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Journal of Physics Conference Series

Double-resonance spectroscopy in Rubidium vapour-cells for high performance and miniature atomic clocks

Mohammadreza Gharavipour, C. Affolderbach, Songbai Kang, G. Mileti

Published Jan 1, 2017• 2 citations
Publisher

Abstract

We report our studies on using microwave-optical double-resonance (DR) spectroscopy for a high-performance Rb vapour-cell atomic clock in view of future industrial applications.The clock physics package is very compact with a total volume of only 0.8 dm 3 .It contains a recently in-house developed magnetron-type cavity and a Rb vapour cell.A homedmade frequency-stabilized laser system with an integrated acousto-optical-modulator (AOM)for switching and controlling the light output power-is used as an optical source in a laser head (LH).The LH has the overall volume of 2.5 dm 3 including the laser diode, optical elements, AOM and electronics.In our Rb atomic clock two schemes of continuous-wave DR and Ramsey-DR schemes are used, where the latter one strongly reduces the light-shift effect by separation of the interaction of light and microwave.Applications of the DR clock approach to more radically miniaturized atomic clocks are discussed.

DOI
10.1088/1742-6596/793/1/012007

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We report our studies on using microwave-optical double-resonance (DR) spectroscopy for a high-performance Rb vapour-cell atomic clock in view of future industrial applications.The clock physics package is very compact with a total volume of only 0.8 dm 3 .It contains a recently in-house developed magnetron-type cavity and a Rb vapour cell.A homedmade frequency-stabilized laser system with an integrated acousto-optical-modulator (AOM)for switching and controlling the light output power-is used as an optical source in a laser head (LH).The LH has the overall volume of 2.5 dm 3 including the laser diode, optical elements, AOM and electronics.In our Rb atomic clock two schemes of continuous-wave DR and Ramsey-DR schemes are used, where the latter one strongly reduces the light-shift effect by separation of the interaction of light and microwave.Applications of the DR clock approach to more radically miniaturized atomic clocks are discussed.
We report our investigations on a compact high-performance rubidium (Rb) vapourcell clock based on microwave-optical double-resonance (DR).These studies are done in both DR continuous-wave (CW) and Ramsey schemes using the same Physics Package (PP), with the same Rb vapour cell and a magnetron-type cavity with only 45 cm 3 external volume.In the CW-DR scheme, we demonstrate a DR signal with a contrast of 26% and a linewidth of 334 Hz; in Ramsey-DR mode Ramsey signals with higher contrast up to 35% and a linewidth of 160 Hz have been demonstrated.Short-term stabilities of 1.4×10 -13 τ -1/2 and 2.4×10 -13 τ -1/2 are measured for CW-DR and Ramsey-DR schemes, respectively.In the Ramsey-DR operation, thanks to the separation of light and microwave interactions in time, the light-shift effect has been suppressed which allows improving the long-term clock stability as compared to CW-DR operation.Implementations in miniature atomic clocks are considered. IntroductionSince the first invention of lamp-pumped rubidium (Rb) clocks in the 1960's [1,2], the demand for a stable, reliable, and compact Rb frequency standard with low power consumption has been growing, for various applications fields such as industry, telecommunication, navigation, space applications (e.g.GPS [3], GALILEO [4] and COMPASS [5]).Recently, thanks to the semiconductor laser technology, laser-pumped Rb clocks have been considered in several studies, for their better optical pumping efficiency results in short-term frequency stabilities at least one order of magnitude better than their lamp-pumped counterparts [6][7][8][9].This opened up also several new schemes for vapour-cell atomic clocks, such as the continuous-wave (CW) Rb clock [9], coherent population trapping (CPT) Cs clock [10] and pulsed optical pumping (POP) Rb clock [11].In this paper we report our studies on high-performance Rb frequency standards based on the laser-microwave double-resonance (DR) scheme, using both CW and Ramsey interrogation.Both CW-DR and Ramsey-DR schemes require two resonant electromagnetic fields of light and microwave.In the case of CW-DR, the laser optically pumps the vapour of the Rb atoms by creating a polarization of the atomic ground-state; simultaneously the microwave field, generated from a quartz oscillator and is near-resonant with the 87 Rb hyperfine clock transition (energy levels 5 2 S 1/2 │F g =1, m F =0˃ ↔│F g =2, m F =0˃), is applied.The opacity of the Rb vapour to the transmitted light signal as a function of microwave frequency is a measure of the atomic ground state polarization known as CW-DR signal [9].In CW-DR, the steps of optical pumping, microwave interrogation and optical detection are applied simultaneously (figure 1(b)).In the case of Ramsey-DR, these three sequences are separated in time, see figure 1(c): first, during optical pumping a strong laser pulse creates a significant atom population imbalance between
We present first results on a laser-pumped, double resonance (DR) Rubidium atomic clock, based on micro-fabricated Rb vapour cells. The study aims towards a miniature atomic clock based on DR, using a low-power laser as pump light source and a miniaturized microwave coupling structure (that will replace the bulky microwave cavity employed in today's much bigger Rb clocks). Good signal amplitude, low background light level, and no need for GHz laser modulation are among the advantages of this approach.
This thesis presents experimental studies on continuous-wave (CW) laser-microwave double-resonance (DR) spectroscopy and metrology in rubidium (87Rb) vapor cells in view of new high-performance, compact Rb-cell atomic clocks. The Rb vapor cell is confined inside a magnetron-type cavity microwave resonator (MWR). The CW DR spectroscopy involves two resonant electromagnetic fields that are operated simultaneously to interrogate the atoms - the optical field to polarize the atoms by optical pumping, and the microwave field to drive the ground-state hyperfine clock transition that serves as an atomic frequency reference. Details on characterization of compact laser heads and microwave synthesizers used in this work are presented. The vapor cell standards are useful in our everyday lives for applications ranging from telecommunications, navigation, metrology etc. In view of improving the performances of the Rb cell standards, two different clock approaches were studied in detail: The first one is on use of vapor cells (1.4 cm3) whose inner walls are coated with anti-relaxation material. A first ever wall-coated cell clock was demonstrated with good short-term frequency stability. The medium- to long-term stability was found to be limited by the temperature coefficient (TC) of the coating material itself. This work gave the insight to important features to be considered in future anti-relaxation coating materials for atomic standards. The second novel approach involves using a bigger cell (12 cm3) within a newly developed, improved MWR towards a high-performance atomic standard. Adopting a larger cell gives a higher atomic Q-factor signal that improves the short-term clock stability. In this approach, the cell was filled with 87Rb and buffer gases. With this clock, we demonstrate the state-of-the-art short-term stability of <1.4×10−13 τ−1/2. Metrological quantitative measurements on parameters influencing the medium- to long-term stability were studied in view of next generation satellite navigation systems that demand a stability level of <1×10−14 at 10 4 s (equivalent to <1 ns/day). The potential of short-term stability and understanding of the limiting factors on medium- to long-term time scales demonstrated in this study pave the way for future work towards the commercialization of high-performance Rb atomic clocks for a variety of applications.
This thesis presents experimental studies on continuous-wave (CW) laser-microwave double-resonance (DR) spectroscopy and metrology in rubidium (87Rb) vapor cells in view of new high-performance, compact Rb-cell atomic clocks. The Rb vapor cell is confined inside a magnetron-type cavity microwave resonator (MWR). The CW DR spectroscopy involves two resonant electromagnetic fields that are operated simultaneously to interrogate the atoms - the optical field to polarize the atoms by optical pumping, and the microwave field to drive the ground-state hyperfine clock transition that serves as an atomic frequency reference. Details on characterization of compact laser heads and microwave synthesizers used in this work are presented. The vapor cell standards are useful in our everyday lives for applications ranging from telecommunications, navigation, metrology etc. In view of improving the performances of the Rb cell standards, two different clock approaches were studied in detail: The first one is on use of vapor cells (1.4 cm3) whose inner walls are coated with anti-relaxation material. A first ever wall-coated cell clock was demonstrated with good short-term frequency stability. The medium- to long-term stability was found to be limited by the temperature coefficient (TC) of the coating material itself. This work gave the insight to important features to be considered in future anti-relaxation coating materials for atomic standards. The second novel approach involves using a bigger cell (12 cm3) within a newly developed, improved MWR towards a high-performance atomic standard. Adopting a larger cell gives a higher atomic Q-factor signal that improves the short-term clock stability. In this approach, the cell was filled with 87Rb and buffer gases. With this clock, we demonstrate the state-of-the-art short-term stability of <1.4×10−13 τ−1/2. Metrological quantitative measurements on parameters influencing the medium- to long-term stability were studied in view of next generation satellite navigation systems that demand a stability level of <1×10−14 at 10 4 s (equivalent to <1 ns/day). The potential of short-term stability and understanding of the limiting factors on medium- to long-term time scales demonstrated in this study pave the way for future work towards the commercialization of high-performance Rb atomic clocks for a variety of applications.
We present the development and complete spectral characterization of our compact and frequency-stabilized laser heads, to be used for rubidium atomic clocks and basic spectroscopy. The light source is a Distributed Feed-Back (DFB) laser diode emitting at 780 nm or 795 nm. The laser frequency is stabilized on a sub-Doppler absorption peak of the 87Rb atom, obtained from an evacuated rubidium cell. These laser heads, including the electronics for the light signals detection, have an overall volume of 0.63 liters. We also present a variant of the laser head into which is integrated an Acousto-Optical Modulator (AOM) that precisely detunes the laser frequency in order to minimize the AC Stark shift in Rb atomic clocks.
We demonstrate and study a microcell microwave atomic clock based on optical-microwave double resonance (DR) interrogation operated in a pulsed Ramsey scheme, called the \ensuremath{\mu}POP clock, based on a microfabricated Rb vapor cell and a micro-loop-gap microwave resonator. For the mm-scale dimensions of this cell, the population and coherence relaxation rates of the Rb clock transition are on the order of 4--5 kHz, which puts constraints on the useful Ramsey times and overall pulse sequence in view of optimized clock performance. Our proof-of-principle demonstration of the \ensuremath{\mu}POP clock shows that the pulsed DR approach is nevertheless feasible and results in a short-term clock stability of 1 \ifmmode\times\else\texttimes\fi{} ${10}^{\ensuremath{-}11}$ \ensuremath{\tau}${}^{\ensuremath{-}1/2}$ and reaching the \ensuremath{\le}2 \ifmmode\times\else\texttimes\fi{} ${10}^{\ensuremath{-}12}$ level at timescales of 1000 s to one day. The short-term instability budget established for the \ensuremath{\mu}POP clock shows that the main limitation to the short-term stability arises from the detection noise. Thanks to the pulsed Ramsey scheme, light-shift effects are strongly reduced in the \ensuremath{\mu}POP clock, which opens perspectives for further improvements of long-term clock stability, in view of future generations of miniature vapor-cell clocks with enhanced performances based on the DR scheme.