiles measured under identical conditions for each regime. Our results confirm predictions that the mean-field theory is not valid throughout the 2D to quasi-2D dimensional crossover. We also clarify that there is no transition between 2D and quasi-2D systems. I also present the first study of pairing in a periodic double well potential. A Green's function method is developed to compute the pairing energies in the lattice. Although further understanding of the results are needed, I provide some preliminary rf spectra measurements supporting the theoretical approach and implying the existence of two types of pairing.
I describe the theory and construction of a new bichromatic optical superlattice to study the pairing and thermodynamics of spin frac12-up and spin frac12-down atoms in periodic double well potentials. Our bichromatic lattice contains lambda1=1064 nm and lambda2=532 nm standing wave lattices. With tunable depth and relative phase between the two lattices, periodic double well potentials of arbitrary local symmetry can be constructed. I present the first systematic experimental study of a two-component ultracold 6Li atomic Fermi gas in a single color 1064 nm lattice, which is continuously tuned from 2D to quasi-2D. A system is 2D if it is free to move in two dimensions while tightly confined in the third direction, such that only the ground state is occupied. Conversely, it is quasi-2D if higher states in the tightly confined direction are also occupied. I describe both radio frequency spectra and radial cloud profiles measured under identical conditions for each regime. Our results confirm predictions that the mean-field theory is not valid throughout the 2D to quasi-2D dimensional crossover. We also clarify that there is no transition between 2D and quasi-2D systems. I also present the first study of pairing in a periodic double well potential. A Green's function method is developed to compute the pairing energies in the lattice. Although further understanding of the results are needed, I provide some preliminary rf spectra measurements supporting the theoretical approach and implying the existence of two types of pairing.
We study the pairing of fermions in a one-dimensional lattice of tunable double-well potentials using radio-frequency spectroscopy. The spectra reveal the coexistence of two types of atom pairs with different symmetries. Our measurements are in excellent quantitative agreement with a theoretical model, obtained by extending the Green's function method of Orso et al. [Phys. Rev. Lett. 95, 060402 (2005)PRLTAO0031-900710.1103/PhysRevLett.95.060402] to a bichromatic 1D lattice with nonzero harmonic radial confinement. The predicted spectra comprise hundreds of discrete transitions, with symmetry-dependent initial state populations and transition strengths. Our work provides an understanding of the elementary pairing states in a superlattice, paving the way for new studies of strongly interacting many-body systems.
Ultracold atoms in optical lattices provide a versatile platform for studying many-body physics in a defect-free system with tunable parameters. For the analog quantum simulation of the Fermi-Hubbard model, fermionic atoms take on the role of the valence electrons and optical lattices provide the periodic potential in place of the solid-state crystal. The dynamics in the system are described by the tunneling amplitude t between neighboring lattice sites and the interaction energy U of two particles occupying the same lattice site. With the depth of the optical lattices and an external magnetic field, both parameters can be tuned to access a wide range of regimes. Two superimposed lattices with different lattice periods form an optical superlattice, where the most common configuration is a bichromatic superlattice with lattice periods different by a factor of two. Depending on the lattice depths and the relative phase of the lattices, the bichromatic superlattice potential ranges from an array of weakly-coupled double wells to a continuous lattice potential with a staggered energy offset. We developed a calibration technique for measuring the depth of an optical lattice with local resolution. The band structure of the optical lattice is probed by modulating the lattice depth and exciting the atoms to higher bands. However, compared to resolving the band occupations in a time-of-flight measurement, we further excite the atoms to an untrapped band to deplete the optical lattice along equipotential lines where the modulation frequency is resonant with the local band transitions. From the profile of the lattice depth, we obtain the calibration factor for the power regulation, the waist of the underlying lattice beams and the position of the lattice axis. This technique combines several calibration measurements, thereby reducing the measurement time and enabling an automation of the lattice alignment. For the bichromatic superlattice we realized an active stabilization of the superlattice phase that enables long-term measurements with a precise control over the superlattice phase. The instability of the superlattice phase is a result of the different refractive indices for the two lattices in air and the optical elements along the optical path. Using environmental sensors, we monitor the temperature, the pressure, and the relative humidity to apply the expected correction to the superlattice phase. The stabilized superlattice phase enabled the investigation of Floquet-driven double wells by modulating the energy offset through the superlattice phase. We used a near-resonant driving frequency with respect to the interaction energy to enhance the pair-tunneling amplitude in doubly-occupied double wells compared to static double wells and compared to the tunneling amplitude in singly-occupied double wells.
This thesis presents quantum simulation of strongly-correlated systems beyond standard Hubbard models, using ultracold fermionic potassium atoms in both static and periodically-driven optical superlattices. For this study, we utilize a three-dimensional optical lattice setup, controlling particle interactions via magnetic Feshbach resonances and tunneling between lattice sites through optical lattice intensity. High-resolution absorption imaging combined with radio-frequency spectroscopy distinguishes between singly and doubly occupied sites. To enhance our systems capabilities beyond the standard Hubbard model, we extend the apparatus with an in-plane optical superlattice, creating a bi-chromatic structure by superposition of two optical lattices with commensurate lattice spacings. Using a phase locked loop with an environmental feed forward, we create an excellent phase stability of the superlattice exceeding 3 mrad. This precision allows us to explore both static and periodically-driven one-dimensional tight-binding models with strong interactions. We characterize the static superlattice through radio-frequency spectroscopy and Rabi oscillations, and validate the experimental data against theoretical calculations. In a tilted superlattice configuration, we successfully prepare and detect repulsively bound atom pairs, representing a highly excited eigenstate of the system. Furthermore, we demonstrate control over pair tunneling dynamics in a double-well potential using Floquet engineering, employing a low-noise periodic modulation of the optical superlattice tilt. Using an adiabatic band mapping technique, we directly observe the tunneling dynamics in the driven superlattice. We realize dynamic localization in quarter-filled wells and density-assisted tunneling up to the third harmonic order in half-filled wells. We observe a crossover from density-assited tunneling to dominant pair tunneling by tuning the effective interactions. Remarkably, the pair tunneling is not only enhanced relative to the suppressed single-particle tunneling but also exceeds the superexchange rate of a static double-well by more than a factor of two. This opens the possibility to study many-body systems with dominant pair tunneling, that extend beyond the standard Hubbard model.
Abstract Atomic Fermi gases have been an ideal platform for simulating conventional and engineering exotic physical systems owing to their multiple tunable control parameters. Here we investigate the effects of mixed dimensionality on the superfluid and pairing phenomena of a two-component ultracold atomic Fermi gas with a short-range pairing interaction, while one component is confined on a one-dimensional (1D) optical lattice whereas the other is in a homogeneous 3D continuum. We study the phase diagram and the pseudogap phenomena throughout the entire BCS-BEC crossover, using a pairing fluctuation theory. We find that the effective dimensionality of the non-interacting lattice component can evolve from quasi-3D to quasi-1D, leading to strong Fermi surface mismatch. Upon pairing, the system becomes effectively quasi-two dimensional in the BEC regime. The behavior of T c bears similarity to that of a regular 3D population imbalanced Fermi gas, but with a more drastic departure from the regular 3D balanced case, featuring both intermediate temperature superfluidity and possible pair density wave ground state. Unlike a simple 1D optical lattice case, T c in the mixed dimensions has a constant BEC asymptote.
The superfluidity and pairing phenomena in ultracold atomic Fermi gases have been of great interest in recent years, with multiple tunable parameters. Here we study the BCS-BEC crossover behavior of balanced two-component Fermi gases in a one-dimensional optical lattice, which is distinct from the simple three-dimensional (3D) continuum and a fully 3D lattice often found in a condensed matter system. We use a pairing fluctuation theory which includes self-consistent feedback effects at finite temperatures and find widespread pseudogap phenomena beyond the BCS regime. As a consequence of the lattice periodicity, the superfluid transition temperature Tc decreases with pairing strength in the BEC regime, where it approaches asymptotically ${T}_{\mathrm{c}}=\ensuremath{\pi}an/2m$, with a being the s-wave scattering length, and n (m) the fermion density (mass). In addition, the quasi-two dimensionality leads to fast-growing (absolute value of the) fermionic chemical potential $\ensuremath{\mu}$ and pairing gap $\mathrm{\ensuremath{\Delta}}$, which depends exponentially on the ratio d/a. Importantly, Tc at unitarity increases with the lattice constant d and hopping integral t. The effect of the van Hove singularity on Tc is identified. The superfluid density exhibits T3/2 power laws at low T, away from the extreme BCS limit. These predictions can be tested in future experiments.
Ultracold atoms have become an essential tool in studying condensed matter phenomena. The advantage of atomic physics experiments is that they provide an easily tunable system. This experiment uses the lowest two ground state hyperfine levels of fermionic lithium. Having two different states creates a pseudo-spin-1/2 system and allows us to emulate electronic systems, such as superconductors and crystal lattices. In our experiment, we can control the ratio between these two states resulting in either a spin-balanced or a spin-imbalanced gas. Imposing an imbalance is analogous to applying a magnetic field to a superconductor which causes the electrons in the material to align to the field (thus breaking the electron pairs which cause superconductivity). This motivates us to understand the phases created when a spin-imbalance is created and the effect of changing the atomic interactions. In a 3D system, we find where superfluidity is suppressed throughout the BEC to BCS crossover. Using phase separation as a guide, we probe the dimensional crossover between 1D and 3D. The phase separation in 1D is inverted from that in 3D, which provides a unique characteristic to distinguish between the dimensions. By varying the tunneling between tubes and the atomic interactions in a 2D optical lattice, we control whether the system is 1D, 3D, or in between. Using the properties of a 3D gas as a guide, we directly observe when the gas has crossed over from being dominated by 1D-like behavior to 3D. In this way, we have found a universal value for the dimensional crossover. The 1D-3D crossover paves the way to search for the exotic FFLO (Fulde-Ferrell-Larkin-Ovchinnikov) superconductor. While most superconductors do not coexist with magnetism, the FFLO phase requires large magnetic fields to support its pairing mechanism. Additionally, this phase is more likely to be found in lower dimensional systems. However, at low dimensions, the effect of temperature fluctuations on the phase is destabilizing, but these temperature effects are reduced with higher dimensionality. Thus, the quasi-1D regime is the optimal region of parameter space to find this phase. The search for direct evidence of FFLO continues in this regime.