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Physical Review A

Neutron interferometer crystallographic imperfections and gravitationally induced quantum interference measurements

B. Heacock, M. Arif, Robert W. Haun, M. G. Huber, Dmitry A. Pushin, Albert R. Young

Published Jan 25, 2017• 15 citations
Publisher

Abstract

Dynamical diffraction leads to an interesting, unavoidable set of interference effects for neutron interferometers. This experiment studies the interference signal from two and three successive Bragg diffractions in the Laue geometry. We find that intrinsic Bragg-plane misalignment in monolithic, "perfect" silicon neutron interferometers is relevant between successive diffracting crystals, as well as within the Borrmann fan for typical interferometer geometries. We show that the dynamical phase correction employed in the Colella, Overhauser, and Werner gravitationally induced quantum interference experiments is attenuated by slight, intrinsic misalignments between diffracting crystals, potentially explaining the long-standing 1% discrepancy between theory and experiment. This systematic may also impact precision measurements of the silicon structure factor, affecting previous and future measurements of the Debye-Waller factor and neutron-electron scattering length as well as potential fifth-force searches. For the interferometers used in this experiment, Bragg planes of different diffracting crystals were found to be misaligned by 10 to 40 nrad.

DOI
10.1103/physreva.95.013840

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Dynamical diffraction leads to an interesting, unavoidable set of interference effects for neutron interferometers. This experiment studies the interference signal from two and three successive Bragg diffractions in the Laue geometry. We find that intrinsic Bragg-plane misalignment in monolithic, "perfect" silicon neutron interferometers is relevant between successive diffracting crystals, as well as within the Borrmann fan for typical interferometer geometries. We show that the dynamical phase correction employed in the Colella, Overhauser, and Werner gravitationally induced quantum interference experiments is attenuated by slight, intrinsic misalignments between diffracting crystals, potentially explaining the long-standing 1% discrepancy between theory and experiment. This systematic may also impact precision measurements of the silicon structure factor, affecting previous and future measurements of the Debye-Waller factor and neutron-electron scattering length as well as potential fifth-force searches. For the interferometers used in this experiment, Bragg planes of different diffracting crystals were found to be misaligned by 10 to 40 nrad.
The proper analysis of experiments to measure the quantum-mechanical phase shift due to potential gradients such as gravity across a perfect-silicon-crystal Mach–Zehnder interferometer for neutrons is complicated by the highly dispersive nature of the dynamical diffraction process describing the propagation of neutrons through a perfect crystal. Through dynamical diffraction, a coherent monochromatic incident beam of neutrons that does not exactly satisfy the Bragg condition is split into two currents within each crystal so that there are 16 possible coherent interfering trajectories by which the neutron can traverse the interferometer. In this work, previous calculations of the effects of dynamical diffraction on gravitationally induced phase-shift measurements are extended to include effects in all exit beams and internal effects within the subbeams for both symmetric and skew-symmetric interferometers. For the interferometers used in a recent experiment in which the gravitationally induced phase shift of the neutron is measured with a statistical uncertainty of the order of 1 part in 1000, it is found that these effects predict an increase of a few percent in the magnitude of the phase shift. Additionally, some consequences on the phase and contrast of restricting the beams within and after the interferometer are discussed. Agreement of this theory with experiment and the general applicability of the model is discussed.
The authors discuss the coherence properties of neutron scattering from perfect crystals and apply them to the splitting and coherent recombination of a neutron beam in a Laue-type interferometer. They also point out the difference between neutron and x-ray scattering in such devices and discuss the effect of a relative displacement of the various interferometer slabs on the fringe pattern. All this can be done without using the detailed dynamical theory of x-ray scattering. Various experiments are discussed, especially the neutron-gravity experiment of Colella, Overhauser, and Werner, which is analyzed both in the laboratory frame and in a frame freely falling with the neutron beam. The older electron diffraction experiment of Marton et al., and its relevance to the Aharonov---Bohm effect, is also discussed and reinterpreted, because the standard interpretation is not consistent with the results of the neutron experiment. An Appendix presents a general discussion of the transformation to a uniformly accelerated reference frame, as a guide to help analyze future such experiments.
Neutron interferometry performed in a noninertial frame is essentially influenced by dynamical diffraction effects occurring in the interferometer crystal which hitherto have not been taken into account. We have developed a corresponding theory from which a corrected phase shift is obtained which applies likewise to interferometry performed under the influence of gravity or on an accelerated neutron interferometer. The theory also predicts fading of interference contrast with increasing acceleration as was observed in the Colella-Overhauser-Werner gravity experiments but could not be explained unambiguously.
Abstract The quantum interference of DeBroglie matter waves is probably one of the most startling and fundamental aspect of quantum mechanics. It continues to tax our imaginations and leads us to new experimental windows on nature. Quantum interference phenomena are vividly displayed in the wide assembly of neutron interferometry experiments, which have been carried out since the first demonstration of a perfect silicon crystal interferometer in 1974. Since the neutron experiences all four fundamental forces of nature (strong, weak, electromagnetic, and gravitational), interferometry with neutrons provides a fertile testing ground for theory and precision measurements. Many Gedanken experiments of quantum mechanics have become real due to neutron interferometry. This book provides the reader with a detailed account of neutron interferometry experiments. The basic ideas and experiments related to coherence properties of matter waves and various post-selection criteria, gravitationally induced phase shifts, Berry's geometrical phase, spinor symmetry and spin superposition, Aharonov-Bohm topological interference effects, and the neutron version of the Sagnac effect are presented in a self-contained and pedagogical way. Interferometry with perfect crystals, artificial lattices, and spin-echo systems are topics of this book. It includes the theoretical motivations as well as connections to other areas of experimental physics, such as quantum optics, nuclear physics, gravitation, and atom interferometry. The book is written in a style that will be suitable at the beginning graduate level, and will excite many students and researchers in neutron physics, quantum optics, and atomic physics. Lecturers teaching courses in modern physics and quantum mechanics will find a number of interesting and historic experiments they may want to include in their lectures.
One of the significant successes in the field of neutron interferometry has been the experimental observation of the phase shift of a neutron de Broglie wave due to the action of the Earth's gravitational field. Past experiments have clearly demonstrated the effect and verified the quantum-mechanical equivalence of gravitational and inertial masses to a precision of about 1%. In this experiment the gravitationally induced phase shift of the neutron is measured with a statistical uncertainty of order 1 part in 1000 in two different interferometers. Nearly harmonic pairs of neutron wavelengths are used to measure and compensate for effects due to the distortion of the interferometer as it is tilted about the incident beam direction. A discrepancy between the theoretically predicted and experimentally measured values of the phase shift due to gravity is observed at the 1% level. Extensions to the theoretical description of the shape of a neutron interferogram as a function of tilt in a gravitational field are discussed and compared with experiment.
The quantum interference of de Broglie matter waves is probably one of the most startling and fundamental aspects of quantum mechanics. It continues to tax our imaginations and leads us to new experimental windows on nature. Quantum interference phenomena are vividly displayed in the wide assembly of neutron interferometry experiments, which have been carried out since the first demonstration of a perfect silicon crystal interferometer in 1974. Since the neutron experiences all four fundamental forces of nature (strong, weak, electromagnetic, and gravitational), interferometry with neutrons provides a fertile testing ground for theory and precision measurements. Many Gedanken experiments of quantum mechanics have become real due to neutron interferometry. Quantum mechanics is a part of physics where experiment and theory are inseparably intertwined. This general theme permeates the second edition of this book. It discusses more than 40 neutron interferometry experiments along with their theoretical motivations and explanations. The basic ideas and results of interference experiments related to coherence and decoherence of matter waves and certain post-selection variations, gravitationally induced quantum phase shifts, Berry's geometrical phases, spinor symmetry and spin superposition, and Bell's inequalities are all discussed and explained in this book. Both the scalar and vector Aharonov-Bohm topological interference effects and the neutron version of the Sagnac effect are presented in a self-contained and pedagogical way. Interferometry with perfect crystals, artificial lattices, and spin-echo systems are also topics of this book. It includes the theoretical underpinning as well as connections to other areas of experimental physics, such as quantum optics, nuclear physics, gravitation, and atom interferometry. The observed phase shifts due to the Earth's gravity and rotation indicate a close connection to relativity theory. Neutron interferometry can be considered as a central technique of quantum optics with massive particles. It has stimulated the development of interferometry with atoms, molecules and clusters. The book is written in a style that will be suitable at the senior undergraduate and beginning of graduate level. It will interest and excite many students and researchers in neutron, nuclear, quantum, gravitational, optical, and atomic physics. Lecturers teaching courses in modern physics and quantum mechanics will find a number of interesting and historic experiments they may want to include in their lectures.