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Optics Letters

Kerr-induced controllable adiabatic frequency conversion in an ultrahigh Q silica toroid microcavity

Wataru Yoshiki, Yoshihiro Honda, Misako Kobayashi, Tomohiro Tetsumoto, Takasumi Tanabe

Published Nov 18, 2016• 18 citations
Publisher

Abstract

In this Letter, we report, based on our knowledge, the first demonstration of Kerr-induced adiabatic frequency conversion in a silica toroid microcavity. Taking advantage of the instantaneous response of the Kerr effect, we achieved adiabatic frequency conversion with a controllable amount of frequency shift and time width. In addition, thanks to the combination of the Kerr effect and the ultrahigh Q (>107) of the silica toroid microcavity, we also observed multiple frequency conversion within a photon lifetime. Furthermore, use of the Kerr effect allowed us to investigate the influence of the relative phase between the original and converted light.

DOI
10.1364/ol.41.005482

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In this Letter, we report, based on our knowledge, the first demonstration of Kerr-induced adiabatic frequency conversion in a silica toroid microcavity. Taking advantage of the instantaneous response of the Kerr effect, we achieved adiabatic frequency conversion with a controllable amount of frequency shift and time width. In addition, thanks to the combination of the Kerr effect and the ultrahigh Q (>107) of the silica toroid microcavity, we also observed multiple frequency conversion within a photon lifetime. Furthermore, use of the Kerr effect allowed us to investigate the influence of the relative phase between the original and converted light.
In this thesis we study ultrafast all-optical switching of microcavities. We employ the electronic Kerr effect to switch the resonance frequency of microcavities operating at telecom wavelengths. We observe the fastest possible switching of a microcavity resonance within 300 fs. The switching speed is only determined by the cavity storage time; only limited by the speed of light and not by material related relaxation properties. For the first time, we derive and measure the non-degenerate three-photon absorption coefficient of GaAs. Using the measured nondegenerate two- and three-photon absorption coefficients we estimate that the trigger laser only lose 22 aJ/µm2 at each switch event, which is a record level of minimum energy loss per switch event. We achieve repeated switching of microcavities within 700 fs, corresponding to THz rates. Therefore to best of our knowledge, we have broken the THz clock rate barrier experimentally using semiconductor cavities for the first time. The THz clock rate that we achieve can be a solution for information technology that is exploring ways to meet the growth rate of the computational demand. The color of light is a main visual perception of light for humans. Indeed, a simple measure for the color of light is given by its frequency since frequency of light is invariant from one medium to another. Although the propagation of light is strongly modified using nanostructures such as photonic crystals and microcavities, the frequency of light stays constant in these structures as well. The color of light can be changed in a nonlinear process or by absorption and re-emission. Using microcavities light is conveniently confined in space and then by dynamical control the medium can be changed to act as a nonlinear medium for light. Remarkably, we show that during the switching of cavities we achieve both up and down frequency conversion of light. The frequency conversion that we observe is a result of the instantaneous refractive index change achieved using the electronic Kerr effect. We achieve repeated frequency conversion at THz rates and generate blue- and red-shifted light pulses at this rate.
Ever since the advent of nonlinear optics, the generation of light by frequency-conversion is drawing continued attention, and leading to emerging applications such as supercontinuum sources for ultra stable clocks and advanced microscopy. A modern approach to frequency-conversion is to switch light confined in micro- and nanocavity resonances to enable on-chip operation. Supposedly, nonlinear frequency conversion in such confined media differs from traditional non-linear optics in three key features regarding output spectrum, frequency shift, and critical time scale. Therefore, we switch GaAs-AlAs microcavities by the electronic Kerr effect, and study a range of quality factors to bridge the confined and the traditional non-linear regimes. We uncover the key role of the density of vacuum fluctuations, i.e., the local density of optical states (LDOS) for newly generated frequencies, a concept inspired by cavity quantum electrodynamics (cQED). As a result, we succeed to establish a framework, which not only describes nonlinear optics both in traditional bulk and in confined media but also opens a new control dimension in changing the color of light.
Abstract All-optical tunable buffering was recently achieved on a chip by using dynamically tuned coupled mode induced transparency, which is an optical analogue of electromagnetically induced transparency. However, the small Q s of about 105 used in those systems were limiting the maximum buffering time to a few hundred ps. Although employing an ultra-high Q whispering gallery mode (WGM) microcavity can significantly improve the maximum buffering time, the dynamic tuning of the WGM has remained challenging because thermo-optic and pressure tunings, which are widely used for WGM microcavities, have a very slow response. Here we demonstrate all-optical tunable buffering utilizing coupled ultra-high Q WGM cavities and the Kerr effect. The Kerr effect can change the refractive index instantaneously, and this allowed us to tune the WGM cavity very quickly. In addition, from among the various WGM cavities we employed a silica toroid microcavity for our experiments because it has an ultra-high Q factor (>2 × 107) and a small mode volume, and can be fabricated on a chip. Use of the Kerr effect and the silica toroid microcavity enabled us to observe an on-chip all-optical tunable buffering operation and achieve a maximum buffering time of 20 ns.
Changing the color of light in a small mode volume is essential for applications that require on-chip operation. Microcavities are profound structures given their property to confine light in a small mode volume. Here, I numerically investigate the frequency conversion of light in a microcavity and show that the frequency converted light intensity is distinguished from an open medium such as an optical fiber or a nonlinear crystal. I observe that the frequency converted light intensity increases with increased rate of change of the refractive index of the microcavity. Notably, this study shows that the intensity of the frequency converted light is maximized when the duration of the index perturbation is matched to the cavity storage time. The results provide a set of optimum parameters for increasing frequency conversion efficiency inside a microcavity.