A source of spin-polarized electrons based on a laser-pumped flowing helium afterglow is described. He(23S) atoms contained in the afterglow are optically pumped using circularly polarized 1.08-μm (23S→23P) radiation provided by a NaF (F2+)* color-center laser. Spin angular momentum conservation in subsequent chemi-ionization reactions with CO2 produces polarized electrons that are extracted from the afterglow. At low currents, ≲1 μA, polarizations of ∼70%–80% are achieved. At higher currents the polarization decreases, falling to ∼40% at 50 μA. The spin polarization can be simply reversed (P→−P) and the source is suitable for use in the majority of low-energy spin-dependent scattering experiments proposed to date.
The polarization of helium (2
3S1) metastable atoms saturates at 50% when the ensemble is optically pumped with the
D0 (2
3${\mathit{S}}_{1--}$2
3P0) transition. We have obtained polarizations approaching 100% with a simple, straightforward modification to the conventional experimental arrangement. The addition of a small amount of \ensuremath{\pi}-polarized
D0 light incident on the cell perpendicular to the defining field direction doubles the polarization produced by circularly polarized ${\mathrm{\ensuremath{\sigma}}}^{+}$ light along the field direction. A simple rate-equation model illustrates the enhancement.