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Electron Spin Polarization in Optically Pumped HELIUM-4.

M. V. McCusker

Published Jan 1, 1969• 0 citations
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Enhanced polarization of electron spins in He4 by simultaneous optical pumping with circularly and linearly polarized resonance radiation

L. D. Schearer, Padetha Tin

The polarization of helium (2 $^{3}$${\mathit{S}}_{1}$) metastable atoms saturates at 50% when the ensemble is optically pumped with the ${\mathit{D}}_{0}$ (2 $^{3}$${\mathit{S}}_{1--}$2 $^{3}$${\mathit{P}}_{0}$) transition. We have obtained polarizations approaching 100% with a simple, straightforward modification to the conventional experimental arrangement. The addition of a small amount of \ensuremath{\pi}-polarized ${\mathit{D}}_{0}$ light incident on the cell perpendicular to the defining field direction doubles the polarization produced by circularly polarized ${\mathrm{\ensuremath{\sigma}}}^{+}$ light along the field direction. A simple rate-equation model illustrates the enhancement.

Physical Review A•Oct 1, 1990•5 citations
A source of spin-polarized electrons based on a laser-pumped flowing helium afterglow is described. He(23S) atoms contained in the afterglow are optically pumped using circularly polarized 1.08-μm (23S→23P) radiation provided by a NaF (F2+)* color-center laser. Spin angular momentum conservation in subsequent chemi-ionization reactions with CO2 produces polarized electrons that are extracted from the afterglow. At low currents, ≲1 μA, polarizations of ∼70%–80% are achieved. At higher currents the polarization decreases, falling to ∼40% at 50 μA. The spin polarization can be simply reversed (P→−P) and the source is suitable for use in the majority of low-energy spin-dependent scattering experiments proposed to date.
The polarization of helium (2 3^{3}3S1{\mathit{S}}_{1}S1​) metastable atoms saturates at 50% when the ensemble is optically pumped with the D0{\mathit{D}}_{0}D0​ (2 3^{3}3${\mathit{S}}_{1--}$2 3^{3}3P0{\mathit{P}}_{0}P0​) transition. We have obtained polarizations approaching 100% with a simple, straightforward modification to the conventional experimental arrangement. The addition of a small amount of \ensuremath{\pi}-polarized D0{\mathit{D}}_{0}D0​ light incident on the cell perpendicular to the defining field direction doubles the polarization produced by circularly polarized ${\mathrm{\ensuremath{\sigma}}}^{+}$ light along the field direction. A simple rate-equation model illustrates the enhancement.