A prototypical experiment in cavity quantum electrodynamics involves controlling the light-matter interaction by tuning the frequency of a cavity mode in- and out-of resonance with the frequency of a quantum emitter,1-3 while the field amplitude is generally unaltered. The opposite situation, where one perturbs the spatial pattern of a cavity mode without changing its frequency, has been considered only recently in a few works.4, 5 Changing the amplitude of the field at the emitter's position has important applications, at it allows a real-time control of the light-matter coupling rate, and therefore a direct control of processes such as spontaneous emission and Rabi oscillations. In view of this large potential, in this paper we discuss general design principles that allow obtaining large variations of the electromagnetic field, without change of the frequency, upon an external perturbation of the cavity. We showcase the application of these rules to two photonic structures, a single Fabry-Perot cavity and a coupled three-cavity system. As showed by our analysis and by the examples provided, a small frequency spacing between the modes of the unperturbed cavity is an important requirement to obtain large field variations upon small perturbations. In this regard, a coupled-cavity system, where the frequency spacing is controlled by the interaction rates between the single cavities, constitutes the most promising system to achieve large modulations of the field amplitude.
A prototypical experiment in cavity quantum electrodynamics involves controlling the light-matter interaction by tuning the frequency of a cavity mode in- and out-of resonance with the frequency of a quantum emitter,1-3 while the field amplitude is generally unaltered. The opposite situation, where one perturbs the spatial pattern of a cavity mode without changing its frequency, has been considered only recently in a few works.4, 5 Changing the amplitude of the field at the emitter's position has important applications, at it allows a real-time control of the light-matter coupling rate, and therefore a direct control of processes such as spontaneous emission and Rabi oscillations. In view of this large potential, in this paper we discuss general design principles that allow obtaining large variations of the electromagnetic field, without change of the frequency, upon an external perturbation of the cavity. We showcase the application of these rules to two photonic structures, a single Fabry-Perot cavity and a coupled three-cavity system. As showed by our analysis and by the examples provided, a small frequency spacing between the modes of the unperturbed cavity is an important requirement to obtain large field variations upon small perturbations. In this regard, a coupled-cavity system, where the frequency spacing is controlled by the interaction rates between the single cavities, constitutes the most promising system to achieve large modulations of the field amplitude.
We propose a scheme for the ultrafast control of the emitter-field coupling rate in cavity quantum electrodynamics. This is achieved by the control of the vacuum field seen by the emitter through a modulation of the optical modes in a coupled-cavity structure. The scheme allows the on/off switching of the coupling rate without perturbing the emitter and without introducing frequency chirps on the emitted photons. It can be used to control the shape of single-photon pulses for high-fidelity quantum state transfer, to control Rabi oscillations and as a gain-modulation method in lasers. We discuss two possible experimental implementations based on photonic crystal cavities and on microwave circuits.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
We propose a scheme for the ultrafast control of the emitter-field coupling rate in cavity quantum electrodynamics. This is achieved by the control of the vacuum field seen by the emitter through a modulation of the optical modes in a coupled-cavity structure. The scheme allows the on-off switching of the coupling rate without perturbing the emitter and without introducing frequency chirps on the emitted photons. It can be used to control the shape of single-photon pulses for high-fidelity quantum state transfer, to control Rabi oscillations, and as a gain-modulation method in lasers. We discuss two possible experimental implementations based on photonic crystal cavities and on microwave circuits.
Rapid advances in quantum technology have made possible the control of quantum states of elementary material quantum systems, such as atoms or molecules, and of the electromagnetic radiation field resulting from spontaneous photon emission of their unstable excited states to such a level of precision that subtle quantum electrodynamical phenomena have become observable experimentally. Recent developments in the area of quantum information processing demonstrate that characteristic quantum electrodynamical effects can even be exploited for practical purposes provided the relevant electromagnetic field modes are controlled by appropriate cavities. A central problem in this context is the realization of an ideal transfer of quantum information between a state of a material quantum system and a quantum state of the electromagnetic radiation field which contains a small number or even a single photon only. Despite much recent work in cavity quantum electrodynamics, which has explored this problem successfully in cases in which the number of accessible electromagnetic field modes is strongly restricted by a cavity, currently still much less is known about ideal quantum state transfer between matter and few-photon quantum states of the electromagnetic field in the extreme opposite case of free space. In this contribution we review recent work which explores characteristic quantum electrodynamical phenomena governing the interaction of a material quantum system with the electromagnetic field in extreme many-mode cases which are close to cavity-free situations. For this purpose the simplest possible quantum electrodynamical situation, namely the interaction of a single material two-level system with the wave packet of a single optical photon, is investigated in free space and in situations in which a large cavity modifies the mode structure of the electromagnetic field modes. It is demonstrated that perfect excitation of an atom by a properly shaped single-photon wave packet is possible even in free space. In particular, it is demonstrated that perfect excitation of an atom can be achieved by a single optical photon which is prepared initially in an appropriate superposition of plane-wave modes, provided this photon is focused subsequently onto the absorbing atom by a parabolic cavity.
Spontaneous emission into micro- or nano-scale structures can be enhanced or inhibited by engineering the local density of optical states using closed quantum cavities. When electromagnetic fields are confined within small mode volumes of a high-Q symmetrical closed quantum cavity, the Purcell effect significantly accelerates the natural spontaneous emission. Due to the statistical nature of spontaneous emission, the emitted fields do not have a well-defined phase; consequently, the emission is incoherent and lacks directional control. The situation becomes more complicated in multi-mode cavities, as selecting a specific mode in a particular direction requires precise detuning between the emitter transition frequency and the cavity mode frequency to ensure strong coupling. In single-mode cavities, only the dominant mode can resonate, and only in a specific direction; thus, an appropriate transition frequency range can be easily determined. Such cavities allow for greater manipulation of the local electromagnetic density of states, facilitating effective control of the direction of spontaneous emission. This property is essential for creating efficient single-photon sources, photonic circuits, and on-chip quantum information.
Recent technological developments have made it increasingly easy to access the non-perturbative regimes of cavity quantum electrodynamics known as ultrastrong or deep strong coupling, where the light-matter coupling becomes comparable to the bare modal frequencies. In this work, we address the adequacy of the broadly used single-mode cavity approximation to describe such regimes. We demonstrate that, in the non-perturbative light-matter coupling regimes, the single-mode models become unphysical, allowing for superluminal signalling. Moreover, considering the specific example of the quantum Rabi model, we show that the multi-mode description of the electromagnetic field, necessary to account for light propagation at finite speed, yields physical observables that differ radically from their single-mode counterparts already for moderate values of the coupling. Our multi-mode analysis also reveals phenomena of fundamental interest on the dynamics of the intracavity electric field, where a free photonic wavefront and a bound state of virtual photons are shown to coexist.