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Journal of Modern Optics

Intrinsic optical bistability in doped polymer

H. Soufi, Hamid Pashaei Adl, M.H. Majles Ara, Dariush Jafari

Published Feb 7, 2017• 3 citations
Publisher

Abstract

One of the most interesting and applicable effects of nonlinear optics is optical bistability. This phenomenon is exhibited by certain resonant optical structures where it is possible to have two stable steady transmission states for the device, depending on the history of the input. Such a bistable device may be useful for optical computing elements as a result of its memory characteristics. Optical bistability behaviour is usually observed by inserting a nonlinear matter inside a Fabry–Perot interferometer. But in this study, it was shown that this can be achieved without the application of any optical resonator. Two laser beams were used to interact with the photorefractive media (doped PMMA polymer) which resulted in the bistability of the intensity of transmitted wave. Feedback was provided by a periodic grating created in the photorefractive polymer PMMA.

DOI
10.1080/09500340.2017.1288831

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One of the most interesting and applicable effects of nonlinear optics is optical bistability. This phenomenon is exhibited by certain resonant optical structures where it is possible to have two stable steady transmission states for the device, depending on the history of the input. Such a bistable device may be useful for optical computing elements as a result of its memory characteristics. Optical bistability behaviour is usually observed by inserting a nonlinear matter inside a Fabry–Perot interferometer. But in this study, it was shown that this can be achieved without the application of any optical resonator. Two laser beams were used to interact with the photorefractive media (doped PMMA polymer) which resulted in the bistability of the intensity of transmitted wave. Feedback was provided by a periodic grating created in the photorefractive polymer PMMA.
It is known that two-wave coupling in photorefractive crystal may result in an intensity-dependent phase shift as well as energy transfer between the two waves without phase crosstalk. In a sense, this kind of phase shift is similar to the intensity-dependent refractive-index effects in Kerr media. Consequently, optical bistability can be established in an optical cavity with a photorefractive crystal. We formulate the model and get the expected bistable transmission with numerical simulations. Several cases, including that of the codirectional coupling and the contradirectional coupling, are considered. The effects of the photorefractive crystal’s distribution absorption and the spatial phase shift between the index grating and the light interference pattern in the crystal on the nonlinear transmission characteristics have also been studied. It is interesting to note that the output of the pumping wave is dependent on the cavity intensity and thus shows bistable behavior with respect to the cavity input as well.
Optical bistability and switching are of great interest in the rapidly and developing field of photonics. Devices that display this behavior could potentially play a major role in the development of optical communication systems and computing. In this article we present experimental results concerning the optical bistability in ferroelectric of photorefractive BaTiO3 crystal. Two laser beams were used to interact with the photorefractive crystal which resulted in the bistability of the intensity of transmitted wave. This was achieved without the application of any optical resonator. High contrast optical bistability is found experimentally in the pump-ratio dependence of the output intensity.
Optical bistability is the quantum optical realization of a first order phase transition far from equilibrium. A resonant nonlinear optical response of it-electron excitations in low dimensional structures provides the nonlinearity essential to the onset of bistability. Saturable absorption studies of glassy polymer films consisting of quasi two-dimensional conjugated disc-like structures of silicon naphthalocyanine demonstrate that on-resonance the system behaves as an optical Bloch system with an intensity dependent refractive index n2 of 1x10-4 cm2/kW in the wavelength range of standard laser diodes. Based on this result, electronic absorptive optical bistability is observed on a nanosecond time scale in a nonlinear Fabry-Perot interferometer employing the saturably absorbing naphthalocyanine film as the nonlinear optical medium.
A theoretical demonstration of optical bistability in periodic layered media, particularly in long-period GaAs/AlAs superlattices is presented. The proposed structure consists of a periodic multilayer system, as opposed to previously demonstrated nonlinear bistable devices which employed Fabry-Perot etalons. The optical resonance effect which is essential for bistable devices is, in this case, induced by a refractive index modulation. The nonlinear active medium is distributed in the whole structure rather than placed between the two mirrors of a Fabry-Perot cavity. It is shown by a complete calculation of wave propagation in the periodic nonlinear medium that a multiple valued feature appears in the structure's nonlinear reflectivity spectrum. The input/output characteristics of the structure exhibit bistable hysteresis similar to that of a nonlinear Fabry-Perot etalon.>