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Beyond photon pairs

S. Cigdem Yorulmaz

Published Jun 10, 2014• 0 citations
OpenAlex

Abstract

In this thesis we explore spatial quantum correlations of high-dimensional multi-photon states. These states are produced using the process of parametric down-conversion and are experimentally explored by measuring correlations with only two detectors. Compared to earlier investigations of multi-photon states, the correlations in this thesis are created in the spatial domain instead of the temporal domain. This has a distinct experimental advantage because it is much easier to measure the emission direction compared to a measurement of the arrival time of the photons.

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In this thesis we explore spatial quantum correlations of high-dimensional multi-photon states. These states are produced using the process of parametric down-conversion and are experimentally explored by measuring correlations with only two detectors. Compared to earlier investigations of multi-photon states, the correlations in this thesis are created in the spatial domain instead of the temporal domain. This has a distinct experimental advantage because it is much easier to measure the emission direction compared to a measurement of the arrival time of the photons.
use of any of the information contained in it must acknowledge this thesis as the source of the quotation or information. This thesis investigates the measurement of spatial correlations of photon pairs gener-ated through spontaneous parametric down-conversion with single-photon sensitive multi-pixel detectors. A custom designed and fabricated 8×1 fibre array detector for time to position multi-plexing was characterised. This detector was then commissioned in an experiment measuring the spatial correlations of photon pairs in position, momentum and in-termediate bases. The fibre array measured eight positions simultaneously with one Single-Photon Avalanche Diode, which led to an eight-fold increase in the data ac-quisition rate compared to traditional experiments, where a single SPAD was scanned across the detection plane. To capture all of the emitted light, an electron-multiplying CCD (EMCCD) camera was used. The spatial correlations were measured for the first time in momentum and pos-
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
The entangled photon pairs (biphotons) produced from parametric down-conversion (PDC) in a χ(2)crystal are the key element for several quantum information and communication schemes. Recent theoretical investigations [1–2] have revealed the peculiar structure of the biphotonic correlation characterizing the entanglement of twin beams in the space-time domain. The biphotonic correlation in type I PDC is characterized in the near field by a X-shaped geometry, which turns out to be non-factorable in space and time, offering thus the relevant possibility of manipulating the temporal bandwidth of biphoton entanglement by acting on their spatial degrees of freedom. The name “X-entanglement” was coined to describe this geometry [1]. An other key feature which emerged is the extreme spatial and temporal localization of the biphotonic correlation, on the micrometer and femtosecond range, respectively.
Non-classical states of light are of fundamental importance for emerging quantum technologies. All optics experiments producing multi-qubit entangled states have until now relied on outcome post-selection, a procedure where only the measurement results corresponding to the desired state are considered. This method severely limits the usefulness of the resulting entangled states. fiere, we show the direct production of polarization- entangled photon triplets by cascading two entangled down-conversion processes[1]. First, a Sagnac source [2] produces non-degenerate entangled photon pairs at 776 nm and 842 nm in a Bell state. The 776 nm photon is sent through a polarizing Mach-Zehnder interferometer with a down-conversion crystal in each arm. If it is down-converted, a photon pair is created in modes 2 and 3 with a polarization state depending on the pump photon. The quantum stete describing the photon triplets is:
We review recent theoretical and experimental works where are proposed and demonstrated how to use photon pairs created by spontaneous parametric down-conversion to generate entangled states of D-dimensional quantum systems, or qudits. This is the first demonstration of high-dimensional entanglement based on the intrinsic transverse momentum entanglement of the type-II down-converted photons. The qudit space is defined by an aperture made up of an opaque screen with D slits (paths), placed in the arms of the twin photons. By manipulating the pump beam profile we can prepare different entangled states of these possible paths. We focus our attention on an important case for applications in quantum information: the maximally entangled states. Experimental results for qudits with D=4 and D=8 are shown and measuring a two-photon conditional interference, we also demonstrate the nonclassical character of the correlations.
We demonstrate coincidence measurements of spatially entangled photons by means of a multi-pixel based detection array. The sensor, originally developed for positron emission tomography applications, is a fully digital 8×16 silicon photomultiplier array allowing not only photon counting but also per-pixel time stamping of the arrived photons with an effective resolution of 265 ps. Together with a frame rate of 500 kfps, this property exceeds the capabilities of conventional charge-coupled device cameras which have become of growing interest for the detection of transversely correlated photon pairs. The sensor is used to measure a second-order correlation function for various non-collinear configurations of entangled photons generated by spontaneous parametric down-conversion. The experimental results are compared to theory.