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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Wavelength diversity in optically pumped alkali vapor lasers

Glen P. Perram

Published Jan 13, 2017• 1 citation
Publisher

Abstract

Alternative wavelengths for optically pumped alkali vapor lasers have been developed using single photon excitation of higher lying P-states, stimulated Raman processes, two-photon excitation of S and D states, and electric quadruple excitation on S-D transitions. Two photon excitation of Cs 72D leads to competing and cascade lasing producing red and infrared lasers operating on the D-P transitions, followed by ultraviolet, blue, the standard near infrared DPAL transitions operating on P-S transitions. The S-D pump transitions are fully bleached at pump intensities exceeding 1 MW/cm2, allowing for lasing transitions that terminate on the ground state. The kinetics of these systems are complex due to competition for population inversion among the many optical transitions. An optically pumped mid-infrared rubidium pulsed, mirrorless laser has also been demonstrated in a heat pipe along both the 62P3/2 - 62S1/2 transition at 2.73 μm and the 62P1/2 - 62S1/2 transition at 2.79 μm with a maximum energy of ~100 nJ. Performance improves dramatically as the rubidium vapor density is increased, in direct contradiction with the prior work. No scaling limitations associated with energy pooling or ionization kinetics have been observed. Practical application for infrared counter measures depends on the further development of blue diode pump sources. Finally, stimulated electronic Raman scattering and hyper-Raman processes in potassium vapor near the D1 and D2 lines have been observed using a stable resonator and pulsed laser excitation. First and second order Stokes and anti-Stokes lines were observed simultaneously and independently for a pump laser tuning range exceeding 70 cm-1. When the pump is tuned between the K D1 and D2 lines, an efficient hyper-Raman process dominates with a slope efficiency that exceeds 10%. Raman shifted laser may be useful as a target illuminator or atmospheric compensation beacon for a high power diode pumped alkali laser.

DOI
10.1117/12.2256256

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Alternative wavelengths for optically pumped alkali vapor lasers have been developed using single photon excitation of higher lying P-states, stimulated Raman processes, two-photon excitation of S and D states, and electric quadruple excitation on S-D transitions. Two photon excitation of Cs 72D leads to competing and cascade lasing producing red and infrared lasers operating on the D-P transitions, followed by ultraviolet, blue, the standard near infrared DPAL transitions operating on P-S transitions. The S-D pump transitions are fully bleached at pump intensities exceeding 1 MW/cm2, allowing for lasing transitions that terminate on the ground state. The kinetics of these systems are complex due to competition for population inversion among the many optical transitions. An optically pumped mid-infrared rubidium pulsed, mirrorless laser has also been demonstrated in a heat pipe along both the 62P3/2 - 62S1/2 transition at 2.73 μm and the 62P1/2 - 62S1/2 transition at 2.79 μm with a maximum energy of ~100 nJ. Performance improves dramatically as the rubidium vapor density is increased, in direct contradiction with the prior work. No scaling limitations associated with energy pooling or ionization kinetics have been observed. Practical application for infrared counter measures depends on the further development of blue diode pump sources. Finally, stimulated electronic Raman scattering and hyper-Raman processes in potassium vapor near the D1 and D2 lines have been observed using a stable resonator and pulsed laser excitation. First and second order Stokes and anti-Stokes lines were observed simultaneously and independently for a pump laser tuning range exceeding 70 cm-1. When the pump is tuned between the K D1 and D2 lines, an efficient hyper-Raman process dominates with a slope efficiency that exceeds 10%. Raman shifted laser may be useful as a target illuminator or atmospheric compensation beacon for a high power diode pumped alkali laser.
Abstract : An optically pumped mid-infrared rubidium (Rb) pulsed laser has been demonstrated in a heat pipe along the 62P3/2 - 62S1/2 transition at 2.730 micrometer and the 62P1/2 - 62S1/2 transition at 2.790 micrometer. The bleached limit, slope efficiency, and maximum laser output energy of the mid-IR Rb laser have been shown to scale linearly with increasing Rb density, contrary to prior laser demonstrations. A maximum output energy of 5 nJ per pulse had previously been observed before a rollover occurred in the scaling of output energy with Rb concentration. In this experiment, the maximum laser output energy observed was 100 nJ, with linear scaling to a Rb concentration of 7 x 10 to the 15th power cm-3. A maximum slope efficiency of 1.7 x 0.0001 was observed. Evidence that only a small percentage (2%) of the available pump photons were absorbed at a concentration of 2 x 10 to the 15th power cm-3 and a pump energy of 10 (mu)J. This indicated that there were 20,000 pump photons per Rb atom at a pump energy of 10 mJ, and that the effective laser efficiency was 0.65 percent or higher. The hyperfine structure and absorption spectral profile of the 52S1/2 - 62P1/2 and 52S1/2 - 62P3/2 (blue) pump transitions were studied using a continuous wave (cw) pump source.
Diode-pumped alkali laser (DPAL) technology offers a means of achieving high-energy gas laser output through optical pumping of the D-lines of Cs, Rb, and K. The exciplex effect, based on weak attractive forces between alkali atoms and polarizable rare gas atoms (Ar, Kr, Xe), provides an alternative approach via broadband excitation of exciplex precursors (XPAL). In XPAL configurations, we have observed multi-quantum excitation within the alkali manifolds which result in infrared emission lines between 1 and 4 μm. The observed excited states include the 42FJ states of both Cs and Rb, which are well above the two-photon energy of the excitation laser in each case. We have observed fluorescence from multi-quantum states for excitation wavelengths throughout the exciplex absorption bands of Cs-Ar, Cs-Kr, and Cs-Xe. The intensity scaling is roughly first-order or less in both pump power and alkali concentration, suggesting a collisional energy pooling excitation mechanism. Collisional up-pumping appears to present a parasitic loss term for optically pumped atomic systems at high intensities, however there may also be excitation of other lasing transitions at infrared wavelengths.
Stimulated emission on the ultraviolet and blue transitions in Cs has been achieved by pumping via two-photon absorption and four-wave mixing for the pump transition 62S12→82D32,52. The emission performance of the optically pumped cesium vapor laser operating in ultraviolet and blue has been extended to 650 nJ/pulse for 387 nm, 1 to 3 μJ/pulse for 388 nm, 200 nJ/pulse for 455 nm, and 500 nJ/pulse for 459 nm. Emission performance improves dramatically as the cesium vapor density is increased, and no scaling limitations associated with energy pooling or ionization kinetics have been observed.
Abstract : Mirrorless lasing has been successfully demonstrated in a Rubidium heat pipe. Lasing was observed on the 6(2)P(sub 3/2)-6(2)S(sub 1/2) energy transition at 2.73 microns and on the 6(2)P(sub 1/2)-6(2)S(sub 1/2) transition at 2.79 microns. The transitions were optically pumped from 5(2)S(sub 1/2)-6(2)P(sub 3/2) at 420.2 nm and from 5(2)S(sub 1/2)-6(2)P(sub 1/2) at 421.7 nm, respectively. The 5(2)S(sub 1/2)-6(2)P(sub 3/2) transition was excited over a 36 GHz band, while the 5(2)S(sub 1/2)-6(2)P(sub 1/2) transition was excited over a 24 GHz band. Both pump transitions showed a high degree of saturation and only a small fraction (1%) of the incident pump energy was absorbed. Output energies of up to 5 nJ were obtained at 2.73 microns and of up to 5.4 nJ at 2.79 microns when pumped at pulse energies of 4 mJ. Both transitions experienced bleaching at this 4 mJ pump energy, limiting further IR output energy. Increasing rubidium concentration at bleached pump energies showed no increase in laser energy after 170 deg. C, likely due to second order processes. Slope efficiency for both transitions, however, increased linearly with rubidium concentration up to 11 x .000001 The addition of small amounts of argon, helium, and ethane (5-45 Torr) were found to fully quench lasing action on both transitions.
Achieving population inversion through multi-photon cascade pumping is almost always difficult, and most laser medium work under 1-photon excitation mechanism. But for alkali atoms such as cesium, relatively large absorption cross sections of several low, cascading energy levels enable them properties such as up conversion. Here we carried out research on two-photon excitation alkali fluorescence. Two photons of near infrared region are used to excite alkali atoms to n 2 D5/2, n 2 D3/2 or higher energy levels, then the blue fluorescence of (n+1) 2 P3/2,(n+1) 2 P1/2→n 2 S1/2 are observed. Different pumping paths are tried and by the recorded spectra, transition routes of cesium are deducted and concluded. Finally the possibility of two-photon style DPALs (diode pumped alkali laser) are discussed, such alkali lasers can give output wavelengths in the shorter end of visual spectroscopy (400-460 nm) and are expected to get application in underwater communication and material laser processing.
Lasing on the 62P1/2→62S1/2(D1) resonance transition of atomic Cs at 894.3 nm has been demonstrated in mixtures of Ar, ethane, and Cs vapor by the photoexcitation of ground state Cs-Ar collision pairs and subsequent dissociation of diatomic, electronically-excited CsAr molecules (exciplexes or excimers). The blue satellites of the alkali D2 lines provide a pathway for optically pumping atomic alkali lasers on the principal series (resonance) transitions with broad linewidth (>2 nm) semiconductor diode lasers. In this paper we discuss different variations of this new laser system and the experiments of the initial demonstration.