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Chinese Physics Letters

Electromagnetically Induced Transparency in a Cold Gas with Strong Atomic Interactions

Yuechun Jiao, Xiaoxuan Han, Zhi-Wei Yang, Jianming Zhao, Suotang Jia

Published Dec 1, 2016• 13 citations
Publisher

Abstract

Electromagnetically induced transparency (EIT) is investigated in a system of cold, interacting cesium Rydberg atoms. The utilized cesium levels 6S 1/2 , 6P 3/2 and nD 5/2 constitute a cascade three-level system, in which a coupling laser drives the Rydberg transition, and a probe laser detects the EIT signal on the 6S 1/2 to 6P 3/2 transition. Rydberg EIT spectra are found to depend on the strong interaction between the Rydberg atoms. Diminished EIT transparency is obtained when the Rabi frequency of the probe laser is increased, whereas the corresponding linewidth remains unchanged. To model the system with a three-level Lindblad equation, we introduce a Rydberg-level dephasing rate γ3 = κ × (ρ33/Ω p ) 2 , with a value κ that depends on the ground-state atom density and the Rydberg level. The simulation results are largely consistent with the measurements. The experiments, in which the principal quantum number is varied between 30 and 43, demonstrate that the EIT reduction observed at large Ω p is due to the strong interactions between the Rydberg atoms.

DOI
10.1088/0256-307x/33/12/123201

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Electromagnetically induced transparency (EIT) is investigated in a system of cold, interacting cesium Rydberg atoms. The utilized cesium levels 6S 1/2 , 6P 3/2 and nD 5/2 constitute a cascade three-level system, in which a coupling laser drives the Rydberg transition, and a probe laser detects the EIT signal on the 6S 1/2 to 6P 3/2 transition. Rydberg EIT spectra are found to depend on the strong interaction between the Rydberg atoms. Diminished EIT transparency is obtained when the Rabi frequency of the probe laser is increased, whereas the corresponding linewidth remains unchanged. To model the system with a three-level Lindblad equation, we introduce a Rydberg-level dephasing rate γ3 = κ × (ρ33/Ω p ) 2 , with a value κ that depends on the ground-state atom density and the Rydberg level. The simulation results are largely consistent with the measurements. The experiments, in which the principal quantum number is varied between 30 and 43, demonstrate that the EIT reduction observed at large Ω p is due to the strong interactions between the Rydberg atoms.
We study Rydberg electromagnetically induced transparency (EIT) of a cascade three-level atom involving 80 D 5/2 state in a strong interaction regime employing a cesium ultracold cloud. In our experiment, a strong coupling laser couples 6 P 3/2 to 80 D 5/2 transition, while a weak probe, driving 6 S 1/2 to 6 P 3/2 transition, probes the coupling induced EIT signal. At the two-photon resonance, we observe that the EIT transmission decreases slowly with time, which is a signature of interaction induced metastability. The dephasing rate γ OD is extracted with optical depth OD = γ OD t . We find that the optical depth linearly increases with time at onset for a fixed probe incident photon number R in before saturation. The dephasing rate shows a nonlinear dependence on R in . The dephasing mechanism is mainly attributed to the strong dipole-dipole interactions, which leads to state transfer from nD 5/2 to other Rydberg states. We demonstrate that the typical transfer time τ 0(80 D ) obtained by the state selective field ionization technique is comparable with the decay time of EIT transmission τ 0(EIT) . The presented experiment provides a useful tool for investigating the strong nonlinear optical effects and metastable state in Rydberg many-body systems.
A high sensitivity spectroscopy of Rydberg atoms is presented by using electromagnetically induced transparency (EIT) in the 6S(1/2)-6P(3/2)-n D ladder-type system of cesium vapor cell at room temperature. The EIT spectra of 40 D Rydberg state are measured and the dependences of the EIT magnitude and linewidth on the coupling laser power are investigated in detail. The Rydberg EIT linewidth is measured to be about 5.6 MHz when the powers of probe and coupling lasers are 50 microW and 5.2 mW, respectively, and which is close to the natural linewidth of cesium atoms. The effect of double resonance optical pumping on EIT is also investigated. The fine structures of nD (n = 39-55) are measured and the experimental result is in agreement with quantum defect theory.
Rydberg atoms, with large principal quantum number n, have been widely investigated in recent years due to their peculiar properties, such as big sizes, long lifetimes and strong interactions with fields and other Rydberg atoms. Rydberg atoms are very sensitive to external fields due to their large polarizabilities scaling as n7.These make Rydberg atoms an ideal candidate for the quantum information, the many-body interaction, etc.In this work, we investigate the Rydberg atoms using electromagneticlly induced transparency (EIT) in a ladder three-level system. The EIT is a quantum interference effect between two excitation path-ways driven by two laser fields. The main idea is performed in a room temperature cesium vapor cell, where the probe laser frequency is modulated. The ground state (6P1/2), excited state (6P3/2), and Rydberg state (nS1/2) constitute a Rydberg three-level system, in which the probe laser is fixed to the 6S1/2 (F = 4)6P3/2 (F = 5) transition by saturated absorption spectrum technique, whereas the coupling laser is scanned across the 6P3/249S1/2 transition. We detect the demodulated EIT signal with the lock-in amplifier (SR830). The modulated EIT signal shows a two-peak structure. The measured spacing between two peaks increases with the frequency detuning, caused by the modulation amplitude, and half the spacing between the peak-to-peak is nearly 1.67 times the modulation amplitude of the probe laser; the measured result shows that the splitting is independent of the modulation frequency. The experimental results are in agreement with the theoretical calculations. The results in our work can be used for real-time monitoring of the laser-line profiles and the fluctuation of laser frequency.
Electromagnetically induced transparency (EIT) and Autler–Townes splitting (ATS) are two similar yet distinct phenomena that modify the transmission of a weak probe field through an absorption medium in the presence of a coupling field, featured in a variety of three-level atomic systems. In many applications it is important to distinguish EIT from ATS splitting. We present EIT and ATS spectra in a three-level cascade system, involving cold cesium atoms in the Rydberg state. The EIT linewidth, γ EIT , defined as the full width at half maximum of the transparency window, and the ATS splitting, γ ATS , defined as the peak-to-peak distance between AT absorption peaks, are used to delineate the EIT and ATS regimes and to characterize the transition between the regimes. In the cold-atom medium, in the weak-coupler (EIT) regime γ EIT ≈ A + B ( + , where Ω c and Ω p are the coupler and probe Rabi frequencies, Γ eg is the spontaneous decay rate of the intermediate 6P 3/2 level, and parameters A and B that depend on the laser linewidth. We explore the transition into the strong-coupler (ATS) regime, which is characterized by the relation γ ATS ≈ Ω c . The experiments are in agreement with numerical solutions of the Master equation. Our analysis accounts for non-ideal conditions that exist in typical realizations of Rydberg-EIT, including laser-frequency jitter, Doppler mismatch of the utilized two-color Rydberg EIT system, and strong probe fields. The obtained criteria to distinguish cold-atom EIT from ATS are readily accessible and applicable in practical implementations.
We perform spectroscopic measurements of electromagnetically induced transparency (EIT) in a strongly interacting Rydberg gas. We observe a significant spectral shift and attenuation of the transparency resonance due to the presence of interactions between Rydberg atoms. We characterize the attenuation as the result of an effective dephasing and show that the shift and the dephasing rate increase versus atomic density, probe Rabi frequency, and principal quantum number of Rydberg states. Moreover, we find that the spectral shift is reduced if the size of a Gaussian atomic cloud is increased and that the dephasing rate increases with the EIT pulse duration at large-parameter regimes. We simulate our experiment with a semianalytical model, which yields results in good agreement with our experimental data.
Abstract We present the electromagnetically induced transparency (EIT) spectra of cold Rydberg four-level cascade atoms consisting of the 6S1/2 → 6P3/2 → 7S1/2 → 60P3/2 scheme. A coupling laser drives the Rydberg transition, a dressing laser couples two intermediate levels and a weak probe laser probes the EIT signal. We numerically solve the Bloch equations and investigate the dependence of the probe transmission rate signal on the coupling and dressing lasers. We find that the probe transmission rate can display an EIT or electromagnetically induced absorption (EIA) profile, depending on the Rabi frequencies of the coupling and dressing lasers. When we increase the Rabi frequency of the coupling laser and keep the Rabi frequency of the probe and dressing laser fixed, flipping of the EIA to EIT spectrum occurs at the critical coupling Rabi frequency. When we apply a microwave field coupling the transition 60P3/2 → 61S1/2, the EIT spectrum shows Autler–Townes splitting, which is employed to measure the microwave field. The theoretical measurement sensitivity can be 1.52 × 10−2 nV⋅cm−1⋅Hz−1/2 at the EIA–EIT flipping point.