In this thesis I report the first experimental observation of an interaction between a postselected single photon and an electromagnetic field containing a few thousand photons.This is the first observation of the nonlinear interactions due to a single freely propagatingphoton. To achieve this pioneering result, we have theoretically and experimentally studied nonlinear optics at the few-photon level. To the best of our knowledge, the pulse energy levels used for our experiments are the lowest energies used for cross-phase modulation in free space.Photon-photon interaction is vanishingly weak; the strength of this interaction can be enhanced in the presence of a material medium as mediator. In our experiment, we use an atomic coherence effect, namely Electromagnetically-induced Transparency (EIT), to produce a `giant' nonlinear interaction between two optical fields. We have observed a nonlinear phase shift of 18 ± 4 µrad per freely propagating single photon. This is done by sending very weak coherent state pulses into the medium and subsequently detecting single photons, inferring the existence of a photon in the interaction region.The optical setup, electronics and software that have been developed during the completion of this thesis provide the basis for several exciting future light-matter interaction experiments. We have produced phase-stable laser beams to create EIT in our cold Rubidium sample prepared in a Magneto-optical Trap (MOT). The laser system and the improved MOT setup have been built to be stable so that we can do very long data acquisition runs. We also have develop ed to ols and software with high precision and stability such that we can measure phase shifts down to micro-radian level.
In this thesis I report the first experimental observation of an interaction between a postselected single photon and an electromagnetic field containing a few thousand photons.This is the first observation of the nonlinear interactions due to a single freely propagatingphoton. To achieve this pioneering result, we have theoretically and experimentally studied nonlinear optics at the few-photon level. To the best of our knowledge, the pulse energy levels used for our experiments are the lowest energies used for cross-phase modulation in free space.Photon-photon interaction is vanishingly weak; the strength of this interaction can be enhanced in the presence of a material medium as mediator. In our experiment, we use an atomic coherence effect, namely Electromagnetically-induced Transparency (EIT), to produce a `giant' nonlinear interaction between two optical fields. We have observed a nonlinear phase shift of 18 ± 4 µrad per freely propagating single photon. This is done by sending very weak coherent state pulses into the medium and subsequently detecting single photons, inferring the existence of a photon in the interaction region.The optical setup, electronics and software that have been developed during the completion of this thesis provide the basis for several exciting future light-matter interaction experiments. We have produced phase-stable laser beams to create EIT in our cold Rubidium sample prepared in a Magneto-optical Trap (MOT). The laser system and the improved MOT setup have been built to be stable so that we can do very long data acquisition runs. We also have develop ed to ols and software with high precision and stability such that we can measure phase shifts down to micro-radian level.
In third order nonlinear mediums, the intensity of one optical field can modify the phase of another optical field. This is known as cross-phase modulation (XPM) and is important for Quantum Information Processing (QIP) as phase shifts of single-photons that exceed π rad can be used to implement two-qubit quantum logic gates. For a conventional XPM scheme, the Kerr nonlinearity responsible for XPM is too small for appreciable phase shifts to be achieved with low intensity optical fields. However, Electromagnetically Induced Transparency (EIT) can increase this nonlinearity by several orders of magnitude. This thesis discusses the experimental construction of a laser-atomic system capable of EIT modulated XPM. This includes construction of a rubidium magneto-optical trap (RbMOT), characterization of this RbMOT, demonstration of EIT in the RbMOT, and a system capable of detecting optical phase shifts produced by EIT. The talk will conclude with an outlook on further implementations to the experiment that will increase this nonlinearity such that phase shifts at the single-photon level are possible. | 76 pages
Photons are good candidates for carrying quantum information because they are very stable particles: they interact weakly with the medium and barely with each other. However, this has drawbacks when you want to process the information because, in this case, it is preferable to have photon-photon interactions. For example, for applications in quantum repeaters, such interactions would allow deterministic Bell state measurements, increasing the entanglement distribution rate between two remote nodes. Getting two photons to interact with each other efficiently requires mapping them into a nonlinear medium at the single-photon level, that is, a medium that reacts differently when it interacts with a single photon than when it does with two. Such strong nonlinearity has been demonstrated with Rydberg atoms, which are atoms excited to a state with a high principal quantum number.
In this thesis we have performed nonlinear quantum optics experiments using an ensemble of cold Rydberg atoms, where we have studied the properties of the quantum light emitted by these atoms. First, we demonstrated nonlinearities at the single-photon level. To reach this stage, we made several improvements to the previous experimental setup available in the group, of which the implementation of a dipole trap was especially relevant. We evidence quantum nonlinearity by measuring photon antibunching for the transmitted light after interacting with the Rydberg state under electromagnetically induced transparency (EIT). We also showed the generation of single photons on-demand after storing weak coherent states of light pulses as collective Rydberg excitations.
Then, we studied the variation of the light statistic throughout the output pulse after propagating through the medium as Rydberg polaritons, which are superposition states of light and Rydberg excitations. We showed that the properties at the beginning and the end of the pulse were different from those of the steady state. In particular, the light detected after the input pulse was abruptly turned off gave much stronger suppression of two-photon events. Then, we investigated how to exploit this effect to generate single photons on demand. To do this, we analyzed the quality of the single photons detected at the end of the pulse as a function of the detection probability and compared the results with those obtained by storing the input pulse as collective Rydberg excitations. We showed that the photons were generated more efficiently when increasing the detection window at the cost of deteriorating the single photons statistics.
Finally, we investigated the indistinguishability of the photons emitted by our Rydberg atomic ensemble, a crucial property for using Rydberg atoms as nodes in quantum networks. We also compared the single photons generated after storage under EIT conditions with those obtained using a two-photon Raman excitation to the Rydberg state. We measured the indistinguishability by making them interfere with weak coherent states of light in a Hong-Ou-Mandel experiment. And we showed that, although we obtained better photon statistics under EIT conditions, the indistinguishability from those obtained with Raman excitation was significantly higher.
This dissertation reports experimental studies of nonlinear optical effects manifested by electromagnetically induced transparency (EIT) in cold Rb atoms. The cold Rb atoms are confined in a magneto-optic trap (MOT) obtained with the standard laser cooling and trapping technique. Because of the near zero Doppler shift and a high phase density, the cold Rb sample is well suited for studies of atomic coherence and interference and related applications, and the experiments can be compared quantitatively with theoretical calculations. It is shown that with EIT induced in the multi-level Rb system by laser fields, the linear absorption is suppressed and the nonlinear susceptibility is enhanced, which enables studies of nonlinear optics in the cold atoms with slow photons and at low light intensities. Three independent experiments are described and the experimental results are presented. First, an experimental method that can produce simultaneously co-propagating slow and fast light pulses is discussed and the experimental demonstration is reported. Second, it is shown that in a three-level Rb system coupled by multi-color laser fields, the multi-channel two-photon Raman transitions can be manipulated by the relative phase and frequency of a control laser field. Third, a scheme for all-optical switching near single photon levels is developed. The scheme is based on the phase-dependent multi-photon interference in a coherently coupled four-level system. The phase dependent multi-photon interference is observed and switching of a single light pulse by a control pulse containing ∼20 photons is demonstrated. These experimental studies reveal new phenomena manifested by quantum coherence and interference in cold atoms, contribute to the advancement of fundamental quantum optics and nonlinear optics at ultra-low light intensities, and may lead to the development of new techniques to control quantum states of atoms and photons, which will be useful for applications in quantum measurements and quantum photonic devices.
This thesis summarizes my work on the interactions between light and matter in the context of optical quantum information processing. I have designed and implemented a phase-sensitive detection scheme for optical-frequency electromagnetic fields, which has been used to measure μrad phase shifts on nanosecond timescales. This phase measurement was developed for the express purpose of detecting cross-phase modulation (XPM), a key ingredient in the construction of optical logic gates. I have implemented the 'N-scheme', a form of XPM which exploits electromagnetically-induced transparency (EIT) and which was promised to yield 'giant' optical nonlinearities sufficient for all-optical quantum information processing. Using a cloud of laser-cooled 85Rb atoms as the nonlinear medium, I present the first ever experimental study of EIT-enhanced XPM in the controversial regime of broadband signal pulses and spectrally narrow EIT windows. The results of this experiment constitute a breakdown of the original proposal for EIT-enhanced XPM. In light of these findings, I conclude with a theoretical analysis of the feasibility of using N-scheme as implemented in our lab to perform a non-demolition measurement of a single photon (a crucial step when using XPM to generate a universal optical logic gate). While possible in principle, the experimental conditions necessary to achieve a signal-to-noise ratio above unity are found to be practically unrealistic, suggesting a more sophisticated scheme is necessary.
The ability to control light with light at ultralow powers has been a major avenue of research in photonics with applications to optical communications, computation, and signal processing. Such light-by-light scattering is achieved in a medium with a strong light-matter interaction, and for the development of quantum information networks it is important to demonstrate such effects near the single-photon level. Alkali-metal vapors such as rubidium (Rb) enable strong light-matter interactions due to the large cross section per atom and well-defined energy level structure, while the use of optical fibers offers the advantage of possible integration with modern optical communication systems. Hollow-core photonic band-gap fibers (PBGFs) can combine both these technologies such that both the atoms and the optical fields are transversely confined to a region that is a few wavelengths in size, which offers the prospect of exploring few-photon nonlinear interactions. We generate large optical depths in such a Rb-PBGF system, and the tight light confinement, high vapor density and long interaction length allow us to perform nonlinear optics at ultralow power. We demonstrate large signal amplification (>100) and frequency conversion using a four-wave mixing process with only microwatts of pump power. This is, to our knowledge, the largest gain observed at such low power. We perturb the coherence of this four-wave mixing to demonstrate all-optical modulation at unprecedented bandwidths (~300 MHz) for an atomic-vapor system, with an energy density of only tens of pho- tons per atomic cross-section, comparable to that achieved in more elaborate setups based on cold-atomic clouds. We then demonstrate an enhancement of several orders of magnitude in degenerate two-photon absorption in our RbPBGF system over that achieved in bulk vapor cells in a focused beam geometry. This allows us to directly measure two-photon absorption from a beam by detecting its intensity on a photodiode. Further, employing a near-resonant, non-degenerate two-photon transition in Rb, we demonstrate all-optical intensity modulation with just a few photons (<20), or only a few attojoules of energy, at relatively large bandwidths (~50 MHz) for such a sensitive scheme. This result takes us to within an order of magnitude of single-photon switching, and improves upon previous experiments for freely propagating optical fields, including those in cold-atoms. Finally, we produce relatively large cross-phase shifts of a few milliradians on a meter beam with <20 signal photons by tuning slightly away from resonance on the same non-degenerate two-photon transition. This corresponds to a phase shift of 0.3 milliradian per photon, with a fast response time of <5 ns. This represents, to our knowledge, the largest such nonlinear phase shift induced in a single-pass through a room temperature medium. Our Rb-PBGF system can thus potentially be employed to realize weak-nonlinearity based quantum computation and quantum non-demolition measurement of photon number. Through these experiments, we show the potential of a Rb-PBGF system for exploring quantum nonlinear optics at ultralow powers. Moreover, our system is simpler and easier to control and manipulate than setups based on cold atomic clouds and/or high-finesse cavities, and holds promise for integration with fiber-optic communication networks.
I present experimental and theoretical work on extending nonlinear optical effects to the quantum domain. First, I experimentally demonstrate an incoherent nonlinear effect linked to the amplification stage of photon detection in a single-photon counter. The detector, in the high-efficiency regime, does not follow Glauber's quantum mechanical model for photodetection and, as a result, quantum interference effects are observable in the singles rate of one detector. I then go on to theoretically describe and experimentally demonstrate two coherent nonlinear optical effects at the single-photon level. In both experiments, the usually weak nonlinear optical properties of a common nonlinear crystal are enhanced by over 10 orders of magnitude using interference. The first of these coherent processes uses interference to frequency double all photon pairs from a couple of very weak laser beams (containing, on average, less than one photon per pulse). I show how this nonlinearity might be used for �phase-sum� entanglement swapping and an experimental demonstration of Hardy's paradox. The second coherent effect is the dispersive analogue to the first; instead of frequency doubling all of the photon pairs, all photon pairs experience an additional nonlinear phase shift. It is analogous to an immensely enhanced Kerr nonlinearity. This effect is applied to the problem of Bell-state discrimination and can be used to entangle and disentangle the polarization states of a pair of photons under certain conditions. The final experiment in this thesis is a demonstration of a technique for creating coherent superpositions of zero and one photon based on the detection of a single, �trigger� photon.